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1. Fast neutron background characterization of the future Ricochet experiment at the ILL research nuclear reactor

   https://doi.org/10.1140/epjc/s10052-022-11150-x  

   Augier, C. ; Baulieu, G. ; Belov, V. ; Berge, L. ; Billard, J. ; Bres, G. ; Bret, J-. L. ; Broniatowski, A. ; Calvo, M. ; Cazes, A. ; et al ( January 2023 , The European Physical Journal C)

   The futureRicochetexperiment aims at searching for new physics in the electroweak sector by providing a high precision measurement of the Coherent Elastic Neutrino-Nucleus Scattering (CENNS) process down to the sub-100 eV nuclear recoil energy range. The experiment will deploy a kg-scale low-energy-threshold detector array combining Ge and Zn target crystals 8.8 m away from the 58 MW research nuclear reactor core of the Institut Laue Langevin (ILL) in Grenoble, France. Currently, theRicochetCollaboration is characterizing the backgrounds at its future experimental site in order to optimize the experiment’s shielding design. The most threatening background component, which cannot be actively rejected by particle identification, consists of keV-scale neutron-induced nuclear recoils. These initial fast neutrons are generated by the reactor core and surrounding experiments (reactogenics), and by the cosmic rays producing primary neutrons and muon-induced neutrons in the surrounding materials. In this paper, we present theRicochetneutron background characterization using$$^3$$${}^3$He proportional counters which exhibit a high sensitivity to thermal, epithermal and fast neutrons. We compare these measurements to theRicochetGeant4 simulations to validate our reactogenic and cosmogenic neutron background estimations. Eventually, we present our estimated neutron background for the futureRicochetexperiment and the resulting CENNS detection significance. Our results show that depending on the effectiveness of the muon veto, we expect a total nuclear recoil background rate between 44 ± 3 and 9 ± 2 events/day/kg in the CENNS region of interest, i.e. between 50 eV and 1 keV. We therefore found that theRicochetexperiment should reach a statistical significance of 4.6 to 13.6 $$\sigma $$$\sigma$for the detection of CENNS after one reactor cycle, when only the limiting neutron background is considered.

    

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2. Evaluation of gadolinium’s action on water Cherenkov detector systems with EGADS

   https://doi.org/10.1016/j.nima.2020.163549  

   Marti, LI ; et, al ( January 2020 , Nuclear instruments methods n physics research)

   Used for both proton decay searches and neutrino physics, large water Cherenkov (WC) detectors have been very successful tools in particle physics. They are notable for their large masses and charged particle detection capabilities. While current WC detectors reconstruct charged particle tracks over a wide energy range, they cannot efficiently detect neutrons. Gadolinium (Gd) has the largest thermal neutron capture cross section of all stable nuclei and produces an 8 MeV gamma cascade that can be detected with high efficiency. Because of the many new physics opportunities that neutron tagging with a Gd salt dissolved in water would open up, a large-scale R&D; program called EGADS was established to demonstrate this technique’s feasibility. EGADS features all the components of a WC detector, chiefly a 200-ton stainless steel water tank furnished with 240 photo-detectors, DAQ, and a water system that removes all impurities from water while keeping Gd in solution. In this paper we discuss the milestones towards demonstrating the feasibility of this novel technique, and the features of EGADS in detail. 

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3. Photovoltaic Response of Thin-Film CdTe Solar Cells under Accelerated Neutron Radiation in a TRIGA Reactor

   Powell, Kaden ; Lund, Matthew ; Wang, Meng-Jen ; Qian, Yang ; Magginetti, David ; Reese, Matthew ; Cazalas, Edward ; Sjoden, Glenn ; Yoon, Heayoung ( June 2020 , Electronic Materials Symposium)

   Cadmium telluride (CdTe) solar cells are a promising photovoltaic (PV) technology for producing power in space owing to their high-efficiency (> 22.1 %), potential for specific power, and cost-effective manufacturing processes. In contrast to traditional space PVs, the high-Z (atomic number) CdTe absorbers can be intrinsically robust under extreme space radiation, offering long-term stability. Despite these advantages, the performance assessment of CdTe solar cells under high-energy particle irradiation (e.g., photons, neutrons, charged particles) is limited in the literature, and their stability is not comprehensively studied. In this work, we present the PV response of n-CdS / p-CdTe PVs under accelerated neutron irradiation. We measure PV properties of the devices at different neutron/photon doses. The equivalent dose deposited in the CdTe samples is simulated with deterministic and Monte Carlo radiation transport methods. Thin-film CdTe solar cells were synthesized on a fluorine-doped tin oxide (FTO) coated glass substrate (≈ 4 cm × 4 cm). CdS:O (≈ 100 nm) was reactively RF sputtered in an oxygen/argon ambient followed by a close-spaced sublimation deposition of CdTe (≈ 3.5 μm) in an oxygen/helium ambient. The sample was exposed to a 10 min vapor CdCl2 in oxygen/helium ambient at 430˚C. The samples were exposed to a wet CuCl2 solution prior to anneal 200ºC. A gold back-contact was formed on CdTe via thermal evaporation. The final sample contains 16 CdTe devices. For neutron irradiation, we cleaved the CdTe substrate into four samples and exposed two samples to ≈ 90 kW reactor power neutron radiation for 5.5 hours and 8.2 hours, respectively, in our TRIGA (Training, Research, Isotopes, General Atomics) reactor. We observed a noticeable color change of the glass substrates to brown after the neutron/gamma reactor exposure. Presumably, the injected high-energy neutrons caused the breaking of chemical bonds and the displacement of atoms in the glass substrates, creating point defects and color centers. The I-V characteristics showed noticeable deterioration with over 8 hour radiations. Specifically, the saturation current of the control devices was ≈ 25 nA increasing to 1 μA and 10 μA for the 5.5-hour and 8.2-hour radiated samples, respectively. The turn-on voltage of the control devices (≈ 0.85 V) decreased with the irradiated sample (≈ 0.75 V for 5.5-hour and ≈ 0.5 V for 8.2-hour exposures), implying noticeable radiation damage occurred at the heterojunction. The higher values of the ideality factor for irradiated devices (n > 2.2) compared to that of the control devices (n ≈ 1.3) also support the deterioration of the p-n junction. We observed the notable decrease in shunt resistance (RSH) and the increase in series resistance (Rs) with the neutron dose. It is possible that Cu ions introduced during the CuCl2 treatment may migrate into CdTe grain boundaries (GBs). The presence of Cu ions at GBs can create additional leakage paths for photocarrier transport, deteriorating the overall PV performance. We estimated the radiation dose of CdTe in comparison to Si (conventional PV) using a UUTR model (e.g., MCNP6 2D UTR Reactor simulations). In this model, we simulated Si and CdTe at the center point of the triangular fuel lattice and used an “unperturbed flux” tally in the water. Our simulations yielded a dose rate of 6916 Gy/s of neutrons and 16 Gy/s of photons for CdTe, and 1 Gy/s of neutrons and 21 Gy/s of photons for Si (doses +/- <1%). The large dose rate of neutrons in CdTe is mainly attributed to the large thermal neutron absorption cross-section of 113Cd. Based on this estimation, we calculate that the exposure of our CdTe PVs is equivalent to several million years in LEO (Low-Earth Orbit), or about 10,000 years for Si in LEO. Currently, we are working on a low-dose neutron/photon radiation on CdTe PVs and their light I-Vs and microstructural characterizations to gain better understanding on the degradation of CdTe PVs. 

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4. Fundamental Neutron Physics at Spallation Sources

   https://doi.org/10.1146/annurev-nucl-121521-051029  

   Fomin, Nadia ; Fry, Jason ; Pattie, Robert W. ; Greene, Geoffrey L. ( September 2022 , Annual Review of Nuclear and Particle Science)

   Low-energy neutrons have been a useful probe in fundamental physics studies for more than 70 years. With advances in accelerator technology, many new sources are spallation based. These new, high-flux facilities are becoming the sites for many next-generation fundamental neutron physics experiments. In this review, we present an overview of the sources and the current and upcoming fundamental neutron physics programs. 

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5. Neutron imaging for paleontology

   Hall, Alexander S. ; Bevitt, Joseph ; Garbe, Ulf ; Hunter, James F ; Nelson, Ron ; Williamson, Thomas ( October 2021 , Journal of Vertebrate Paleontology, Program and Abstracts)

   X-ray radiography and computed tomography (CT) reveal hidden subsurface features within fossil specimens embedded in matrix. With X-rays, distinguishing features from the background (i.e., contrast) results from sample density and atomic X-ray attenuation—fundamental properties of the sample. However, even high energy X-rays may poorly resolve hard and soft tissue structures when the matrix has similar density or X-ray attenuation to the fossil. Here, neutron radiography and neutron tomography complement X-ray imaging, as the source of contrast comes instead from how a neutron beam interacts with the sample's atomic nuclei. The contrast is highly nonlinear across the periodic table, and so researchers can see enhanced contrast between adjacent features when X-ray imaging could not. As the signal source is completely different than X-ray imaging, some intuition from X-rays must be discarded. For instance, neutrons quite easily pass through lead, but are blocked by hydrogen. Since neutron imaging is uncommon within paleontology, we introduce this exciting technology at a high level with an emphasis on applications to paleontology. We cover some basic physics underlying neutron imaging, where one can perform such experiments, and sample considerations. The neutron source, concepts of beam flux, and image resolution will also be covered. As neutron imaging typically complements X-ray imaging, we discuss how to digitally combine modalities for segmentation and inference. We present examples of how neutron imaging informed fossil descriptions. This includes the skull of a Paleocene mammal Tetraclaenodon from New Mexico and a variety of Permian vertebrate specimens from Richards Spur, Oklahoma and imaged at the DINGO nuclear imaging facility in Australia. Though neutron sources will always be difficult to access, we aim to assist interested researchers considering this exciting imaging technology for their paleontology research. 

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