Unidirectionally propagated electromagnetic waves are rare in nature but heavily sought after due to their potential applications in backscatter-free optical information processing setups. It was theoretically shown that the distinct bulk optical band topologies of a gyrotropic metal and an isotropic metal can enable topologically protected unidirectional surface plasmon polaritons (SPPs) at their interface. Here, we experimentally identify such interfacial modes at terahertz frequencies. Launching the interfacial SPPs via a tailored grating coupler, the far-field spectroscopy data obtained reveals strongly nonreciprocal SPP dispersions that are highly consistent with the theoretical predictions. The directionality of the interfacial SPPs studied here is flexibly tunable by either varying the external field or adjusting the metallic characteristics of the bulk materials. The experimental realization of actively tunable unidirectional SPPs sets the foundation for developing nanophotonic information processing devices based on topologically protected interfacial waves.
Titanium nitride (TiN) has been identified as a promising refractory material for high temperature plasmonic applications such as surface plasmon polaritons (SPPs) waveguides, lasers and light sources, and near field optics. Such SPPs are sensitive not only to the highly metallic nature of the TiN, but also to its low loss. We have formed highly metallic, low-loss TiN thin films on MgO substrates to create SPPs with resonances between 775-825 nm. Scanning near-field optical microscopy (SNOM) allowed imaging of the SPP fringes, the accurate determination of the effective wavelength of the SPP modes, and propagation lengths greater than 10 microns. Further, we show the engineering of the band structure of the plasmonic modes in TiN in the mid-IR regime and experimentally demonstrate, for the first time, the ability of TiN to support Spoof Surface Plasmon Polaritons in the mid-IR (6 microns wavelength).
- Publication Date:
- NSF-PAR ID:
- 10146930
- Journal Name:
- Optics Express
- Volume:
- 28
- Issue:
- 10
- Page Range or eLocation-ID:
- Article No. 14536
- ISSN:
- 1094-4087; OPEXFF
- Publisher:
- Optical Society of America
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract Spectrally narrow optical resonances can be used to generate slow light, i.e., a large reduction in the group velocity. In a previous work, we developed hybrid 2D semiconductor plasmonic structures, which consist of propagating optical frequency surface-plasmon polaritons interacting with excitons in a semiconductor monolayer. Here, we use coupled exciton-surface plasmon polaritons (E-SPPs) in monolayer WSe 2 to demonstrate slow light with a 1300 fold decrease of the SPP group velocity. Specifically, we use a high resolution two-color laser technique where the nonlinear E-SPP response gives rise to ultra-narrow coherent population oscillation (CPO) resonances, resulting in a group velocity on order of 10 5 m/s. Our work paves the way toward on-chip actively switched delay lines and optical buffers that utilize 2D semiconductors as active elements.
-
Probe is the core component of an optical scanning probe microscope such as scattering-type scanning near-field optical microscopy (s-SNOM). Its ability of concentrating and localizing light determines the detection sensitivity of nanoscale spectroscopy. In this paper, a novel plasmonic probe made of a gradient permittivity material (GPM) is proposed and its nanofocusing performance is studied theoretically and numerically. Compared with conventional plasmonic probes, this probe has at least two outstanding advantages: First, it doesn't need extra structures for surface plasmon polaritons (SPPs) excitation or localized surface plasmon resonance (LSPR), simplifying the probe system; Second, the inherent nanofocusing effects of the conical probe structure can be further reinforced dramatically by designing the distribution of the probe permittivity. As a result, the strong near-field enhancement and localization at the tip apex improve both spectral sensitivity and spatial resolution of a s-SNOM. We also numerically demonstrate that a GPM probe as well as its enhanced nanofocusing effects can be realized by conventional semiconductor materials with designed doping distributions. The proposed novel plasmonic probe promises to facilitate subsequent nanoscale spectroscopy applications.
-
Geometric diodes represent a relatively new class of diodes used in rectennas that rely on the asymmetry of a conducting thin film. Here, we numerically investigate a plasmonic analogue of geometric diodes to realize nanoscale optical asymmetric transmission. The device operates based on spatial symmetry breaking that relies on a unique property of surface plasmon polaritons (SPPs), namely, adiabatic nanofocusing. We show that the structure can realize on-chip asymmetric electromagnetic transmission with a total dimension of
. We demonstrate a signal contrast of 0.7 and an asymmetric optical transmission ratio of 4.77 dB. We investigate the origin of the asymmetric transmission and show that it is due mainly to asymmetric out-coupling of SPPs to far-field photons. We highlight the role of evanescent field coupling of SPPs in undermining the asymmetric transmission efficiency and show that by adjusting the plasmonic waveguide dimensions, a signal contrast of 0.94 and an asymmetric optical transmission ratio of 5.18 dB can be obtained. Our work presents a new paradigm for on-chip nanoscale asymmetric optical transmission utilizing the unique properties of SPPs. -
The infrared (IR) gas sensing technique is excellent for CO 2 gas detection systems that require high accuracy and safety standard; however, there is a significant barrier to its application due to its high cost and difficulty in miniaturization. CO 2 sensors that are functional within near- or short-wavelength IR have the potential to reduce this barrier. In this work, a highly sensitive plasmonic material based on nanostructured covellite copper sulfide (CuS), which exhibits desired localized surface plasmon resonance for surface-enhanced IR absorption (SEIRA) throughout near- and mid-IR ranges, was investigated. We prepared CuS thin films facilely in an additive manner based on a spatial successive ionic layer adsorption and reaction process at room temperature. The resulting CuS thin film possesses a structure consisting of hexagonal nanoflakes, and demonstrates significant SEIRA for 100 ppm CO 2 with an enhancement factor of 10 4 .
