More Like this

1. The metastable Q ³ Δ ₂ state of ThO: a new resource for the ACME electron EDM search

   https://doi.org/10.1088/1367-2630/ab6a3a  

   Wu, X. ; Han, Z. ; Chow, J. ; Ang, D. G. ; Meisenhelder, C. ; Panda, C. D. ; West, E. P. ; Gabrielse, G. ; Doyle, J. M. ; DeMille, D. ( February 2020 , New Journal of Physics)

   The best upper limit for the electron electric dipole moment was recently set by the ACME collaboration. This experiment measures an electron spin-precession in a cold beam of ThO molecules in their metastable$H{(}^3{\mathrm{\Delta }}_1)$state. Improvement in the statistical and systematic uncertainties is possible with more efficient use of molecules from the source and better magnetometry in the experiment, respectively. Here, we report measurements of several relevant properties of the long-lived$Q{(}^3{\mathrm{\Delta }}_2)$state of ThO, and show that this state is a very useful resource for both these purposes. TheQstate lifetime is long enough that its decay during the time of flight in the ACME beam experiment is negligible. The large electric dipole moment measured for theQstate, giving rise to a large linear Stark shift, is ideal for an electrostatic lens that increases the fraction of molecules detected downstream. The measured magnetic moment of theQstate is also large enough to be used as a sensitive co-magnetometer in ACME. Finally, we show that theQstate has a large transition dipole moment to the$C{(}^1{\mathrm{\Pi }}_1)$state, which allows for efficient population transfer between the ground statewidth='0.50em'/>(1Σ+)and theQstate via$X-C-Q$Stimulated Raman Adiabatic Passage (STIRAP). We demonstrate 90 % STIRAP transfer efficiency. In the course of these measurements, we also determine the magnetic moment ofCstate, the$X\to C$transition dipole moment, and branching ratios of decays from theCstate.

   « less
2. Intermediate valence state in YbB ₄ revealed by resonant x-ray emission spectroscopy

   https://doi.org/10.1088/1361-648X/ac7629  

   Frontini, Felix ; Lebert, Blair W. ; Cho, K. K. ; Song, M. S. ; Cho, B. K. ; Pollock, Christopher J. ; Kim, Young-June ( June 2022 , Journal of Physics: Condensed Matter)

   We report the temperature dependence of the Yb valence in the geometrically frustrated compound${\mathrm{Y}\mathrm{b}\mathrm{B}}_4$from 12 to 300 K using resonant x-ray emission spectroscopy at the Yb$L_{{\alpha }_1}$transition. We find that the Yb valence,v, is hybridized between thev = 2 andv = 3 valence states, increasing from$v=2.61\pm 0.01$at 12 K to$v=2.67\pm 0.01$at 300 K, confirming that${\mathrm{Y}\mathrm{b}\mathrm{B}}_4$is a Kondo system in the intermediate valence regime. This result indicates that the Kondo interaction in${\mathrm{Y}\mathrm{b}\mathrm{B}}_4$is substantial, and is likely to be the reason why${\mathrm{Y}\mathrm{b}\mathrm{B}}_4$does not order magnetically at low temperature, rather than this being an effect of geometric frustration. Furthermore, the zero-point valence of the system is extracted from our data and compared with other Kondo lattice systems. The zero-point valence seems to be weakly dependent on the Kondo temperature scale, but not on the valence change temperature scaleT_v.
3. Formation and evolution of post-solitons following a high intensity laser-plasma interaction with a low-density foam target

   https://doi.org/10.1088/1361-6587/abf85c  

   Blackman, David R. ; Adak, Amitava ; Singh, Prashant K. ; Lad, Amit D. ; Chatterjee, Gourab ; Ridgers, Christopher P. ; Del Sorbo, Dario ; Trines, Raoul M. G. M. ; Robinson, A. P. L. ; Nazarov, Wigen ; et al ( May 2021 , Plasma Physics and Controlled Fusion)

   The formation and evolution of post-solitons has been discussed for quite some time both analytically and through the use of particle-in-cell (PIC) codes. It is however only recently that they have been directly observed in laser-plasma experiments. Relativistic electromagnetic (EM) solitons are localised structures that can occur in collisionless plasmas. They consist of a low-frequency EM wave trapped in a low electron number-density cavity surrounded by a shell with a higher electron number-density. Here we describe the results of an experiment in which a 100 TW Ti:sapphire laser (30 fs, 800 nm) irradiates a$0.03\mathrm{g}\mathrm{c}{\mathrm{m}}^{-3}$TMPTA foam target with a focused intensity$I_{\mathrm{l}}=9.5\times {10}^{17}\mathrm{W}\mathrm{c}{\mathrm{m}}^{-2}$. A third harmonic (${\lambda }_{\mathrm{p}\mathrm{r}\mathrm{o}\mathrm{b}\mathrm{e}}\simeq 266$nm) probe is employed to diagnose plasma motion for 25 ps after the main pulse interaction via Doppler-Spectroscopy. Both radiation-hydrodynamics and 2D PIC simulations are performed to aid in the interpretation of the experimental results. We show that the rapid motion of the probe critical-surface observed in the experiment might be a signature of post-soliton wall motion.
4. Enhanced cavity coupling to silicon vacancies in 4H silicon carbide using laser irradiation and thermal annealing

   https://doi.org/10.1073/pnas.2021768118  

   Gadalla, Mena N. ; Greenspon, Andrew S. ; Defo, Rodrick Kuate ; Zhang, Xingyu ; Hu, Evelyn L. ( March 2021 , Proceedings of the National Academy of Sciences)

   The negatively charged silicon monovacancy${\mathrm{V}}_{\text{Si}}^{-}$in 4H silicon carbide (SiC) is a spin-active point defect that has the potential to act as a qubit in solid-state quantum information applications. Photonic crystal cavities (PCCs) can augment the optical emission of the${\mathrm{V}}_{\text{Si}}^{-}$, yet fine-tuning the defect–cavity interaction remains challenging. We report on two postfabrication processes that result in enhancement of the$\mathrm{V}1\prime$optical emission from our PCCs, an indication of improved coupling between the cavity and ensemble of silicon vacancies. Below-bandgap irradiation at 785-nm and 532-nm wavelengths carried out at times ranging from a few minutes to several hours results in stable enhancement of emission, believed to result from changing the relative ratio of${\mathrm{V}}_{\text{Si}}^0$(“dark state”) to${\mathrm{V}}_{\text{Si}}^{-}$(“bright state”). The much faster change effected by 532-nm irradiation may result from cooperative charge-state conversion due to proximal defects. Thermal annealing at 100 °C, carried out over 20 min, also results in emission enhancements and may be explained by the relatively low-activation energy diffusion of carbon interstitials${\mathrm{C}}_{\mathrm{i}}$, subsequently recombining with other defects to create additional${\mathrm{V}}_{\text{Si}}^{-}$s. These PCC-enabled experiments reveal insights into defect modifications and interactions within a controlled, designated volume and indicate pathways tomore »improved defect–cavity interactions.

   « less
5. Optical spectral weight, phase stiffness, and T _c bounds for trivial and topological flat band superconductors

   https://doi.org/10.1073/pnas.2106744118  

   Verma, Nishchhal ; Hazra, Tamaghna ; Randeria, Mohit ( August 2021 , Proceedings of the National Academy of Sciences)

   We present exact results that give insight into how interactions lead to transport and superconductivity in a flat band where the electrons have no kinetic energy. We obtain bounds for the optical spectral weight for flat-band superconductors that lead to upper bounds for the superfluid stiffness and the two-dimensional (2D)$T_c$. We focus on on-site attraction$\left|U\right|$on the Lieb lattice with trivial flat bands and on the π-flux model with topological flat bands. For trivial flat bands, the low-energy optical spectral weight${\tilde{D}}_{\text{low}}\le \tilde{n}\left|U\right|\mathrm{\Omega }/2$with$\tilde{n}=min\left(n,2-n\right)$, where n is the flat-band density and Ω is the Marzari–Vanderbilt spread of the Wannier functions (WFs). We also obtain a lower bound involving the quantum metric. For topological flat bands, with an obstruction to localized WFs respecting all symmetries, we again obtain an upper bound for${\tilde{D}}_{low}$linear in$\left|U\right|$. We discuss the insights obtained from our bounds by comparing them with mean-field and quantum Monte Carlo results.