skip to main content


Title: All-fiber single-cavity dual-comb for coherent anti-Stokes Raman scattering spectroscopy based on spectral focusing

We report an all-fiber free-running bidirectional dual-comb laser system for coherent anti-Stokes Raman scattering spectroscopy based on spectral focusing. The mode-locked oscillator is a bidirectional ring-cavity erbium fiber laser running at a repetition rate of∼<#comment/>114MHz. One output of the bidirectional laser is wavelength-shifted from 1560 to 1060 nm via supercontinuum generation for use as the pump source. We have been able to record the Raman spectra of various samples such as polystyrene, olive oil, polymethyl methacrylate (PMMA), and polyethylene in the C–H stretching window. We believe that this all-fiber laser design has promising potential for coherent Raman spectroscopy and also label-free imaging for a variety of practical applications.

 
more » « less
NSF-PAR ID:
10207274
Author(s) / Creator(s):
; ; ;
Publisher / Repository:
Optical Society of America
Date Published:
Journal Name:
Optics Letters
Volume:
46
Issue:
1
ISSN:
0146-9592; OPLEDP
Page Range / eLocation ID:
Article No. 146
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. The counterpropagating all-normal dispersion (CANDi) fiber laser is an emerging high-energy single-cavity dual-comb laser source. Its relative timing jitter (RTJ), a critical parameter for dual-comb timing precision and spectral resolution, has not been comprehensively investigated. In this paper, we enhance the state-of-the-art CANDi fiber laser pulse energy from 1 nJ to 8 nJ. We then introduce a reference-free RTJ characterization technique that provides shot-to-shot measurement capability at femtosecond precision. The measurement noise floor reaches1.6×<#comment/>10−<#comment/>7fs2/Hz, and the corresponding integrated measurement precision is only 1.8 fs (1 kHz, 20 MHz). With this characterization tool, we are able to study the physical origin of the CANDi laser’s RTJ in detail. We first verify that the cavity length fluctuation does not contribute to the RTJ. Then we measure the integrated RTJ to be 39 fs (1 kHz, 20 MHz) and identify the pump relative intensity noise (RIN) to be the dominant factor responsible for it. In particular, pump RIN is coupled to the RTJ through the Gordon–Haus effect. Finally, solutions to reduce the free-running CANDi laser’s RTJ are discussed. This work provides a general guideline to improve the performance of compact single-cavity dual-comb systems such as the CANDi laser, benefitting various dual-comb applications.

     
    more » « less
  2. Soluble, small amyloid-β<#comment/>oligomers (Aβ<#comment/>O) are recognized as significant contributors to the pathology of Alzheimer’s disease (AD). Although drugs for treating AD symptoms have been approved, no therapy targeting amyloid-β<#comment/>(Aβ<#comment/>) capable of modifying the course of the disease is available. In an effort to develop a label-free method for screening new anti-AD therapeutic agents, we show the use of a surface-enhanced Raman scattering (SERS) active substrate for detecting the interactions betweenAβ<#comment/>peptides and spin-labeled fluorine (SLF), a peptide aggregation inhibitor. Changes in the peak positions and intensity ratios of two spectral peaks near1600cm−<#comment/>1and2900cm−<#comment/>1can be used to monitor the molecular interactions between SLF andAβ<#comment/>. This study demonstrates the potential of SERS spectroscopy for rapidly screening and identifying new anti-Aβ<#comment/>therapeutic agents.

     
    more » « less
  3. We experimentally demonstrate the use of a high-coherence hybrid silicon (Si)/III–V semiconductor laser as the light source for a transmitter generating 20 Gbaud 16- and 64- quadrature amplitude modulated (QAM) data signals over an 80 km single-mode fiber (SMF) link. The hybrid Si/III–V laser has a measured Schawlow–Townes linewidth of∼<#comment/>10kHz, which is achieved by storing modal optical energy in low-loss Si, rather than the relatively lossy III–V materials. We measure a received bit error rate (BER) of4.1×<#comment/>10−<#comment/>3when transmitting the 64-QAM data over an 80 km SMF using the hybrid Si/III–V laser. Furthermore, we measure a BER of<<#comment/>1×<#comment/>10−<#comment/>4with the Viterbi–Viterbi digital carrier phase recovery method when transmitting the 16-QAM data over an 80 km SMF using the hybrid Si/III–V laser. This performance is achieved at power penalties lower than those obtained with an exemplary distributed feedback laser and slightly higher than those with an exemplary narrow-linewidth external cavity laser.

     
    more » « less
  4. A study of short-gated 10 nanosecond (ns), 100 picosecond (ps), and 100 femtosecond (fs) laser induced breakdown spectroscopy (LIBS) was conducted for fuel-to-air ratio (FAR) measurements in an atmospheric Hencken flame. The intent of the work is to understand which emission lines are available near the optical range in each pulse width regime and which emission ratios may be favorable for generating equivalence ratio calibration curves. The emission spectra in the range of 550–800 nm for ns-LIBS and ps-LIBS are mostly similar with slightly elevated atomic oxygen lines by ps-LIBS. Spectra from fs-LIBS show the lowest continuum background and prominent individual atomic lines, though have significantly weaker ionic emission from nitrogen. A qualitative explanation based on assumed local thermodynamic equilibrium and electron temperatures calculated by theNII(565nm)andNII(594nm)emissions is presented. In studying line emission ratios for FAR calculation, it is found thatHα<#comment/>(656nm)/NII(568nm)is best for FAR measurements with ns-LIBS and remains viable for ps-LIBS, whileHα<#comment/>(656nm)/OI(777nm)is optimal for the ps-LIBS and fs-LIBS cases. Due to low continuum background and short time delay for spectra collection, fs-LIBS is very promising for high-speed FAR measurements using short-gated LIBS.

     
    more » « less
  5. We investigated the filamentation in air of 7 ps laser pulses of up to 200 mJ energy from a 1.03 μm-wavelength Yb:YAG laser at repetition rates up tof=1kHz. Interferograms of the wake generated show that while pulses in a train of repetition ratef=0.1kHzencounter a nearly unperturbed environment, atf=1kHz, a channel with an axial air density hole of∼<#comment/>20%<#comment/>is generated and maintained at all times by the cumulative effect of preceding laser pulses. Measurements atf=1kHzshow that the energy deposited decreases proportional to the air channel density depletion, becoming more pronounced as the repetition rate and pulse energy increase. Numerical simulations indicate that contrary to filaments generated by shorter duration pulses, the electron avalanche is the dominant energy loss mechanism during filamentation with 7 ps pulses. The results are of interest for the atmospheric propagation of joule-level picosecond pulses from Yb:YAG lasers, of which average powers now surpass 1 kW, and for channeling other directed energy beams.

     
    more » « less