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Broken spatial and time reversal symmetries in materials often give rise to new emergent phenomena in the interaction between light and matter. The combination of chirality and broken time reversal symmetry in a magnetic field leads to magneto–chiral phenomena, such as the nonreciprocity of transmission. Here, we construct a terahertz hybrid metamaterial that combines the natural optical activity of a chiral metallic gammadion bilayer and the magneto-optical activity of semiconductor indium antimonide in a magnetic field. We report a resonant magneto–chiral effect that leads to polarization-independent nonreciprocal optical transmittance. Furthermore, we discover a magneto-optical Faraday effect that is resonantly controlled by the natural optical activity of the chiral gammadion bilayer. Unlike optical activity due to chirality, the novel Faraday effect is odd under time reversal. Both phenomena are activated by a modest magnetic field, which may open doors for their potential applications in polarization-independent optical isolation and highly efficient polarization control at terahertz frequencies.
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Observation of magneto-electric rectification at non-relativistic intensities
Abstract The subject of electromagnetism has often been called electrodynamics to emphasize the dominance of the electric field in dynamic light–matter interactions that take place under non-relativistic conditions. Here we show experimentally that the often neglected optical magnetic field can nevertheless play an important role in a class of optical nonlinearities driven by both the electric and magnetic components of light at modest (non-relativistic) intensities. We specifically report the observation of magneto-electric rectification, a previously unexplored nonlinearity at the molecular level which has important potential for energy conversion, ultrafast switching, nano-photonics, and nonlinear optics. Our experiments were carried out in nanocrystalline pentacene thin films possessing spatial inversion symmetry that prohibited second-order, all-electric nonlinearities but allowed magneto-electric rectification.
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- Award ID(s):
- 1947070
- PAR ID:
- 10213211
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 11
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript
- Journal Article:
- https://doi.org/10.1038/s41467-020-19125-w
