Non-equilibrium photocarriers in multilayer WSe2injected by femtosecond laser pulses exhibit extraordinary nonlinear dynamics in the presence of intense THz fields. The THz absorption in optically excited WSe2rises rapidly in the low THz field regime and gradually ramps up at high intensities. The strong THz pulses drive the photocarriers into sidebands of higher mobility and release trapped charge carriers, which consequently enhance the transient conductivity of WSe2. The spectrally analyzed conductivity reveals distinctive features, indicating that the photocarriers undergo resonant interactions such as carrier-photon scattering.
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Strong-field terahertz control of plasmon induced opacity in photoexcited metamaterial
A terahertz (THz) metamaterial consisting of radiative slot antennas and subradiant complementary split-ring resonators exhibits plasmon induced opacity in a narrow spectral range due to the destructive interference between the bright and dark modes of the coupled oscillators. Femtosecond optical excitations instantly quench the mode coupling and plasmon oscillations, injecting photocarriers into the metamaterial. The plasmon resonances in the coupled metamaterial are restored by intense THz pulses in a subpicoseond time scale. The strong THz fields induce intervalley scattering and interband tunneling of the photocarriers and achieve significant reduction of the photocarrier mobility. The ultrafast dynamics of the nonlinear THz interactions reveals intricate interplay between photocarriers and plasmon oscillations. The high-field THz control of the plasmon oscillations implies potential applications to ultrahigh-speed plasmonics.
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- Award ID(s):
- 1905634
- PAR ID:
- 10216919
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Journal of the Optical Society of America B
- Volume:
- 38
- Issue:
- 4
- ISSN:
- 0740-3224; JOBPDE
- Format(s):
- Medium: X Size: Article No. 1163
- Size(s):
- Article No. 1163
- Sponsoring Org:
- National Science Foundation
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Non-equilibrium photocarriers in multilayer WSe2 injected by femtosecond laser pulses exhibit extraordinary nonlinear dynamics in the presence of intense THz fields. The THz absorption in optically excited WSe2 rises rapidly in the low THz field regime and gradually ramps up at high intensities. The strong THz pulses drive the photocarriers into sidebands of higher mobility and release trapped charge carriers, which consequently enhance the transient conductivity of WSe2. The spectrally analyzed conductivity reveals distinctive features, indicating that the photocarriers undergo resonant interactions such as carrier-photon scattering.more » « less
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