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Jetting dynamics from bursting bubbles play a key role in mediating mass and momentum transport across the air–liquid interface, and have attracted widespread interest from researchers across disciplines. In marine environments, this phenomenon has drawn considerable attention due to its role in releasing biochemical contaminants, such as extracellular polymeric substances, into the atmosphere through aerosol production. These biocontaminants often exhibit non-Newtonian characteristics, yet the physics of bubble bursting with a rheologically complex layer at the bubble–liquid interface remains largely unexplored. In this study, we experimentally investigate the jetting dynamics of bubble bursting events in the presence of such a polymeric compound layer. Using bubbles coated by a polyethylene oxide solution, we document the cavity collapse and jetting dynamics produced by bubble bursting. At a fixed polymer concentration, the jet velocity increases while the jet radius decreases with an increasing compound layer volume fraction, as a result of stronger capillary wave damping due to capillary wave separation at the compound interface as well as the formation of smaller cavity cone angles during bubble cavity collapse. These dynamics produce smaller and more numerous jet drops. Meanwhile, as the polymer concentration increases, the jet velocity decreases while the jet radius increases for the same compound layer fraction due to the increasing viscoelastic stresses. In addition, fewer jet drops are ejected as the jets become slower and broader with increasing polymer concentration, as viscoelastic stresses persist throughout the jet formation and thinning process. We further obtain, for the first time, a regime map delineating the conditions for jet drop ejection versus no jet drop ejection in bursting bubbles coated with a polymeric compound layer. Our results may provide new insights into the mechanisms of mass transport of organic materials in bubble-mediated aerosolization processes, advancing our understanding of marine biology and environmental science.
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Jet Dynamics Associated with Drop Impact on Micropillared Substrate
The jetting phenomenon associated with droplet impact upon a hydrophilic micropillared substrate was analyzed in detail using a high-speed camera. Viscosities of the fluids were varied using differing concentrations of glycerol in deionized water. This paper aims to connect similarities between this form of capillary jetting and another well-known jetting phenomenon from the bubble bursting. Both experience a cavity collapse when opposing fluid fronts collide which causes a singularity at the liquid surface, thus leading to the occurrence of jetting. Following processes used to define scaling laws for bubble bursting, a similar approach was taken to derive scaling laws for the dimensionless jet height, jet radius, base height, and radius of the jet base with respect to dimensionless time for the jetting phenomenon associated with the droplet impact. The development of a top droplet before the breakup of the jet also allows the examination of a scaling law for the necking diameter. We find that with the proper scaling factors, the evolution of the jet profile can collapse into a master profile for different fluids and impact velocities. The time dependence of the necking diameter before the jet breakup follows the power law with an exponent of ~2/3. Contrastingly, for other jet parameters such as the radius and height, the power law relationship with time dependence was not found to have a clear pattern that emerged from these studies.
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- Award ID(s):
- 1701339
- PAR ID:
- 10274020
- Date Published:
- Journal Name:
- Fluids
- Volume:
- 6
- Issue:
- 4
- ISSN:
- 2311-5521
- Page Range / eLocation ID:
- 155
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.3390/fluids6040155
