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1. Highly Efficient Anisotropic Chiral Plasmonic Metamaterials for Polarization Conversion and Detection

   Bai, Jing ; Yao, Yu ( August 2021 , ACS nano)

   null (Ed.)

   Plasmonic chiral metamaterials have attracted broad research interest because of their potential applications in optical communication, biomedical diagnosis, polarization imaging, and circular dichroism spectroscopy. However, optical losses in plasmonic structures severely limit practical applications. Here, we present the design concept and experimental demonstration for highly efficient subwavelength-thick plasmonic chiral metamaterials with strong chirality. The proposed designs utilize plasmonic metasurfaces to control the phase and polarization of light and exploit anisotropic thin-film interference effects to enhance optical chirality while minimizing optical loss. Based on such design concepts, we demonstrated experimentally optical devices such as circular polarization filters with transmission efficiency up to 90% and extinction ratio >180, polarization converters with conversion efficiency up to 90%, as well as on-chip integrated microfilter arrays for full Stokes polarization detection with high accuracy over a broad wavelength range (3.5–5 μm). The proposed design concepts are applicable from near-infrared to Terahertz regions via structural engineering. 

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2. Broadband Enhanced Chirality with Tunable Response in Hybrid Plasmonic Helical Metamaterials

   https://doi.org/10.1002/adfm.202010329  

   Kilic, Ufuk ; Hilfiker, Matthew ; Ruder, Alexander ; Feder, Rene ; Schubert, Eva ; Schubert, Mathias ; Argyropoulos, Christos ( February 2021 , Advanced Functional Materials)

   Designing broadband enhanced chirality is of strong interest to the emerging fields of chiral chemistry and sensing, or to control the spin orbital momentum of photons in recently introduced nanophotonic chiral quantum and classical optical applications. However, chiral light‐matter interactions have an extremely weak nature, are difficult to control and enhance, and cannot be made tunable or broadband. In addition, planar ultrathin nanophotonic structures to achieve strong, broadband, and tunable chirality at the technologically important visible to ultraviolet spectrum still remain elusive. Here, these important problems are tackled by experimentally demonstrating and theoretically verifying spectrally tunable, extremely large, and broadband chiroptical response by nanohelical metamaterials. The reported new designs of all‐dielectric and dielectric‐metallic (hybrid) plasmonic metamaterials permit the largest and broadest ever measured chiral Kuhn's dissymmetry factor achieved by a large‐scale nanophotonic structure. In addition, the strong circular dichroism of the presented bottom‐up fabricated optical metamaterials can be tuned by varying their dimensions and proportions between their dielectric and plasmonic helical subsections. The currently demonstrated ultrathin optical metamaterials are expected to provide a substantial boost to the developing field of chiroptics leading to significantly enhanced and broadband chiral light‐matter interactions at the nanoscale.

    

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3. Chiral Grayscale Imaging with Plasmonic Metasurfaces of Stepped Nanoapertures

   https://doi.org/10.1002/adom.201801467  

   Chen, Yang ; Gao, Jie ; Yang, Xiaodong ( January 2019 , Advanced Optical Materials)

   Optical chiral imaging, as an important tool in chemical and biological analysis, has recently undergone a revolution with the development of chiral metamaterials and metasurfaces. However, the existing chiral imaging approaches based on metamaterials or metasurfaces can only display binary images with 1 bit pixel depth having either black or white pixels. Here, the unique chiral grayscale imaging based on plasmonic metasurfaces of stepped V‐shaped nanoapertures is reported with both high circular dichroism and large polarization linearity in transmission. By interlacing two subarrays of chiral nanoaperture enantiomers into one metasurface, two specific linear polarization profiles are independently generated in transmission under different incident handedness, which can then be converted into two distinct intensity profiles for demonstrating spin‐controlled grayscale images with 8 bit pixel depth. The proposed chiral grayscale imaging approach with subwavelength spatial resolution and high data density provides a versatile platform for many future applications in image encryption and decryption, dynamic display, advanced chiroptical sensing, and optical information processing.

    

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4. Spin-controlled wavefront shaping with plasmonic chiral geometric metasurfaces

   https://doi.org/10.1038/s41377-018-0086-x  

   Chen, Yang ; Yang, Xiaodong ; Gao, Jie ( October 2018 , Light: Science & Applications)

   Metasurfaces, as a two-dimensional (2D) version of metamaterials, have drawn considerable attention for their revolutionary capability in manipulating the amplitude, phase, and polarization of light. As one of the most important types of metasurfaces, geometric metasurfaces provide a versatile platform for controlling optical phase distributions due to the geometric nature of the generated phase profile. However, it remains a great challenge to design geometric metasurfaces for realizing spin-switchable functionalities because the generated phase profile with the converted spin is reversed once the handedness of the incident beam is switched. Here, we propose and experimentally demonstrate chiral geometric metasurfaces based on intrinsically chiral plasmonic stepped nanoapertures with a simultaneously high circular dichroism in transmission (CDT) and large cross-polarization ratio (CPR) in transmitted light to exhibit spin-controlled wavefront shaping capabilities. The chiral geometric metasurfaces are constructed by merging two independently designed subarrays of the two enantiomers for the stepped nanoaperture. Under a certain incident handedness, the transmission from one subarray is allowed, while the transmission from the other subarray is strongly prohibited. The merged metasurface then only exhibits the transmitted signal with the phase profile of one subarray, which can be switched by changing the incident handedness. Based on the chiral geometric metasurface, both chiral metasurface holograms and the spin-dependent generation of hybrid-order Poincaré sphere beams are experimentally realized. Our approach promises further applications in spin-controlled metasurface devices for complex beam conversion, image processing, optical trapping, and optical communications.

    

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5. Observation of a Giant Nonlinear Chiro‐Optical Response in Planar Plasmonic–Photonic Metasurfaces

   https://doi.org/10.1002/adom.201900744  

   Wang, Feng ; Harutyunyan, Hayk ( June 2019 , Advanced Optical Materials)

   Plasmonic nanosystems and metamaterials have recently attracted considerable attention because of their ability to enhance the light–matter interactions. One of such optical phenomena is the chiral‐ or handedness‐dependent response which typically requires 3D samples. Planar structures that can exhibit chiral response are highly desirable because of their facile fabrication, however fundamental challenges arising from the 2D nature of these systems prevent the generation of strong chiro‐optical effects. In this work, giant enhancement of the handedness‐dependent optical response in planar metallic nanostructures is shown by exploring the hybridization of plasmonic–photonic modes in a chiral metasurface. The resulting planar hybrid metasurface exhibits over an order of magnitude difference in nonlinear optical response when illuminated with excitation light of opposite circular polarizations. The unique properties of the hybridized plasmonic–photonic modes are shown to be responsible for the giant chiral nonlinear response. This platform allows to study the fundamental framework of chiral optical effects that arise from the combination of planar chirality and collective interaction of discrete nanosystems.

    

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