skip to main content


Title: Observations and Modeling of Rime Splintering in Southern Ocean Cumuli
Abstract

Recent studies have suggested a correct representation of cloud phase in the Southern Ocean region is important in climate models for an accurate representation of the energy balance. Satellite retrievals indicate many of the clouds are predominantly liquid, despite their low temperatures. However, clouds containing high numbers of ice crystals have sometimes been observed in this region and implicated the secondary ice production process called rime splintering. This study re‐examines rime splintering in Southern Ocean cumuli using both a new data set and high‐resolution numerical modeling. Measurements acquired during the Southern Ocean Clouds Radiation Aerosol Transport Experimental Study (SOCRATES) provide an evaluation of the amount of ice in shallow cumuli sampled over two days in this region. The measurements sometimes exhibit seven orders of magnitude or more ice particles compared to amounts expected from measurements of ice‐nucleating particles (INP) on the same days. Cumuli containing multiple updrafts had the greatest tendency to contain high ice concentrations and meet the expected conditions for rime splintering. Idealized numerical modeling, constrained by the observations, suggests that the multiple updrafts produce more frozen raindrops/graupel, and allow them to travel through the rime‐splintering zone over an extended period of time, increasing the number of ice particles by many orders of magnitude. The extremely low number of INP in the Southern Ocean thus appears to require special conditions like multiple updrafts to help glaciate the cumuli in this region, potentially explaining the predominance of supercooled cumuli observed there.

 
more » « less
Award ID(s):
1660486
NSF-PAR ID:
10446114
Author(s) / Creator(s):
 ;  ;  ;  ;  ;  ;  ;  
Publisher / Repository:
DOI PREFIX: 10.1029
Date Published:
Journal Name:
Journal of Geophysical Research: Atmospheres
Volume:
126
Issue:
23
ISSN:
2169-897X
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    Maritime boundary‐layer clouds over the Southern Ocean (SO) have a large shortwave radiative effect. Yet, climate models have difficulties in representing these clouds and, especially, their phase in this observationally sparse region. This study aims to increase the knowledge of SO cloud phase by presenting in‐situ cloud microphysical observations from the Southern Ocean Clouds, Radiation, Aerosol, Transport Experimental Study (SOCRATES). We investigate the occurrence of ice in summertime marine stratocumulus and cumulus clouds in the temperature range between 6 and −25°C. Our observations show that in ice‐containing clouds, maximum ice number concentrations of up to several hundreds per liter were found. The observed ice crystal concentrations were on average one to two orders of magnitude higher than the simultaneously measured ice nucleating particle (INP) concentrations in the temperature range below −10°C and up to five orders of magnitude higher than estimated INP concentrations in the temperature range above −10°C. These results highlight the importance of secondary ice production (SIP) in SO summertime marine boundary‐layer clouds. Evidence for rime splintering was found in the Hallett‐Mossop (HM) temperature range but the exact SIP mechanism active at lower temperatures remains unclear. Finally, instrument simulators were used to assess simulated co‐located cloud ice concentrations and the role of modeled HM rime‐splintering. We found that CAM6 is deficient in simulating number concentrations across the HM temperature range with little sensitivity to the model HM process, which is inconsistent with the aforementioned observational evidence of highly active SIP processes in SO low‐level clouds.

     
    more » « less
  2. Abstract

    In clouds containing both liquid and ice with temperatures between −3°C and −8°C, liquid droplets collide with large ice crystals, freeze, and shatter, producing a plethora of small ice splinters. This process, known as Hallett‐Mossop rime splintering, and other forms of secondary ice production, can cause clouds to reflect less sunlight and to have shorter lifetimes. We show its impact on Southern Ocean shallow cumuli using a novel suite of five global storm‐resolving simulations, which partition the Earth's atmosphere into 2–4 km wide columns. We evaluate simulated clouds and radiation over the Southern Ocean with aircraft observations from the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES), and satellite observations from Clouds and the Earth's Radiant Energy System (CERES) and Himawari. Simulations with large concentrations of ice crystals in boundary layer clouds, which agree better with SOCRATES observations, have reduced mixed‐phase cumulus cloud cover and weaker shortwave cloud radiative effects (CREs) that are less biased compared with CERES. Using a pair of simulations differing only in their treatment of Hallett‐Mossop rime splintering, we show that including this process increases ice crystal concentrations in cumulus clouds and weakens shortwave CREs over the Southern Ocean by 10 W m−2. We also demonstrate the key role that global storm‐resolving models can play in detangling the effects of clouds on Earth's climate across scales, making it possible to trace the impact of changes in individual cumulus cloud anvils (10 km2) on the radiative budget of the massive Southern Ocean basin (107 km2).

     
    more » « less
  3. Abstract

    Oceans are, generally, relatively weak sources of ice nucleating particles (INPs). Thus, dust transported from terrestrial regions can dominate atmospheric INP concentrations even in remote marine regions. Studies of ocean‐emitted INPs have focused upon sea spray aerosols containing biogenic species. Even though large concentrations of dust are transported over marine regions, resuspended dust has never been explicitly considered as another possible source of ocean‐emitted INPs. Current models assume that deposited dust is not re‐emitted from surface waters. Our laboratory studies of aerosol particles produced from coastal seawater and synthetic seawater doped with dust show that dust can indeed be ejected from water during bubble bursting. INP concentration measurements show these ejected dust particles retain ice nucleating activity. Doping synthetic seawater to simulate a strong dust deposition event produced INPs active at temperatures colder than −13°C and INP concentrations 1 to 2 orders of magnitude greater than either lab sea spray or marine boundary layer measurements. The relevance of these laboratory findings is highlighted by single‐particle composition measurements along the Californian coast where at least 9% of dust particles were mixed with sea salt. Additionally, global modeling studies show that resuspension of dust from the ocean could exert the most impact over the Southern Ocean, where ocean‐emitted INPs are thought to dominate atmospheric INP populations. More work characterizing the factors governing the resuspension of dust particles is required to understand the potential impact upon clouds.

     
    more » « less
  4. Abstract

    Global climate models (GCMs) are challenged by difficulties in simulating cloud phase and cloud radiative effect over the Southern Ocean (SO). Some of the new‐generation GCMs predict too much liquid and too little ice in mixed‐phase clouds. This misrepresentation of cloud phase in GCMs results in weaker negative cloud feedback over the SO and a higher climate sensitivity. Based on a model comparison with observational data obtained during the Southern Ocean Cloud Radiation and Aerosol Transport Experimental Study, this study addresses a key uncertainty in the Community Earth System Model version 2 (CESM2) related to cloud phase, namely ice formation in pristine remote SO clouds. It is found that sea spray organic aerosols (SSOAs) are the most important type of ice nucleating particles (INPs) over the SO with concentrations 1 order of magnitude higher than those of dust INPs based on measurements and CESM2 simulations. Secondary ice production (SIP) which includes riming splintering, rain droplet shattering, and ice‐ice collisional fragmentation as implemented in CESM2 is the dominant ice production process in moderately cold clouds with cloud temperatures greater than −20°C. SIP enhances the in‐cloud ice number concentrations (Ni) by 1–3 orders of magnitude and predicts more mixed‐phase (with percentage occurrence increased from 15% to 21%), in better agreement with the observations. This study highlights the importance of accurately representing the cloud phase over the pristine remote SO by considering the ice nucleation of SSOA and SIP processes, which are currently missing in most GCM cloud microphysics parameterizations.

     
    more » « less
  5. Abstract. Cirrus clouds that form in the tropical tropopause layer(TTL) can play a key role in vertical transport through the uppertroposphere and lower stratosphere, which can significantly impact theradiative energy budget and stratospheric chemistry. However, the lack ofrealistic representation of natural ice cloud habits in microphysicalparameterizations can lead to uncertainties in cloud-related processes andcloud–climate feedbacks. The main goal of this study is to investigate therole of different cloud regimes and the associated ice habits in regulatingthe properties of the TTL. We compare aircraft measurements from theStratoClim field campaign to a set of numerical experiments at the scale of large-eddy simulations (LESs) for the same case study that employ differentmicrophysics schemes. Aircraft measurements over the southern slopes of theHimalayas captured high ice water content (HIWC) up to 2400 ppmv and iceparticle aggregates exceeding 700 µm in size with unusually longresidence times. The observed ice particles were mainly of liquid origin,with a small amount formed in situ. The corresponding profile of ice water content (IWC) fromthe ERA5 reanalysis corroborates the presence of HIWC detrained from deep-convective plumes in the TTL but underestimates HIWC by an order ofmagnitude. In the TTL, only the scheme that predicts ice habits canreproduce the observed HIWC, ice number concentration, and bimodal iceparticle size distribution. The lower range of particle sizes is mostlyrepresented by planar and columnar habits, while the upper range isdominated by aggregates. Large aggregates with sizes between 600 and 800 µm have fall speeds of less than 20 cm s−1, which explains thelong residence time of the aggregates in the TTL. Planar ice particles ofliquid origin contribute substantially to HIWC. The columnar and aggregatehabits are in the in situ range with lower IWC and number concentrations. Forall habits, the ice number concentration increases with decreasingtemperature. For the planar ice habit, relative humidity is inverselycorrelated with fall speed. This correlation is less evident for the othertwo ice habits. In the lower range of supersaturation with respect to ice,the columnar habit has the highest fall speed. The difference in ice numberconcentration across habits can be up to 4 orders of magnitude, withaggregates occurring in much smaller numbers. We demonstrate and quantifythe linear relationship between the differential sedimentation of pristineice crystals and the size of the aggregates that form when pristine crystalscollide. The slope of this relationship depends on which pristine ice habitsediments faster. Each simulated ice habit is associated with distinctradiative and latent heating rates. This study suggests that a modelconfiguration nested down to LES scales with a microphysicalparameterization that predicts ice shape evolution is crucial to provide anaccurate representation of the microphysical properties of TTL cirrus andthus the associated (de)hydration process. 
    more » « less