skip to main content


Title: Anomalous metals: From “failed superconductor” to “failed insulator”
Resistivity saturation is found on both superconducting and insulating sides of an “avoided” magnetic-field-tuned superconductor-to-insulator transition (H-SIT) in a two-dimensional In/InO x composite, where the anomalous metallic behavior cuts off conductivity or resistivity divergence in the zero-temperature limit. The granular morphology of the material implies a system of Josephson junctions (JJs) with a broad distribution of Josephson coupling E J and charging energy E C , with an H-SIT determined by the competition between E J and E C . By virtue of self-duality across the true H-SIT, we invoke macroscopic quantum tunneling effects to explain the temperature-independent resistance where the “failed superconductor” side is a consequence of phase fluctuations and the “failed insulator” side results from charge fluctuations. While true self-duality is lost in the avoided transition, its vestiges are argued to persist, owing to the incipient duality of the percolative nature of the dissipative path in the underlying random JJ system.  more » « less
Award ID(s):
1808385
NSF-PAR ID:
10348815
Author(s) / Creator(s):
; ;
Date Published:
Journal Name:
Proceedings of the National Academy of Sciences
Volume:
119
Issue:
29
ISSN:
0027-8424
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    Many experiments investigating magnetic-field tuned superconductor-insulator transition (H-SIT) often exhibit low-temperature resistance saturation, which is interpreted as an anomalous metallic phase emerging from a ‘failed superconductor’, thus challenging conventional theory. Here we study a random granular array of indium islands grown on a gateable layer of indium-oxide. By tuning the intergrain couplings, we reveal a wide range of magnetic fields where resistance saturation is observed, under conditions of careful electromagnetic filtering and within a wide range of linear response. Exposure to external broadband noise or microwave radiation is shown to strengthen the tendency of superconductivity, where at low field a global superconducting phase is restored. Increasing magnetic field unveils an ‘avoided H-SIT’ that exhibits granularity-induced logarithmic divergence of the resistance/conductance above/below that transition, pointing to possible vestiges of the original emergent duality observed in a true H-SIT. We conclude that anomalous metallic phase is intimately associated with inherent inhomogeneities, exhibiting robust behavior at attainable temperatures for strongly granular two-dimensional systems.

     
    more » « less
  2. Abstract

    Experiments investigating magnetic-field-tuned superconductor–insulator transition (HSIT) mostly focus on two-dimensional material systems where the transition and its proximate ground-state phases, often exhibit features that are seemingly at odds with the expected behavior. Here we present a complementary study of a three-dimensional pressure-packed amorphous indium-oxide (InOx) powder where granularity controls the HSIT. Above a low threshold pressure of ∼0.2 GPa, vestiges of superconductivity are detected, although neither a true superconducting transition nor insulating behavior are observed. Instead, a saturation at very high resistivity at low pressure is followed by saturation at very low resistivity at higher pressure. We identify both as different manifestations of anomalous metallic phases dominated by superconducting fluctuations. By analogy with previous identification of the low resistance saturation as a ‘failed superconductor’, our data suggests that the very high resistance saturation is a manifestation of a ‘failed insulator’. Above a threshold pressure of ∼6 GPa, the sample becomes fully packed, and superconductivity is robust, withTCtunable with pressure. A quantum critical point atPC∼ 25 GPa marks the complete suppression of superconductivity. For a finite pressure belowPC, a magnetic field is shown to induce a HSIT from a true zero-resistance superconducting state to a weakly insulating behavior. Determining the critical field,HC, we show that similar to the 2D behavior, the insulating-like state maintains a superconducting character, which is quenched at higher field, above which the magnetoresistance decreases to its fermionic normal state value.

     
    more » « less
  3. The magnetic-field–tuned superconductor-to-insulator transition was studied in a hybrid system of superconducting indium islands, deposited on an indium oxide (InOx) thin film, which exhibits global superconductivity at low magnetic fields. Vacuum annealing was used to tune the conductivity of the InOx film, thereby tuning the inergrain coupling and the nature of the transition. The hybrid system exhibits a “giant” magnetoresistance above the magnetic-field–tuned superconductor-to-insulator transition (H-SIT), with critical behavior similar to that of uniform InOx films but at much lower magnetic fields, that manifests the duality between Cooper pairs and vortices. A key feature of this hybrid system is the separation between the quantum criticality and the onset of nonequilibrium behavior.

     
    more » « less
  4. Even the particle world is not immune to identity politics. Bosons have been in a bit of an identity crisis, or so it has seemed since 1989 ( 1 ). Quantum mechanics requires bosons made of two paired electrons to either condense into a superfluid with a well-defined phase with zero electrical resistance or localize in an insulating state with infinite resistance. The direct transition from superconducting to insulating states was widely observed in a range of thin films ( 2 – 4 ). The most popular model for explaining these observations ( 5 ) claims that the destruction of superconductivity occurs when the resistance of the thin film exceeds a critical value. For bosons on the brink of localization, electrically insulating behavior is observed if the resistance is greater than the quantum of resistance, R q = h /4 e 2 , otherwise superconductivity persists, where h is Planck's constant and e is the electric charge. On page 1505 of this issue, Yang et al. ( 6 ) offer a counterexample by establishing that a bosonic metallic phase disrupts the superconductor-insulator transition (SIT) in the high-temperature superconductor YBa 2 Cu 3 O 7– x (YBCO). 
    more » « less
  5. Abstract

    The interplay between charge transfer and electronic disorder in transition-metal dichalcogenide multilayers gives rise to superconductive coupling driven by proximity enhancement, tunneling and superconducting fluctuations, of a yet unwieldy variety. Artificial spacer layers introduced with atomic precision change the density of states by charge transfer. Here, we tune the superconductive coupling betweenNbSe2monolayers from proximity-enhanced to tunneling-dominated. We correlate normal and superconducting properties inSnSe1+δmNbSe21tailored multilayers with varying SnSe layer thickness (m=115). From high-field magnetotransport the critical fields yield Ginzburg–Landau coherence lengths with an increase of140%cross-plane (m=19), trending towards two-dimensional superconductivity form>9. We show cross-overs between three regimes: metallic with proximity-enhanced coupling (m=14), disordered-metallic with intermediate coupling (m=59) and insulating with Josephson tunneling (m>9). Our results demonstrate that stacking metal mono- and dichalcogenides allows to convert a metal/superconductor into an insulator/superconductor system, prospecting the control of two-dimensional superconductivity in embedded layers.

     
    more » « less