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1. Entanglement-assisted capacity regions and protocol designs for quantum multiple-access channels

   https://doi.org/10.1038/s41534-021-00412-3  

   Shi, Haowei ; Hsieh, Min-Hsiu ; Guha, Saikat ; Zhang, Zheshen ; Zhuang, Quntao ( December 2021 , npj Quantum Information)

   null (Ed.)

   Abstract We solve the entanglement-assisted (EA) classical capacity region of quantum multiple-access channels (MACs) with an arbitrary number of senders. As an example, we consider the bosonic thermal-loss MAC and solve the one-shot capacity region enabled by an entanglement source composed of sender-receiver pairwise two-mode squeezed vacuum states. The EA capacity region is strictly larger than the capacity region without entanglement-assistance. With two-mode squeezed vacuum states as the source and phase modulation as the encoding, we also design practical receiver protocols to realize the entanglement advantages. Four practical receiver designs, based on optical parametric amplifiers, are given and analyzed. In the parameter region of a large noise background, the receivers can enable a simultaneous rate advantage of 82.0% for each sender. Due to teleportation and superdense coding, our results for EA classical communication can be directly extended to EA quantum communication at half of the rates. Our work provides a unique and practical network communication scenario where entanglement can be beneficial. 

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2. Large-alphabet time-bin quantum key distribution and Einstein–Podolsky–Rosen steering via dispersive optics

   https://doi.org/10.1088/2058-9565/ad0f6f  

   Chang, Kai-Chi ; Sarihan, Murat Can ; Cheng, Xiang ; Zhang, Zheshen ; Wong, Chee Wei ( December 2023 , Quantum Science and Technology)

   Quantum key distribution (QKD) has established itself as a groundbreaking technology, showcasing inherent security features that are fundamentally proven. Qubit-based QKD protocols that rely on binary encoding encounter an inherent constraint related to the secret key capacity. This limitation restricts the maximum secret key capacity to one bit per photon. On the other hand, qudit-based QKD protocols have their advantages in scenarios where photons are scarce and noise is present, as they enable the transmission of more than one secret bit per photon. While proof-of-principle entangled-based qudit QKD systems have been successfully demonstrated over the years, the current limitation lies in the maximum distribution distance, which remains at 20 km fiber distance. Moreover, in these entangled high-dimensional QKD systems, the witness and distribution of quantum steering have not been shown before. Here we present a high-dimensional time-bin QKD protocol based on energy-time entanglement that generates a secure finite-length key capacity of 2.39 bit/coincidences and secure cryptographic finite-length keys at 0.24 Mbits s⁻¹in a 50 km optical fiber link. Our system is built entirely using readily available commercial off-the-shelf components, and secured by nonlocal dispersion cancellation technique against collective Gaussian attacks. Furthermore, we set new records for witnessing both energy-time entanglement and quantum steering over different fiber distances. When operating with a quantum channel loss of 39 dB, our system retains its inherent characteristic of utilizing large-alphabet. This enables us to achieve a secure key rate of 0.30 kbits s⁻¹and a secure key capacity of 1.10 bit/coincidences, considering finite-key effects. Our experimental results closely match the theoretical upper bound limit of secure cryptographic keys in high-dimensional time-bin QKD protocols (Moweret al2013Phys. Rev.A87062322; Zhanget al2014Phys. Rev. Lett.112120506), and outperform recent state-of-the-art qubit-based QKD protocols in terms of secure key throughput using commercial single-photon detectors (Wengerowskyet al2019Proc. Natl Acad. Sci.1166684; Wengerowskyet al2020npj Quantum Inf.65; Zhanget al2014Phys. Rev. Lett.112120506; Zhanget al2019Nat. Photon.13839; Liuet al2019Phys. Rev. Lett.122160501; Zhanget al2020Phys. Rev. Lett.125010502; Weiet al2020Phys. Rev.X10031030). The simple and robust entanglement-based high-dimensional time-bin protocol presented here provides potential for practical long-distance quantum steering and QKD with multiple secure bits-per-coincidence, and higher secure cryptographic keys compared to mature qubit-based QKD protocols.

    

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3. Entanglement-enhanced optomechanical sensing

   https://doi.org/10.1038/s41566-023-01178-0  

   Xia, Yi ; Agrawal, Aman R. ; Pluchar, Christian M. ; Brady, Anthony J. ; Liu, Zhen ; Zhuang, Quntao ; Wilson, Dalziel J. ; Zhang, Zheshen ( June 2023 , Nature Photonics)

   Optomechanical systems have been exploited in ultrasensitive measurements of force, acceleration and magnetic fields. The fundamental limits for optomechanical sensing have been extensively studied and now well understood—the intrinsic uncertainties of the bosonic optical and mechanical modes, together with backaction noise arising from interactions between the two, dictate the standard quantum limit. Advanced techniques based on non-classical probes, in situ ponderomotive squeezed light and backaction-evading measurements have been developed to overcome the standard quantum limit for individual optomechanical sensors. An alternative, conceptually simpler approach to enhance optomechanical sensing rests on joint measurements taken by multiple sensors. In this configuration, a pathway to overcome the fundamental limits in joint measurements has not been explored. Here we demonstrate that joint force measurements taken with entangled probes on multiple optomechanical sensors can improve the bandwidth in the thermal-noise-dominant regime or the sensitivity in the shot-noise-dominant regime. Moreover, we quantify the overall performance of entangled probes with the sensitivity–bandwidth product and observe a 25% increase compared with that of classical probes. The demonstrated entanglement-enhanced optomechanical sensors would enable new capabilities for inertial navigation, acoustic imaging and searches for new physics. 

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4. Long-baseline interferometry using single photon states as a non-local oscillator

   https://doi.org/10.1117/12.2610314  

   Brown, Matthew ; Thiel, Valerian ; Allgaier, Markus ; Raymer, Michael ; Smith, Brian ; Kwiat, Paul ; Monnier, John ( January 2022 , Proceedings Volume 12015, Quantum Computing, Communication, and Simulation II; 120150E (2022))

   Hemmer, Philip R. ; Migdall, Alan L. (Ed.)

   Recent proposals suggest that distributed single photons serving as a ‘non-local oscillator’ can outperform coherent states as a phase reference for long-baseline interferometric imaging of weak sources [1,2]. Such nonlocal quantum states distributed between telescopes can, in-principle, surpass the limitations of conventional interferometric-based astronomical imaging approaches for very-long baselines such as: signal-to-noise, shot noise, signal loss, and faintness of the imaged objects. Here we demonstrate in a table-top experiment, interference between a nonlocal oscillator generated by equal-path splitting of an idler photon from a pulsed, separable, parametric down conversion process and a spectrally single-mode, quasi-thermal source. We compare the single-photon nonlocal oscillator to a more conventional local oscillator with uncertain photon number. Both methods enabled reconstruction of the source’s Gaussian spatial distribution by measurement of the interference visibility as a function of baseline separation and then applying the van Cittert-Zernike theorem [3,4]. In both cases, good qualitative agreement was found with the reconstructed source width and the known source width as measured using a camera. We also report an increase of signal-to-noise per ‘faux’ stellar photon detected when heralding the idler photon. 1593 heralded (non-local oscillator) detection events led to a maximum visibility of ~17% compared to the 10412 unheralded (classical local oscillator) detection events, which gave rise to a maximum visibility of ~10% – the first instance of quantum-enhanced sensing in this context. 

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5. Molecular qubits based on photogenerated spin-correlated radical pairs for quantum sensing

   https://doi.org/10.1063/5.0084072  

   Mani, Tomoyasu ( June 2022 , Chemical Physics Reviews)

   Photogenerated spin-correlated radical pairs (SCRPs) in electron donor–bridge–acceptor (D–B–A) molecules can act as molecular qubits and inherently spin qubit pairs. SCRPs can take singlet and triplet spin states, comprising the quantum superposition state. Their synthetic accessibility and well-defined structures, together with their ability to be prepared in an initially pure, entangled spin state and optical addressability, make them one of the promising avenues for advancing quantum information science. Coherence between two spin states and spin selective electron transfer reactions form the foundation of using SCRPs as qubits for sensing. We can exploit the unique sensitivity of the spin dynamics of SCRPs to external magnetic fields for sensing applications including resolution-enhanced imaging, magnetometers, and magnetic switch. Molecular quantum sensors, if realized, can provide new technological developments beyond what is possible with classical counterparts. While the community of spin chemistry has actively investigated magnetic field effects on chemical reactions via SCRPs for several decades, we have not yet fully exploited the synthetic tunability of molecular systems to our advantage. This review offers an introduction to the photogenerated SCRPs-based molecular qubits for quantum sensing, aiming to lay the foundation for researchers new to the field and provide a basic reference for researchers active in the field. We focus on the basic principles necessary to construct molecular qubits based on SCRPs and the examples in quantum sensing explored to date from the perspective of the experimentalist. 

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