The hypothetical axion particle (of unknown mass) is a leading candidate for dark matter (DM). Many experiments search for axions with microwave cavities, where an axion may convert into a cavity photon, leading to a feeble excess in the output power of the cavity. Recent work [Backes et al., Nature 590, 238 (2021)] has demonstrated that injecting squeezed vacuum into the cavity can substantially accelerate the axion search. Here, we go beyond and provide a theoretical framework to leverage the benefits of quantum squeezing in a network setting consisting of many sensor cavities. By forming a local sensor network, the signals among the cavities can be combined coherently to boost the axion search. Furthermore, injecting multipartite entanglement across the cavities—generated by splitting a squeezed vacuum—enables a global noise reduction. We explore the performance advantage of such a local, entangled sensor network, which enjoys both coherence between the axion signals and entanglement between the sensors. Our analyses are pertinent to next-generation DM-axion searches aiming to leverage a network of sensors and quantum resources in an optimal way. Finally, we assess the possibility of using a more exotic quantum state, the Gottesman-Kitaev-Preskill (GKP) state. Despite a constant-factor improvement in the scan time relative to a single-mode squeezed state in the ideal case, the advantage of employing a GKP state disappears when a practical measurement scheme is considered.
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Generation of entangled-photons by a quantum dot cascade source in polarized cavities: Using cavity resonances to boost signals and preserve the entanglements
Motivated by recent advances in the development of single photon emitters for quantum information sciences, here we design and formulate a quantum cascade model that describes cascade emission by a quantum dot (QD) in a cavity structure while preserving entanglement that stores information needed for single photon emission. The theoretical approach is based on a photonic structure that consists of two orthogonal cavities in which resonance with either the first or second of the two emitted photons is possible, leading to amplification and rerouting of the entangled light. The cavity–QD scheme uses a four-level cascade emitter that involves three levels for each polarization, leading to two spatially entangled photons for each polarization. By solving the Schrodinger equation, we identify the characteristic properties of the system, which can be used in conjunction with optimization techniques to achieve the “best” design relative to a set of prioritized criteria or constraints in our optical system. The theoretical investigations include an analysis of emission spectra in addition to the joint spectral density profile, and the results demonstrate the ability of the cavities to act as frequency filters for the photons that make up the entanglements and to modify entanglement properties. The results provide new opportunities for the experimental design and engineering of on-demand single photon sources.
more » « less- Award ID(s):
- 2055565
- NSF-PAR ID:
- 10406373
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- The Journal of Chemical Physics
- Volume:
- 158
- Issue:
- 14
- ISSN:
- 0021-9606
- Page Range / eLocation ID:
- Article No. 144106
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Multiphoton absorption of entangled photons offers ways for obtaining unique information about chemical and biological processes. Measurements with entangled photons may enable sensing biological signatures with high selectivity and at very low light levels to protect against photodamage. In this paper, we present a theoretical and experimental study of the excitation wavelength dependence of the entangled two-photon absorption (ETPA) process in a molecular system, which provides insights into how entanglement affects molecular spectra. We demonstrate that the ETPA excitation spectrum can be different from that of classical TPA as well as that for one-photon resonant absorption (OPA) with photons of doubled frequency. These results are modeled by assuming the ETPA cross-section is governed by a two-photon excited state radiative linewidth rather than by electron-phonon interactions, and this leads to excitation spectra that match the observed results. Further, we find that the two-photon-allowed states with highest TPA and ETPA intensities have high electronic entanglements, with ETPA especially favoring states with the longest radiative lifetimes. These results provide concepts for the development of quantum light–based spectroscopy and microscopy that will lead to much higher efficiency of ETPA sensors and low-intensity detection schemes.more » « less
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