- Award ID(s):
- 1736668
- NSF-PAR ID:
- 10420160
- Date Published:
- Journal Name:
- Scientific Reports
- Volume:
- 11
- Issue:
- 1
- ISSN:
- 2045-2322
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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null (Ed.)We investigate the dynamics of cohesive particles in homogeneous isotropic turbulence, based on one-way coupled simulations that include Stokes drag, lubrication, cohesive and direct contact forces. We observe a transient flocculation phase, followed by a statistically steady equilibrium phase. We analyse the temporal evolution of floc size and shape due to aggregation, breakage and deformation. Larger turbulent shear and weaker cohesive forces yield smaller elongated flocs. Flocculation proceeds most rapidly when the fluid and particle time scales are balanced and a suitably defined Stokes number is $O(1)$ . During the transient stage, cohesive forces of intermediate strength produce flocs of the largest size, as they are strong enough to cause aggregation, but not so strong as to pull the floc into a compact shape. Small Stokes numbers and weak turbulence delay the onset of the equilibrium stage. During equilibrium, stronger cohesive forces yield flocs of larger size. The equilibrium floc size distribution exhibits a preferred size that depends on the cohesive number. We observe that flocs are generally elongated by turbulent stresses before breakage. Flocs of size close to the Kolmogorov length scale preferentially align themselves with the intermediate strain direction and the vorticity vector. Flocs of smaller size tend to align themselves with the extensional strain direction. More generally, flocs are aligned with the strongest Lagrangian stretching direction. The Kolmogorov scale is seen to limit floc growth. We propose a new flocculation model with a variable fractal dimension that predicts the temporal evolution of the floc size and shape.more » « less
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Abstract Due to the flocculation process, suspended mud aggregates carried by rivers to the coastal ocean are thought to undergo changes in size and shape in response to environmental drivers such as turbulence, sediment concentration, organic matter (OM), and salinity. Some have assumed that salt is necessary for floc formation, and that mud, therefore, reaches the estuary unflocculated. Yet mud flocs exist in freshwater systems long before the estuarine zone, likely due to the presence of OM acting as a floc‐promoting binder. Therefore, it is important to consider how salinity affects flocculation, if at all, in the presence of OM. Here, we used experiments to examine the flocculation of a natural mud with and without OM. Results showed that the rate of floc growth and equilibrium size both increase with salinity regardless of the presence or absence of OM. However, the response of both to salinity was stronger when OM was present. In deionized water, natural sediment with OM was seen to produce large flocs. However, the size distribution of the suspension tended to be bimodal. With the addition of salt, increasing amounts of unflocculated material became bound within flocs, producing a more unimodal size distribution. Here, the enhancing effects of salt were noticeable at even 0.5 ppt, and increases in salinity past 3–5 ppt only marginally increased the floc growth rate and final size. Data from the experiment were used to develop a salinity‐dependent model to account for changes in floc growth rate and equilibrium size.
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Muddy sediment constitutes a major fraction of the suspended sediment mass carried by the Mississippi River. Thus, adequate knowledge of the transport dynamics of suspended mud in this region is critical in devising efficient management plans for coastal Louisiana. We conducted laboratory tank experiments on the sediment suspended in the lower reaches of the Mississippi River to provide insight into the flocculation behavior of the mud. In particular, we measure how the floc size distribution responds to changing environmental factors of turbulent energy, sediment concentration, and changes in base water composition and salinity during summer and winter. We also compare observations from the tank experiments to
in situ observations. Turbulence shear rate, a measure of river hydrodynamic energy, was found to be the most influential factor in determining mud floc size. All flocs produced at a given shear rate could be kept in suspension down to shear rates of approximately 20 s−1. At this shear rate, flocs on the order of 150–200 μm and larger can settle out. Equilibrium floc size was not found to depend on sediment concentration; flocs larger than 100 μm formed in sediment concentrations as low as 20 mgL−1. An increase in salinity generated by adding salts to river water suspensions did not increase the flocculation rate or equilibrium size. However, the addition of water collected from the Gulf of Mexico to river-water suspensions did enhance the flocculation rate and the equilibrium sizes. We speculate that the effects of Gulf of Mexico water originate from its biomatter content rather than its ion composition. Floc sizes in the mixing tanks were comparable to those from the field for similar estimated turbulent energy. Flocs were found to break within minutes under increased turbulence but can take hours to grow under conditions of reduced shear in freshwater settings. Growth was faster with the addition of Gulf of Mexico water. Overall, the experiments provide information on how suspended mud in the lower reaches of the Mississippi might respond to changes in turbulence and salinity moving from the fluvial to marine setting through natural distributary channels or man-made diversions. -
Uijttewaal, W. ; Franca, J. ; Valero, M. ; Chavarrias, D. ; Ylla Arbós, V. ; Schielen, C. ; Crosato, A. (Ed.)Turbid rivers and density currents carry, distribute, and deposit considerable quantities of fine muddy sediment within rivers, coastal regions, and reservoirs. The muddy sediment in these flows has the potential to flocculate, and knowing and predicting the floc size is critical for predicting mud movement. Flocs are notoriously difficult to measure. Imaging of flocs either within a turbulent suspension or in a separate settling chamber are methods widely considered to be the most accurate ways to measure floc size. The benefit of imaging flocs within the suspension is that the measurements are made within the conditions that gave rise to those particular flocs. The drawback is that it is not possible to make measurements in suspensions with concentrations > 400 mg/L. Transferring a suspension sample to a settling chamber allows for imaging of flocs from suspensions with higher concentration. But, it also removes flocs from the environment in which they were formed, possibly leading to floc growth or breakup. In this study, we compare these two methods to determine whether or not the flocs imaged in a settling chamber are representative of the flocs found in a turbulent suspension. For the experiments, flocs are formed from kaolinite and montmorillonite clay mixed with saltwater at different concentrations and mixing conditions. The suspension is then imaged within the mixing tank, and samples from the mixing tank are imaged in a settling chamber. Results show that flocs imaged in the settling chamber tend to be slightly smaller than those imaged in the mixing chamber, though the differences are minimal if care is taken in the transfer process. Additional trends in the difference between the two methods with turbulent shear rate and concentration are discussed.more » « less
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Abstract To better understand the nature of flocs of varying organic content in estuarine surface waters, Laser in situ Scattering and Transmissometry, video settling, and pump sampling were deployed in the York River estuary. A new in situ method was developed to simultaneously solve the floc fractal dimension (
F ), primary particle size (d p ), and primary particle density (ρ p ) by fitting a simple fractal model to observations of effective floc density (Δρ ) as a function of floc diameter (d f ), while ensuring that the integrated particle size distribution was consistent with measurements of bulk apparent density (ρ a ). When fractal fits were statistically justified, application of the above methods showed the bulk fraction of organic matter (f org) to be well correlated to multiple floc properties. Asf orgincreased,d p andρ a also increased, whileρ p , total suspended solids (TSS), and median floc size decreased. Notably for microflocs, neitherF nor Δρ was significantly related to eitherf orgor TSS. This indicates that organic matter may partially displace water content within microflocs without fundamentally changing the flocs' inorganic structure. When pooling multiple samples, a marked decrease inF was seen at the transition to macroflocs, and most strongly for highf orgcases. This suggested that settling velocities ≥ ∼1 mm/s may produce turbulent stresses that tend to tear macroflocs apart. This study also found that when the fractal theory held,ρ p had a near 1:1 correlation with the bulk dry density of filtered TSS, implying that primary particles are tightly bound aggregates of combined mineral and organic components.