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Title: In 2 Se 3 , In 2 Te 3 , and In 2 (Se,Te) 3 Alloys as Photovoltaic Materials
Award ID(s):
1652994
NSF-PAR ID:
10430403
Author(s) / Creator(s):
; ; ; ; ; ;
Date Published:
Journal Name:
The Journal of Physical Chemistry Letters
Volume:
13
Issue:
51
ISSN:
1948-7185
Page Range / eLocation ID:
12026 to 12031
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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  1. Abstract

    The interface between 2D topological Dirac states and ans‐wave superconductor is expected to support Majorana‐bound states (MBS) that can be used for quantum computing applications. Realizing these novel states of matter and their applications requires control over superconductivity and spin‐orbit coupling to achieve spin‐momentum‐locked topological interface states (TIS) which are simultaneously superconducting. While signatures of MBS have been observed in the magnetic vortex cores of bulk FeTe0.55Se0.45, inhomogeneity and disorder from doping make these signatures unclear and inconsistent between vortices. Here superconductivity is reported in monolayer (ML) FeTe1–ySey(Fe(Te,Se)) grown on Bi2Te3by molecular beam epitaxy (MBE). Spin and angle‐resolved photoemission spectroscopy (SARPES) directly resolve the interfacial spin and electronic structure of Fe(Te,Se)/Bi2Te3heterostructures. Fory = 0.25, the Fe(Te,Se) electronic structure is found to overlap with the Bi2Te3TIS and the desired spin‐momentum locking is not observed. In contrast, fory = 0.1, reduced inhomogeneity measured by scanning tunneling microscopy (STM) and a smaller Fe(Te,Se) Fermi surface with clear spin‐momentum locking in the topological states are found. Hence, it is demonstrated that the Fe(Te,Se)/Bi2Te3system is a highly tunable platform for realizing MBS where reduced doping can improve characteristics important for Majorana interrogation and potential applications.

     
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  2. null (Ed.)