An official website of the United States government
Abstract In response to rising , chemistry‐climate models (CCMs) project that extratropical stratospheric ozone will increase, except around 10 and 17 km. We call the muted increases or reductions at these altitudes the “double dip.” The double dip results from surface warming (not stratospheric cooling). Using an idealized photochemical‐transport model, surface warming is found to produce the double dip via tropospheric expansion, which converts ozone‐rich stratospheric air into ozone‐poor tropospheric air. The lower dip results from expansion of the extratropical troposphere, as previously understood. The upper dip results from expansion of the tropical troposphere, low‐ozone anomalies from which are then transported into the extratropics. Large seasonality in the double dip in CCMs can be explained, at least in part, by seasonality in the stratospheric overturning circulation. The remote effects of the tropical tropopause on extratropical ozone complicate the use of (local) tropopause‐following coordinates to remove the effects of global warming.
more »
« less
Tropospheric Expansion Under Global Warming Reduces Tropical Lower Stratospheric Ozone
Abstract In response to global warming, ozone is predicted to increase aloft due to stratospheric cooling but decrease in the tropical lower stratosphere. The ozone reductions have been primarily attributed to a strengthening Brewer‐Dobson circulation, which upwells ozone‐poor air. Yet, this paper finds that strengthening upwelling only explains part of the reduction. The reduction is also driven by tropospheric expansion under global warming, which erodes the ozone layer from below, the low ozone anomalies from which are advected upwards. Strengthening upwelling and tropospheric expansion are correlated under global warming, making it challenging to disentangle their relative contributions. Therefore, chemistry‐climate model output is used to validate an idealized model of ozone photochemistry and transport with a tropopause lower boundary condition. In our idealized decomposition, strengthening upwelling and tropospheric expansion both contribute at leading order to reducing tropical ozone. Tropospheric expansion drives bottom‐heavy reductions in ozone, which decay in magnitude into the mid‐stratosphere.
more »
« less
- PAR ID:
- 10444130
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Geophysical Research Letters
- Volume:
- 49
- Issue:
- 19
- ISSN:
- 0094-8276
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract This study investigates changes in stratosphere‐troposphere exchange (STE) of air masses and ozone concentrations from 1960 to 2099 using multiple model simulations from Chemistry Climate Model Initiative (CCMI) under climate change scenario RCP6.0. We employ a lowermost stratosphere mass budget approach with dynamic isentropic surfaces fitted to the tropical tropopause as the upper boundary of lowermost stratosphere. The multi‐model mean (MMM) trends of air mass STEs are all small over all regions, which are within 0.3 (0.1) % decade−1for 1960–2000 (2000–2099). The MMM trends of ozone STE for 1960–2000 are 0.3%, −2.7%, 3.4%, −0.9%, and −2.7% decade−1over the Northern hemisphere (NH) extratropics, Southern hemisphere (SH) extratropics, tropics, extratropics, and globe, respectively. The corresponding ozone STE trends for 2000–2099 are 3.0%, 4.3%, 0.8%, 3.5%, and 4.7% decade−1. Changes in ozone STEs are dominated by ozone concentration changes, driven by climate‐induced changes and ozone‐depleting substance (ODS) changes. For 1960–2000, small changes in ozone STEs in the NH extratropics are due to a cancellation between effects of climate‐induced changes and ODS increases, while the ODS effect dominates in the SH extratropics, leading to a large ozone STE magnitude decrease. Increased ozone transport from tropical troposphere to stratosphere for 1960–2000 is due to increased tropospheric ozone. A decreased global ozone STE magnitude for 1960–2000 was largely caused by ODS‐induced ozone loss that is partly compensated by climate‐induced ozone changes. For 2000–2099, about two‐thirds of global ozone STE magnitude increases are caused by ozone increases in the extratropical lower stratosphere due to climate‐induced changes. The remaining one‐third is caused by ozone recovery due to the phaseout of ODS.more » « less
-
Abstract There are a myriad of ways atmospheric circulation responds to increased CO 2 . In the troposphere, the region of the tropical upwelling narrows, the Hadley Cells expand, and the upper level subtropical zonal winds that comprise the subtropical jet strengthen. In the stratosphere, the tropical upwelling narrows and strengthens, enhancing the Brewer-Dobson Circulation. Despite the robustness of these projections, dynamical coupling between the features remains unclear. In this study, we analyze output from the NASA Goddard Institute for Space Studies (GISS) ModelE coupled climate model to examine any connection between the upper tropospheric and lower stratospheric circulation by considering the features’ seasonality, hemispheric asymmetry, scaling, and transient response to a broad range of CO 2 forcings. We find that a narrowing and strengthening of upper tropospheric upwelling occurs with a strengthening of the subtropical jet. There is also a narrowing and strengthening of lower stratospheric upwelling that is related to an equatorward shift in critical latitude for wave breaking and the associated strengthening of the subtropical lower stratosphere’s zonal winds. However, the stratospheric responses display different seasonal, hemispheric, and transient patterns than those in the troposphere, indicating independent circulation changes between the two domains.more » « less
-
Abstract The steady response of the stratosphere to tropospheric thermal forcing via an SST perturbation is considered in two separate theoretical models. It is first shown that an SST anomaly imposes a geopotential anomaly at the tropopause. Solutions to the linearized quasigeostrophic potential vorticity equations are then used to show that the vertical length scale of a tropopause geopotential anomaly is initially shallow, but significantly increased by diabatic heating from radiative relaxation. This process is a quasi-balanced response of the stratosphere to tropospheric forcing. A previously developed, coupled troposphere–stratosphere model is then introduced and modified. Solutions under steady, zonally symmetric SST forcing in the linearβ-plane model show that the upward stratospheric penetration of the corresponding tropopause geopotential anomaly is controlled by two nondimensional parameters: 1) a dynamical aspect ratio and 2) a ratio between tropospheric and stratospheric drag. The meridional scale of the SST anomaly, radiative relaxation rate, and wave drag all significantly modulate these nondimensional parameters. Under Earthlike estimates of the nondimensional parameters, the theoretical model predicts stratospheric temperature anomalies 2–3 larger in magnitude than that in the boundary layer, approximately in line with observational data. Using reanalysis data, the spatial variability of temperature anomalies in the troposphere is shown to have remarkable coherence with that of the lower stratosphere, which further supports the existence of a quasi-balanced response of the stratosphere to SST forcing. These findings suggest that besides mechanical and radiative forcing, there is a third way the stratosphere can be forced—through the tropopause via tropospheric thermal forcing. Significance StatementUpward motion in the tropical stratosphere, the layer of atmosphere above where most weather occurs, is thought to be controlled by weather disturbances that propagate upward and dissipate in the stratosphere. The strength of this upward motion is important since it sets the global distribution of ozone. We formulate and use simple mathematical models to show the vertical motion in the stratosphere can also depend on the warming in the troposphere, the layer of atmosphere where humans live. We use the theory as an explanation for our observations of inverse correlations between the ocean temperature and the stratosphere temperature. These findings suggest that local stratospheric cooling may be coupled to local tropospheric warming.more » « less
-
Abstract Stratospheric ozone depletion from halocarbons is partly countered by pollution‐driven increases in tropospheric ozone, with transport connecting the two. While recognizing this connection, the ozone assessment's evaluation of observations and processes have often split the chapters at the tropopause boundary. Using a chemistry‐transport model we find that air‐pollution ozone enhancements in the troposphere spill over into the stratosphere at significant rates, that is, 13%–34% of the excess tropospheric burden appears in the lowermost extra‐tropical stratosphere. As we track the anticipated recovery of the observed ozone depletion, we should recognize that two tenths of that recovery may come from the transport of increasing tropospheric ozone into the stratosphere.more » « less
