Abstract Agricultural soils play a dual role in regulating the Earth's climate by releasing or sequestering carbon dioxide (CO2) in soil organic carbon (SOC) and emitting non‐CO2greenhouse gases (GHGs) such as nitrous oxide (N2O) and methane (CH4). To understand how agricultural soils can play a role in climate solutions requires a comprehensive assessment of net soil GHG balance (i.e., sum of SOC‐sequestered CO2and non‐CO2GHG emissions) and the underlying controls. Herein, we used a model‐data integration approach to understand and quantify how natural and anthropogenic factors have affected the magnitude and spatiotemporal variations of the net soil GHG balance in U.S. croplands during 1960–2018. Specifically, we used the dynamic land ecosystem model for regional simulations and used field observations of SOC sequestration rates and N2O and CH4emissions to calibrate, validate, and corroborate model simulations. Results show that U.S. agricultural soils sequestered Tg CO2‐C year−1in SOC (at a depth of 3.5 m) during 1960–2018 and emitted Tg N2O‐N year−1and Tg CH4‐C year−1, respectively. Based on the GWP100 metric (global warming potential on a 100‐year time horizon), the estimated national net GHG emission rate from agricultural soils was Tg CO2‐eq year−1, with the largest contribution from N2O emissions. The sequestered SOC offset ~28% of the climate‐warming effects resulting from non‐CO2GHG emissions, and this offsetting effect increased over time. Increased nitrogen fertilizer use was the dominant factor contributing to the increase in net GHG emissions during 1960–2018, explaining ~47% of total changes. In contrast, reduced cropland area, the adoption of agricultural conservation practices (e.g., reduced tillage), and rising atmospheric CO2levels attenuated net GHG emissions from U.S. croplands. Improving management practices to mitigate N2O emissions represents the biggest opportunity for achieving net‐zero emissions in U.S. croplands. Our study highlights the importance of concurrently quantifying SOC‐sequestered CO2and non‐CO2GHG emissions for developing effective agricultural climate change mitigation measures.
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Evaluating Cropland N 2 O Emissions and Fertilizer Plant Greenhouse Gas Emissions With Airborne Observations
Abstract Agricultural activity is a significant source of greenhouse gas emissions. The fertilizer production process emits N2O, CO2, and CH4, and fertilized croplands emit N2O. We present continuous airborne observations of these trace gases in the Lower Mississippi River Basin to quantify emissions from both fertilizer plants and croplands during the early growing season. Observed hourly emission rates from two fertilizer plants are compared with reported inventory values, showing agreement for N2O and CO2emissions but large underestimation in reported CH4emissions by up to a factor of 100. These CH4emissions are consistent with loss rates of 0.6–1.2%. We quantify regional emission fluxes (100 km) of N2O using the airborne mass balance technique, a first application for N2O, and explore linkages to controlling processes. Finally, we demonstrate the ability to use airborne measurements to distinguish N2O emission differences between neighboring fields, determining we can distinguish different emission behaviors of regions on the order of 2.5 km2with emissions differences of approximately 0.026μmol m−2s−1. This suggests airborne approaches such as outlined here could be used to evaluate the impact of different agricultural practices at critical field‐size spatial scales.
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- Award ID(s):
- 1650682
- PAR ID:
- 10450919
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Volume:
- 125
- Issue:
- 16
- ISSN:
- 2169-897X
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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