skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Geometrically Tunable Beamed Light Emission from a Quantum‐Dot Ensemble Near a Gradient Metasurface
Abstract Optical metasurfaces have been widely investigated in recent years as a means to tailor the wavefronts of externally incident light for passive device applications. At the same time, their use in active optoelectronic devices such as light emitters is far less established. This work explores their ability to control the radiation properties of a nearby continuous ensemble of randomly oriented incoherent dipole sources via near‐field interactions. Specifically, a film of colloidal quantum dots is deposited on a plasmonic metasurface consisting of a 1D array of metallic nanoantennas on a metal film. The array is designed to introduce a linear phase profile upon reflection, and a bi‐periodic nanoparticle arrangement is introduced to ensure adequate sampling of the desired phase gradient. Highly directional radiation patterns are correspondingly obtained from the quantum dots at an enhanced emission rate. The underlying radiation mechanism involves the near‐field excitation of surface plasmon polaritons at the metal film, and their selective diffractive scattering by the metasurface into well‐collimated beams along predetermined geometrically tunable directions. These results underscore the distinctive ability of metasurfaces to control radiation properties directly at the source level, which is technologically significant for the continued miniaturization and large‐scale integration of optoelectronic devices.  more » « less
Award ID(s):
1711156
PAR ID:
10458249
Author(s) / Creator(s):
 ;  ;  ;  ;  ;  
Publisher / Repository:
Wiley Blackwell (John Wiley & Sons)
Date Published:
Journal Name:
Advanced Optical Materials
Volume:
8
Issue:
8
ISSN:
2195-1071
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Metasurfaces, composed of engineered nanoantennas, enable unprecedented control over electromagnetic waves by leveraging multipolar resonances to tailor light–matter interactions. This review explores key physical mechanisms that govern their optical properties, including the role of multipolar resonances in shaping metasurface responses, the emergence of bound states in the continuum (BICs) that support high-quality factor modes, and the Purcell effect, which enhances spontaneous emission rates at the nanoscale. These effects collectively underpin the design of advanced photonic devices with tailored spectral, angular, and polarization-dependent properties. This review discusses recent advances in metasurfaces and applications based on them, highlighting research that employs full-wave numerical simulations, analytical and semi-analytic techniques, multipolar decomposition, nanofabrication, and experimental characterization to explore the interplay of multipolar resonances, bound and quasi-bound states, and enhanced light–matter interactions. A particular focus is given to metasurface-enhanced photodetectors, where structured nanoantennas improve light absorption, spectral selectivity, and quantum efficiency. By integrating metasurfaces with conventional photodetector architectures, it is possible to enhance responsivity, engineer photocarrier generation rates, and even enable functionalities such as polarization-sensitive detection. The interplay between multipolar resonances, BICs, and emission control mechanisms provides a unified framework for designing next-generation optoelectronic devices. This review consolidates recent progress in these areas, emphasizing the potential of metasurface-based approaches for high-performance sensing, imaging, and energy-harvesting applications. 
    more » « less
  2. Abstract Since their inception, quantum dots have proven to be advantageous for light management applications due to their high brightness and well‐controlled absorption, scattering, and emission properties. As quantum dots become commercially available at large scale, the need for robust, stable, and flexible optical components continues to drive the development of robust and flexible quantum dot composite materials. In this review, after a thorough introduction to quantum dots, discussion delves into methods for fabricating quantum dot loaded composite optical elements such as thin films, microfabricated patterns, and microstructures. The importance of surface chemistry and ligand engineering, host matrixes, wet processing, and unique patterning methodologies is presented by considering photostability, aggregation, and phase separation of quantum dots in corresponding composites. With regard to prospective optical applications of quantum dot materials, emphasis is placed on light emitting and guiding composite materials for lasing applications, specifically whispering gallery mode‐based photonic microsystems. These developments will enable novel flexible, portable, and miniaturized optoelectronic devices such as light‐emitting diodes, flexible pixelated displays, solar cells, large‐area microwaveguides, omnidirectional micromirrors, optical metasurfaces, and directional microlasers. 
    more » « less
  3. Abstract All‐optical control and detection of magnetic states for high‐density recording necessitate nanophotonic approaches to amplify local light intensity below the diffraction limit. Sculpting the near‐field phase and polarization can additionally strengthen magneto‐optical effects that rely on circularly polarized pulses, such as all‐optical helicity‐dependent switching, imaging, and spin‐wave excitation. Here, high‐refractive‐index dielectric nanoantennas illuminated with circularly polarized light resonantly enhance local electric field rotation by more than sixfold within [Pt/Co]Nthin films. Sub‐wavelength arrays of amorphous Si nanodisks, or metasurfaces, patterned on perpendicularly magnetized films support Mie‐type resonances that modulate reflection and transmission dissymmetry by >±2% in experiments. Spatial and spectral interference between dipolar modes, proximity effects, and gain are evaluated by varying disk aspect ratio, metasurface–metal separation, and magnetic film thickness, respectively. Simulated enhancements in magnetic circular birefringence and differential absorption are correlated with amplified local field rotation at electric dipolar modes. Greater achievable amplifications are shown via simulations with single‐crystalline Si metasurfaces exhibiting lower losses, including a 12‐fold strengthened electric field rotation within ferromagnetic layers. The metasurface design rules established here could enable nanoscale localization of all‐optical magnetic switching with lowered laser fluence thresholds, as well as enhanced magneto‐optical responses for light‐assisted reading in spintronic devices. 
    more » « less
  4. Abstract Metasurfaces offer complete control of optical wavefront at the subwavelength scale, advancing a new class of artificial planar optics, including lenses, waveplates, and holograms, with unprecedented merits over conventional optical components. In particular, the ultrathin, flat, and compact characteristics of metasurfaces facilitate their integration with semiconductor devices for the development of miniaturized and multifunctional optoelectronic systems. In this work, generation of structured light is implemented at an ultracompact wafer‐level through the monolithic integration of metasurface with standard vertical cavity surface‐emitting lasers (VCSELs). This work opens new perspectives for the design of structured light systems with compactness, lightweight, and scalability. Ultracompact beam structured laser chips with versatile functionalities are experimentally demonstrated, including multichannel beams array generation, on‐chip large‐angle beam steering up to 60°, and wafer‐level holographic beam shaping with a wide field of view (about 124°). The results will promote the development of compact light structuring systems with great potential in 3D imaging, displays, robotic vision, human–computer interaction, and augmented/virtual reality. 
    more » « less
  5. Plasmonic nanostructures and metasurfaces are appealing hosts for investigation of novel optical devices and exploration of new frontiers in physical/optical processes and materials research. Recent studies have shown that these structures hold the promise of greater control over the optical and electronic properties of quantum emitters, offering a unique horizon for ultra-fast spin-controlled optical devices, quantum computation, laser systems, and sensitive photodetectors. In this Perspective, we discuss how heterostructures consisting of metal oxides, metallic nanoantennas, and dielectrics can offer a material platform wherein one can use the decay of plasmons and their near fields to passivate the defect sites of semiconductor quantum dots while enhancing their radiative decay rates. Such a platform, called functional metal-oxide plasmonic metasubstrates (FMOPs), relies on formation of two junctions at very close vicinity of each other. These include an Au/Si Schottky junction and an Si/Al oxide charge barrier. Such a double junction allows one to use hot electrons to generate a field-passivation effect, preventing migration of photo-excited electrons from quantum dots to the defect sites. Prospects of FMOP, including impact of enhancement exciton–plasmon coupling, collective transport of excitation energy, and suppression of quantum dot fluorescence blinking, are discussed. 
    more » « less