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Title: Spin structure and dynamics of the topological semimetal Co3Sn2-xInxS2
Abstract The anomalous Hall effect (AHE), typically observed in ferromagnetic (FM) metals with broken time-reversal symmetry, depends on electronic and magnetic properties. In Co3Sn2-xInxS2, a giant AHE has been attributed to Berry curvature associated with the FM Weyl semimetal phase, yet recent studies report complicated magnetism. We use neutron scattering to determine the spin dynamics and structures as a function ofxand provide a microscopic understanding of the AHE and magnetism interplay. Spin gap and stiffness indicate a contribution from Weyl fermions consistent with the AHE. The magnetic structure evolves fromc-axis ferromagnetism at$$x = 0$$ x = 0 to a canted antiferromagnetic (AFM) structure with reducedc-axis moment and in-plane AFM order at$$x = 0.12$$ x = 0.12 and further reducedc-axis FM moment at$$x = 0.3$$ x = 0.3 . Since noncollinear spins can induce non-zero Berry curvature in real space acting as a fictitious magnetic field, our results revealed another AHE contribution, establishing the impact of magnetism on transport.  more » « less
Award ID(s):
2100741
PAR ID:
10466674
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Publisher / Repository:
npj Quantum Materials
Date Published:
Journal Name:
npj Quantum Materials
Volume:
7
Issue:
1
ISSN:
2397-4648
Page Range / eLocation ID:
112
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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