skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Spin structure and dynamics of the topological semimetal Co3Sn2-xInxS2
Abstract The anomalous Hall effect (AHE), typically observed in ferromagnetic (FM) metals with broken time-reversal symmetry, depends on electronic and magnetic properties. In Co3Sn2-xInxS2, a giant AHE has been attributed to Berry curvature associated with the FM Weyl semimetal phase, yet recent studies report complicated magnetism. We use neutron scattering to determine the spin dynamics and structures as a function ofxand provide a microscopic understanding of the AHE and magnetism interplay. Spin gap and stiffness indicate a contribution from Weyl fermions consistent with the AHE. The magnetic structure evolves fromc-axis ferromagnetism at$$x = 0$$ x = 0 to a canted antiferromagnetic (AFM) structure with reducedc-axis moment and in-plane AFM order at$$x = 0.12$$ x = 0.12 and further reducedc-axis FM moment at$$x = 0.3$$ x = 0.3 . Since noncollinear spins can induce non-zero Berry curvature in real space acting as a fictitious magnetic field, our results revealed another AHE contribution, establishing the impact of magnetism on transport.  more » « less
Award ID(s):
2100741
PAR ID:
10466674
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Publisher / Repository:
npj Quantum Materials
Date Published:
Journal Name:
npj Quantum Materials
Volume:
7
Issue:
1
ISSN:
2397-4648
Page Range / eLocation ID:
112
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe2is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetryYandTpoints and disperse along the crystallographic$$\hat{b}$$ b ̂ -axis. In applied magnetic fields to at leastμ0H= 11 T along the$$\hat{c}-{\rm{axis}}$$ c ̂ axis , the magnetism is found to be field-independent in the (hk0) plane. The scattering intensity is consistent with that expected from U3+/U4+ f-electron spins with preferential orientation along the crystallographic$$\hat{a}$$ a ̂ -axis, and a fluctuating magnetic moment ofμeff=1.7(5)μB. We propose interband spin excitons arising fromf-electron hybridization as a possible origin of the magnetic excitations in UTe2
    more » « less
  2. Abstract We define the half-volume spectrum$$\{{\tilde{\omega }_p\}_{p\in \mathbb {N}}}$$ { ω ~ p } p N of a closed manifold$$(M^{n+1},g)$$ ( M n + 1 , g ) . This is analogous to the usual volume spectrum ofM, except that we restrict top-sweepouts whose slices each enclose half the volume ofM. We prove that the Weyl law continues to hold for the half-volume spectrum. We define an analogous half-volume spectrum$$\tilde{c}(p)$$ c ~ ( p ) in the phase transition setting. Moreover, for$$3 \le n+1 \le 7$$ 3 n + 1 7 , we use the Allen–Cahn min-max theory to show that each$$\tilde{c}(p)$$ c ~ ( p ) is achieved by a constant mean curvature surface enclosing half the volume ofMplus a (possibly empty) collection of minimal surfaces with even multiplicities. 
    more » « less
  3. Abstract The crystal structure and bonding environment of K2Ca(CO3)2bütschliite were probed under isothermal compression via Raman spectroscopy to 95 GPa and single crystal and powder X-ray diffraction to 12 and 68 GPa, respectively. A second order Birch-Murnaghan equation of state fit to the X-ray data yields a bulk modulus,$${K}_{0}=46.9$$ K 0 = 46.9 GPa with an imposed value of$${K}_{0}^{\prime}= 4$$ K 0 = 4 for the ambient pressure phase. Compression of bütschliite is highly anisotropic, with contraction along thec-axis accounting for most of the volume change. Bütschliite undergoes a phase transition to a monoclinicC2/mstructure at around 6 GPa, mirroring polymorphism within isostructural borates. A fit to the compression data of the monoclinic phase yields$${V}_{0}=322.2$$ V 0 = 322.2  Å3$$,$$ , $${K}_{0}=24.8$$ K 0 = 24.8 GPa and$${K}_{0}^{\prime}=4.0$$ K 0 = 4.0 using a third order fit; the ability to access different compression mechanisms gives rise to a more compressible material than the low-pressure phase. In particular, compression of theC2/mphase involves interlayer displacement and twisting of the [CO3] units, and an increase in coordination number of the K+ion. Three more phase transitions, at ~ 28, 34, and 37 GPa occur based on the Raman spectra and powder diffraction data: these give rise to new [CO3] bonding environments within the structure. 
    more » « less
  4. Abstract Charge density wave (CDW) ordering has been an important topic of study for a long time owing to its connection with other exotic phases such as superconductivity and magnetism. The$$R{\textrm{Te}}_{3}$$ R Te 3 (R= rare-earth elements) family of materials provides a fertile ground to study the dynamics of CDW in van der Waals layered materials, and the presence of magnetism in these materials allows to explore the interplay among CDW and long range magnetic ordering. Here, we have carried out a high-resolution angle-resolved photoemission spectroscopy (ARPES) study of a CDW material$${\textrm{Gd}}{\textrm{Te}}_{3}$$ Gd Te 3 , which is antiferromagnetic below$$\sim \mathrm {12~K}$$ 12 K , along with thermodynamic, electrical transport, magnetic, and Raman measurements. Our ARPES data show a two-fold symmetric Fermi surface with both gapped and ungapped regions indicative of the partial nesting. The gap is momentum dependent, maximum along$${\overline{\Gamma }}-\mathrm{\overline{Z}}$$ Γ ¯ - Z ¯ and gradually decreases going towards$${\overline{\Gamma }}-\mathrm{\overline{X}}$$ Γ ¯ - X ¯ . Our study provides a platform to study the dynamics of CDW and its interaction with other physical orders in two- and three-dimensions. 
    more » « less
  5. Abstract LetXbe ann-element point set in thek-dimensional unit cube$$[0,1]^k$$ [ 0 , 1 ] k where$$k \ge 2$$ k 2 . According to an old result of Bollobás and Meir (Oper Res Lett 11:19–21, 1992) , there exists a cycle (tour)$$x_1, x_2, \ldots , x_n$$ x 1 , x 2 , , x n through thenpoints, such that$$\left( \sum _{i=1}^n |x_i - x_{i+1}|^k \right) ^{1/k} \le c_k$$ i = 1 n | x i - x i + 1 | k 1 / k c k , where$$|x-y|$$ | x - y | is the Euclidean distance betweenxandy, and$$c_k$$ c k is an absolute constant that depends only onk, where$$x_{n+1} \equiv x_1$$ x n + 1 x 1 . From the other direction, for every$$k \ge 2$$ k 2 and$$n \ge 2$$ n 2 , there existnpoints in$$[0,1]^k$$ [ 0 , 1 ] k , such that their shortest tour satisfies$$\left( \sum _{i=1}^n |x_i - x_{i+1}|^k \right) ^{1/k} = 2^{1/k} \cdot \sqrt{k}$$ i = 1 n | x i - x i + 1 | k 1 / k = 2 1 / k · k . For the plane, the best constant is$$c_2=2$$ c 2 = 2 and this is the only exact value known. Bollobás and Meir showed that one can take$$c_k = 9 \left( \frac{2}{3} \right) ^{1/k} \cdot \sqrt{k}$$ c k = 9 2 3 1 / k · k for every$$k \ge 3$$ k 3 and conjectured that the best constant is$$c_k = 2^{1/k} \cdot \sqrt{k}$$ c k = 2 1 / k · k , for every$$k \ge 2$$ k 2 . Here we significantly improve the upper bound and show that one can take$$c_k = 3 \sqrt{5} \left( \frac{2}{3} \right) ^{1/k} \cdot \sqrt{k}$$ c k = 3 5 2 3 1 / k · k or$$c_k = 2.91 \sqrt{k} \ (1+o_k(1))$$ c k = 2.91 k ( 1 + o k ( 1 ) ) . Our bounds are constructive. We also show that$$c_3 \ge 2^{7/6}$$ c 3 2 7 / 6 , which disproves the conjecture for$$k=3$$ k = 3 . Connections to matching problems, power assignment problems, related problems, including algorithms, are discussed in this context. A slightly revised version of the Bollobás–Meir conjecture is proposed. 
    more » « less