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Abstract Cloud condensation and hydrometeor evaporation fractionate stable isotopes of water, enriching liquid with heavy isotopes; whereupon updrafts, downdrafts, and rain vertically redistribute water and its isotopes in the lower troposphere. These vertical water fluxes through the marine boundary layer affect low cloud climate feedback and, combined with isotope fractionation, are hypothesized to explain the depletion of tropical precipitation at higher precipitation rates known as the “amount effect.” Here, an efficient and numerically stable quasi‐analytical model simulates the evaporation of raindrops and enrichment of their isotope composition. It is applied to a drop size distribution and subcloud environment representative of Atlantic trade cumulus clouds. Idealized physics experiments artificially zero out selected processes to discern the separate effects on the isotope ratio of raindrops, of exchange with the environment, evaporation, and kinetic molecular diffusion. A parameterization of size‐dependent molecular and eddy diffusion is formulated that enriches raindrops much more strongly (+5‰ for deuterated water [HDO] and +3.5‰ for O) than equilibrium evaporation as they become smaller than 1 mm. The effect on evaporated vapor is also assessed. Rain evaporation enriches subcloud vapor by +12‰ per mm rain (for HDO), explaining observations of enriched vapor in cold pools sourced by evaporatively cooled downdrafts. Drops smaller than 0.5 mm evaporate completely before falling 700 m in typical subtropical marine boundary layer conditions. The early and complete evaporation of these smaller drops in the rain size distribution enriches the vapor produced by rain evaporation.
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Sub-cloud rain evaporation in the North Atlantic winter trade winds derived by pairing isotopic data with a bin-resolved microphysical model
Sub-cloud rain evaporation in the trade wind region significantly influences the boundary layer mass and energy budgets. Parameterizing it is, however, difficult due to the sparsity of well-resolved rain observations and the challenges of sampling short-lived marine cumulus clouds. In this study, sub-cloud rain evaporation is analyzed using a steady-state, one-dimensional model that simulates changes in drop sizes, relative humidity, and rain isotopic composition. The model is initialized with relative humidity, raindrop size distributions, and water vapor isotope ratios (e.g., δDv, δ18Ov) sampled by the NOAA P3 aircraft during the Atlantic Tradewind Ocean–Atmosphere Mesoscale Interaction Campaign (ATOMIC), which was part of the larger EUREC4A (ElUcidating the RolE of Clouds–Circulation Coupling in ClimAte) field program. The modeled surface precipitation isotope ratios closely match the observations from EUREC4A ground-based and ship-based platforms, lending credibility to our model. The model suggests that 63 % of the rain mass evaporates in the sub-cloud layer across 22 P3 cases. The vertical distribution of the evaporated rain flux is top heavy for a narrow (σ) raindrop size distribution (RSD) centered over a small geometric mean diameter (Dg) at the cloud base. A top-heavy profile has a higher rain-evaporated fraction (REF) and larger changes in the rain deuterium excess (d=δD-8×δ18O) between the cloud base and the surface than a bottom-heavy profile, which results from a wider RSD with larger Dg. The modeled REF and change in d are also more strongly influenced by cloud base Dg and σ rather than the concentration of raindrops. The model results are accurate as long as the variations in the relative humidity conditions are accounted for. Relative humidity alone, however, is a poor indicator of sub-cloud rain evaporation. Overall, our analysis indicates the intricate dependence of sub-cloud rain evaporation on both thermodynamic and microphysical processes in the trade wind region.
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- PAR ID:
- 10469790
- Publisher / Repository:
- EGU
- Date Published:
- Journal Name:
- Atmospheric Chemistry and Physics
- Volume:
- 23
- Issue:
- 19
- ISSN:
- 1680-7324
- Page Range / eLocation ID:
- 12671 to 12690
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.5194/acp-23-12671-2023
