Halide Vacancies Create No Charge Traps on Lead Halide Perovskite Surfaces but Can Generate Deep Traps in the Bulk
- Award ID(s):
- 2154367
- PAR ID:
- 10493616
- Publisher / Repository:
- ACS
- Date Published:
- Journal Name:
- The Journal of Physical Chemistry Letters
- Volume:
- 14
- Issue:
- 26
- ISSN:
- 1948-7185
- Page Range / eLocation ID:
- 6028 to 6036
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
null (Ed.)Abstract We develop a model of social learning from complementary information: short-lived agents sequentially choose from a large set of flexibly correlated information sources for prediction of an unknown state, and information is passed down across periods. Will the community collectively acquire the best kinds of information? Long-run outcomes fall into one of two cases: (i) efficient information aggregation, where the community eventually learns as fast as possible; (ii) “learning traps,” where the community gets stuck observing suboptimal sources and information aggregation is inefficient. Our main results identify a simple property of the underlying informational complementarities that determines which occurs. In both regimes, we characterize which sources are observed in the long run and how often.more » « less
-
We propose engineering optical traps over plasmonic surfaces and precisely controlling the trap position with an external bias by inducing in-plane nonreciprocity on the surface. The platform employs an incident Gaussian beam to polarize targeted nanoparticles, and exploits the interplay between nonreciprocal and spin-orbit lateral recoil forces to construct stable optical traps and manipulate their position within the surface. To model this process, we develop a theoretical framework based on the Lorentz force combined with nonreciprocal Green’s functions and apply it to calculate the trapping potential. Rooted on this formalism, we explore the exciting possibilities offered by graphene to engineer stable optical traps using low-power laser beams in the mid-IR and to manipulate the trap position in a continuous manner by applying a longitudinal drift bias. Nonreciprocal metasurfaces may open new possibilities to trap, assemble and manipulate nanoparticles and overcome many challenges faced by conventional optical tweezers while dealing with nanoscale objects.more » « less