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This content will become publicly available on June 25, 2025

Title: Giant optical second- and third-order nonlinearities at a telecom wavelength

A material platform that excels in both optical second- and third-order nonlinearities at a telecom wavelength is theoretically and experimentally demonstrated. In this TiN-based coupled metallic quantum well structure, electronic subbands are engineered to support doubly resonant inter-subband transitions for an exceptionally high second-order nonlinearity and provide single-photon transitions for a remarkable third-order nonlinearity within the 1400–1600 nm bandwidth. The second-order susceptibilityχ(2)reaches 2840 pm/V at 1440 nm, while the Kerr coefficientn2arrives at 2.8 × 10−10 cm2/W at 1460 nm. The achievement of simultaneous strong second- and third-order nonlinearities in one material at a telecom wavelength creates opportunities for multi-functional advanced applications in the field of nonlinear optics.

 
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PAR ID:
10517352
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
Optical Society of America
Date Published:
Journal Name:
Optics Letters
Volume:
49
Issue:
13
ISSN:
0146-9592; OPLEDP
Format(s):
Medium: X Size: Article No. 3725
Size(s):
Article No. 3725
Sponsoring Org:
National Science Foundation
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