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5. Photoassociation of ${}^{84}\mathrm{Sr}$ $n{}^1{D}_2$ ultralong-range Rydberg dimers

   https://doi.org/10.1103/ppv2-mlfd  

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   Measurements of the production of $5snd{}^1{D}_2–5s^2{}^1{S}_0$ ultralong-range Rydberg dimers through photoassocation in an ultracold ${}^{84}\mathrm{Sr}$ atomic gas are reported. The molecular potential associated with the Rydberg $D$ state is anisotropic and the molecular states are characterized by the vibrational quantum number $\nu$ and the total angular momentum $\vec{K}=\vec{L}+\vec{N}$ , where $\vec{L}$ and $\vec{N}$ are the electronic orbital angular momentum and rotational angular momentum, respectively. The measured molecular binding energies agree reasonably well with theoretical predictions. Additionally, the electron-atom scattering leads to broader line shapes in the photoassociation spectrum than might be expected simply from the angular momentum of the initial colliding cold-atom pairs. 

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