Forced immersion cooling, where a dielectric fluid flows in contact with the cells, is an effective cooling approach for lithium-ion batteries. While previous models demonstrated effectiveness, they generally focused on thermal-fluid aspects and often neglected the coupling between temperature, cell potential, and heat generation (in other words, the electrochemistry remained unaffected by cooling conditions). Here, we use a fully coupled modeling approach that solves the detailed electrochemical model (with temperature-dependent properties) in conjunction with the thermal-fluid transport models at each time step. For an 18650 cell, we compare forced immersion cooling (water and mineral oil) to forced air cooling. Improved temperature control with immersion cooling leads to higher heat generation with increased capacity loss: a 3 K temperature rise corresponds to 10% loss, whereas 42 K temperature rise results in 0.4% loss at 5C discharge. Neglecting two-way coupling prohibits accurate analysis of the effectiveness of immersion cooling. Furthermore, the thermal conductivity and heat capacity of the fluid most significantly impact the electrochemical and thermal response. Finally, we define a new metric to compare performance with different flow parameters without computationally-expensive numerical simulations. Overall, this study provides insights that will be useful in understanding and design of immersion-cooled battery systems.
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Single Phase Static Immersive Cooling of Cylindrical Battery - Insight of Measuring Methods and Result
As the demand for utilizing lithium-ion batteries (LIB) has increased due to the entering of the informational era and the efforts of carbon neutrality, battery thermal management has become an important topic. Previous work has focused on removing heat using forced air and indirect liquid cooling. Due to the cost-effective cooling performance, single-phase static direct immersive cooling has recently gained attention. This paper aims to understand single cylindrical LIB’s thermal behavior under different surroundings when implementing single-phase static immersive cooling. This paper also aimed to explore how different methods of attaching thermocouples affect the precision of the measurement. By attaching thermocouples with various orientations and attachment methods on the different regions of the LIB, the temperature measurement by thermocouples is obtained by varying two battery brands, four fluid types, two submerging percentages, and four discharge rates. The expected result is that Sony battery reaches the maximum temperature of 34 °C when under 3C discharge rate and 90% under AmpCool-110 engineering fluid, which is 25 °C cooler relative to the same setup when cooling by 23 °C ambient air. The experiment also expected horizontal-orientated thermocouples with additional TIM between the cell’s wall and the probe to provide the most accurate measurement of temperature. The present study will serve as the foundation for validating and tuning the computational model of the battery, which will be utilized to research the optimal configuration of the battery pack for cooling performance per energy density.
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- Award ID(s):
- 2143043
- PAR ID:
- 10527957
- Publisher / Repository:
- Purdue University
- Date Published:
- Format(s):
- Medium: X
- Location:
- West Lafayette, IN
- Sponsoring Org:
- National Science Foundation
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