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The multipole interference (MPI) effect plays pivotal roles in the formation of electromagnetic responses in various settings. In the optics regime, it has been realized typically through the Mie resonance that necessitates high‐index, deep‐subwavelength‐scale dielectric resonators that are challenging to fabricate. Herein, a new, diffraction‐based MPI scheme that can be realized with low‐index, mesoscale dielectric structures is demonstrated. It is verified that this “diffractive MPI” concept by realizing various MPI states using micrometric polymeric cuboids fabricated by soft‐lithography. Subsequent analyses reveal that the MPI states with a distinct near‐zero forward scattering (NZFS) characteristic played crucial roles in shaping the cuboid's transmission spectrum. A hitherto unreported NZFS state, which exhibits a unique, “trifolium” radiation pattern, is also identified. The spectral position of such NZFS states turns out to be strongly dependent on the cuboid's geometry. By combining these results, the diffractive NZFS formation is related to the important phenomena of induced transparency and structural color generation.
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Structural coloring with low-index polymer nanostructures via multipolar decomposition-based design and optimization
Recently, there have been notable advances in nanophotonic structural color generation which enabled various applications in display, anti-counterfeiting, sensors and detectors. However, most advances in this domain have been achieved through the use of high-index materials which require expensive and complex fabrication. In this work, we enable low-index polymer nanostructures to generate structural colors using the multipolar decomposition technique which allows a better understanding and design of the scattering process by identifying the dominant multipole modes from the scattered fields. We set a polymeric (n~1.56) cuboid as the structural color generation platform, examined the contributions of various multipoles from the wave scattered by it, and synthesized the desired color spectrum by adjusting only the height of the cuboid. To validate our findings, we fabricated the designed structural color pixels via light-controlled, low-pressure nanoimprinting and measured the color and spectrum from them. Our experimental results agreed well with the simulation results, providing insights for bringing further advances to structural coloring.
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- Award ID(s):
- 2129796
- PAR ID:
- 10535339
- Editor(s):
- Piyawattanametha, Wibool; Park, Yong-Hwa; Zappe, Hans
- Publisher / Repository:
- SPIE
- Date Published:
- ISBN:
- 9781510670587
- Page Range / eLocation ID:
- 28
- Format(s):
- Medium: X
- Location:
- San Francisco, United States
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Conference Paper:
- https://doi.org/10.1117/12.3002806
