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1. The Transition from Supercooled Liquid Water to Ice Crystals in Mixed-phase Clouds based on Airborne In-situ Observations

   Flor Vanessa Maciel; Minghui Diao (October 2022, Atmospheric measurement techniques Papers in open discussion)

   The on-set of ice nucleation in mixed-phase clouds determines cloud lifetime and their microphysical properties. In this work, we develop a novel method that differentiates the early and later transition phases of mixed-phase clouds, i.e., ice crystals are initially surrounded by supercooled liquid water droplets, then as they grow, pure ice segments are formed. Using this method, we examine the relationship between the macrophysical and microphysical properties of mixed-phase clouds. The results show that evolution of cloud macrophysical properties, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the evolution of microphysical properties, represented by the increasing ice water content and decreasing liquid water content. The mass partition transition from liquid to ice becomes more significant during the later transition phase (i.e., transition phase 3) when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show significant transition from liquid to ice at a similar temperature (i.e., -17.5 °C) among three types of definitions of mixed-phase clouds based on ice mass fraction, ice number fraction, or ice spatial ratio. Aerosol indirect effects are quantified for different transition phases using number concentrations of aerosols greater than 100 nm or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice nucleating particles, which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant on the earlier transition phase when ice crystals just start to appear compared with the later transition phase. The thermodynamic and dynamic conditions are quantified for each transition phase. The results show in-cloud turbulence as a main mechanism for both the initiation of ice nucleation and the maintenance of supercooled liquid water, while updrafts are important for the latter but not the former. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics throughout cloud evolution based on this new method that categorizes cloud transition phases. 

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2. Ice and Supercooled Liquid Water Distributions Over the Southern Ocean Based on In Situ Observations and Climate Model Simulations

   https://doi.org/10.1029/2021JD036045  

   Yang, Ching An; Diao, Minghui; Gettelman, Andrew; Zhang, Kai; Sun, Jian; McFarquhar, Greg; Wu, Wei (December 2021, Journal of Geophysical Research: Atmospheres)

   Abstract Three climate models are evaluated using in situ airborne observations from the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) campaign. The evaluation targets cloud phases, microphysical properties, thermodynamic conditions, and aerosol indirect effects from −40°C to 0°C. Compared with 580‐s averaged observations (i.e., 100 km horizontal scale), the Community Atmosphere Model version 6 (CAM6) shows the most similar result for cloud phase frequency distribution and allows more liquid‐containing clouds below −10°C compared with its predecessor—CAM5. The Energy Exascale Earth System Model (E3SM) underestimates (overestimates) ice phase frequencies below (above) −20°C. CAM6 and E3SM show liquid and ice water contents (i.e., LWC and IWC) similar to observations from −25°C to 0°C, but higher LWC and lower IWC than observations at lower temperatures. Simulated in‐cloud RH shows higher minimum values than observations, possibly restricting ice growth during sedimentation. As number concentrations of aerosols larger than 500 nm (Na₅₀₀) increase, observations show increases of LWC, IWC, liquid, and ice number concentrations (N_liq, N_ice). Number concentrations of aerosols larger than 100 nm (Na₁₀₀) only show positive correlations with LWC and N_liq. From −20°C to 0°C, higher aerosol number concentrations are correlated with lower glaciation ratio and higher cloud fraction. From −40°C to −20°C, large aerosols show positive correlations with glaciation ratio. CAM6 shows small increases of LWC and N_liqwith Na₅₀₀and Na₁₀₀. E3SM shows small increases of N_icewith Na₅₀₀. Overall, CAM6 and E3SM underestimate aerosol indirect effects on ice crystals and supercooled liquid droplets over the Southern Ocean. 

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3. Characterizing the Occurrence and Spatial Heterogeneity of Liquid, Ice, and Mixed Phase Low‐Level Clouds Over the Southern Ocean Using in Situ Observations Acquired During SOCRATES

   https://doi.org/10.1029/2020JD034482  

   D'Alessandro, John J.; McFarquhar, Greg M.; Wu, Wei; Stith, Jeff L.; Jensen, Jorgen B.; Rauber, Robert M. (June 2021, Journal of Geophysical Research: Atmospheres)

   Abstract Supercooled liquid water (SLW) and mixed phase clouds containing SLW and ice over the Southern Ocean (SO) are poorly represented in global climate and numerical weather prediction models. Observed SLW exists at lower temperatures than threshold values used to characterize its detrainment from convection in model parameterizations, and processes controlling its formation and removal are poorly understood. High‐resolution observations are needed to better characterize SLW over the SO. This study characterizes the frequency and spatial distribution of different cloud phases (liquid, ice, and mixed) using in situ observations acquired during the Southern Ocean Clouds, Radiation, Aerosol Transport Experiment Study. Cloud particle phase is identified using multiple cloud probes. Results show occurrence frequencies of liquid phase samples up to 70% between −20°C and 0°C and of ice phase samples up to 10% between −5°C and 0°C. Cloud phase spatial heterogeneity is determined by relating the total number of 1 s samples from a given cloud to the number of segments whose neighboring samples are the same phase. Mixed phase conditions are the most spatially heterogeneous from −20°C to 0°C, whereas liquid phase conditions from −10°C to 0°C and ice phase conditions from −20°C to −10°C are the least spatially heterogeneous. Greater spatial heterogeneity is associated with broader distributions of vertical velocity. Decreasing droplet concentrations and increasing number‐weighted mean liquid diameters occur within mixed phase clouds as the liquid water fraction decreases, possibly suggesting preferential evaporation of smaller drops during the Wegener‐Bergeron‐Findeisen process. 

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4. A Case Study of Cloud Microphysical Response to Cloud Seeding in Wintertime Orographic Clouds

   https://doi.org/10.1175/JAMC-D-25-0001.1  

   Xie, Zhixing; Friedrich, Katja; Xue, Lulin; Chen, Sisi; Tessendorf, Sarah A; French, Jeffery R; Hohman, Christopher C (September 2025, Journal of Applied Meteorology and Climatology)

   Abstract Cloud seeding has been widely used for enhancing wintertime snowfall, particularly to augment water resources. This study examines microphysical responses to airborne glaciogenic seeding with silver iodide (AgI) during a specific case from the Seeded and Natural Orographic Wintertime Clouds: Idaho Experiment (SNOWIE) on 11 January 2017. Ground-based and airborne remote sensing and in situ measurements were employed to assess the impact of cloud seeding on cloud properties and precipitation formation. On 11th January, AgI propagated downwind along prevailing winds, and any potential ice and snow particles created from it were identified by ground-based radar as zigzag lines of enhanced reflectivity compared to background reflectivity. As the aircraft flew several times through these seeded clouds, microphysical properties within seeded clouds can be compared to those observed in unseeded clouds. The results indicate that seeded clouds exhibited significantly enhanced ice water content (IWC; reaching up to 0.20 g m⁻³) and precipitating-size (>400μm) ice particle concentrations (>7 L⁻¹) relative to unseeded clouds. Additionally, seeded clouds exhibited a 30% decrease in the mean liquid water content (LWC) and cloud droplet concentrations, indicating efficient glaciation processes influenced by AgI. Precipitating snow development in seeded clouds occurred within 15–40 min following AgI release, marked by a transition from mixed-phase clouds with abundant supercooled liquid water (SLW) to ice clouds, with lidar-measured linear depolarization ratio (LDR) increasing to >0.3. These findings underscore the effectiveness of cloud seeding in enhancing snowfall by facilitating ice initiation and growth. Significance StatementThis study investigates the microphysical response of wintertime orographic clouds to airborne glaciogenic seeding, highlighting its role in enhancing precipitation. By introducing silver iodide (AgI) into clouds with supercooled liquid water, the seeding process facilitates ice particle formation, leading to increased snowfall. Through a detailed analysis of microphysical conditions using advanced in situ and remote sensing instruments, the study reveals enhanced ice water content and efficient conversion of liquid water to ice in seeded clouds. These findings provide critical insights into cloud-seeding efficacy, particularly in regions with abundant supercooled liquid water, offering a scientific foundation for enhancing snowpack in water-scarce mountainous areas. 

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5. Hemispheric Asymmetry of Phase Partition in Mixed‐Phase Clouds Based on Near Global‐Scale Airborne Observations

   https://doi.org/10.1029/2025GL115946  

   Yang, Ching_An; Diao, Minghui; Shi, Yang; Liu, Xiaohong (September 2025, Geophysical Research Letters)

   Abstract Mixed‐phase clouds contribute to substantial uncertainties in global climate models due to their complex microphysical properties. Former model evaluations almost exclusively rely on satellite observations to assess cloud phase distributions globally. This study investigated mixed‐phase cloud properties using near global‐scale in situ observation data sets from 14 flight campaigns in combination with collocated output from a global climate model. The Southern Hemisphere (SH) shows significantly higher occurrence frequencies and higher mass fractions of supercooled liquid water than Northern Hemisphere (NH) based on observations at 0.2 and 100 km horizontal scales. Such hemispheric asymmetry is not captured by the model. The model also consistently overestimates liquid water content (LWC) in all cloud phases but shows ice water content (IWC) biases that vary with phase. Key processes contributing to model biases in phase partition can be identified through the combination of evaluation of phase frequency, liquid mass fraction, LWC and IWC. 

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