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Title: Resonant X-ray excitation of the nuclear clock isomer 45Sc
Abstract Resonant oscillators with stable frequencies and large quality factors help us to keep track of time with high precision. Examples range from quartz crystal oscillators in wristwatches to atomic oscillators in atomic clocks, which are, at present, our most precise time measurement devices1. The search for more stable and convenient reference oscillators is continuing2–6. Nuclear oscillators are better than atomic oscillators because of their naturally higher quality factors and higher resilience against external perturbations7–9. One of the most promising cases is an ultra-narrow nuclear resonance transition in45Sc between the ground state and the 12.4-keV isomeric state with a long lifetime of 0.47 s (ref. 10). The scientific potential of45Sc was realized long ago, but applications require45Sc resonant excitation, which in turn requires accelerator-driven, high-brightness X-ray sources11that have become available only recently. Here we report on resonant X-ray excitation of the45Sc isomeric state by irradiation of Sc-metal foil with 12.4-keV photon pulses from a state-of-the-art X-ray free-electron laser and subsequent detection of nuclear decay products. Simultaneously, the transition energy was determined as$${\mathrm{12,389.59}}_{+0.12\left({\rm{syst}}\right)}^{\pm 0.15\left({\rm{stat}}\right)}\,{\rm{eV}}$$ 12,389.59 + 0.12 syst ± 0.15 stat eV with an uncertainty that is two orders of magnitude smaller than the previously known values. These advancements enable the application of this isomer in extreme metrology, nuclear clock technology, ultra-high-precision spectroscopy and similar applications.  more » « less
Award ID(s):
2012194
PAR ID:
10545989
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more » ; ; ; ; ; ; ; ; ; ; ; ; ; « less
Publisher / Repository:
Nature Portfolio
Date Published:
Journal Name:
Nature
Volume:
622
Issue:
7983
ISSN:
0028-0836
Page Range / eLocation ID:
471 to 475
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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