Abstract Existing motor vehicle pollutant measurement techniques, including those that employ ground-based and multirotor small uncrewed aircraft system (sUAS) methods, can accurately measure traffic-related air pollution (TRAP) concentrations at a single location. However, these techniques often lack the mobility to assess pollutant trends across a large horizontal area. Fixed-wing sUAS represents an alternative instrument platform compared to ground-based systems and multirotor sUAS, as fixed-wing sUASs are able to carry air pollutant monitor payloads, have extended endurance, and offer expansive three-dimensional ranges across a field site. To demonstrate the utility of fixed-wing sUAS for urban TRAP assessment, we conducted two flights using a Super Robust Autonomous Aerial Vehicle–Endurant Nimble (RAAVEN) sUAS [University of Colorado (CU) Boulder] at a large field site adjacent to a major highway in Erie, Colorado. Concentrations of solid particulate matter (PM10) and gas-phase (carbon monoxide) pollutants displayed decay as a function of altitude. During the morning flight, PM10concentrations decreased from 19.0μg m−3at ground level to a minimum concentration of 14.3μg m−3at 90 m above ground level. During the afternoon flight, concentrations of PM10displayed minimal vertical stratification, ranging from 8.9 at ground level to 10.0μg m−3at 45 m above ground level. Similarly, pollutants displayed decreasing concentrations as the horizontal distance from the roadway increased. Concentrations of TRAP may be significantly elevated in the area both above and beyond roadways, which contribute to additional pollutant exposure from on-road pollution sources. This study demonstrated that the general behavior of TRAP in near-road environments and that the use of fixed-wing sUAS are viable option for urban air quality measurements. Significance StatementThis study represents one of the first uses of a fixed-wing small uncrewed aircraft system (sUAS) to assess near-roadside concentrations of traffic-related air pollution (TRAP) in urbanized areas. We found that local meteorology, including local wind and solar radiation, had a substantial influence on the concentrations of common air pollutants, including particulate matter, black carbon, carbon monoxide, and carbon dioxide. Furthermore, we found large-scale spatiotemporal variation in pollutant concentrations as a function of the vertical and horizontal distance from the highway, indicating that diminished spatial variation employed in multirotor sUAS studies may not be sufficient to fully assess TRAP in roadside environments.
more »
« less
Spatiotemporal air quality prediction using stochastic advection–diffusion model for multimodal data fusion
Abstract Particulate matter poses significant risks to respiratory and cardiovascular health. Monitoring ambient particulate matter concentrations can provide information on potential exposures and inform mitigation strategies, but ground-based measurements are sparse. Data fusion approaches that integrate data from multiple sources can complement existing observation networks and reveal insights that single-sensor data might miss to better manage pollutant exposure risks. However, data fusion approaches face multiple challenges, including incompatible measurement units, varying data resolutions, and differing levels of uncertainty. As a result, the optimal method for data fusion remains an open question. Here, we propose a probabilistic spatiotemporal model, based on the stochastic advection–diffusion (SAD) equation, as a data fusion method to process multimodal air quality data to predict hourly concentrations of fine particulate matter (PM2.5). We employ a variational inference method to calibrate the probabilistic model using ground-level observations and the numerical output of two simulation models. We then evaluate the prediction performance of our model for two scenarios: (1) incorporating simulation outputs and ground-level observations from sparse regulatory-grade stations and (2) using ground-level observations from both low-cost and regulatory-grade stations. For the first scenario, the data fusion method reduces prediction error by 14% compared to the nearest regulatory-grade air monitor located 20 km away. For the second scenario, error is reduced by 40% compared to the nearest regulatory-grade monitor and 11% compared to the nearest low-cost sensor located approximately 1 km away. The model captures 78% of observed data within a 75% confidence interval across both scenarios, demonstrating its ability to accurately represent uncertainty. Our findings demonstrate that the proposed SAD model can effectively integrate multimodal data to provide improved prediction of particulate matter concentrations at high spatial resolution. Model outputs can inform individual and community-level decision-making to mitigate air pollutant exposures.
more »
« less
- Award ID(s):
- 2231557
- PAR ID:
- 10565360
- Publisher / Repository:
- IOP Publishing
- Date Published:
- Journal Name:
- Environmental Research Letters
- Volume:
- 20
- Issue:
- 1
- ISSN:
- 1748-9326
- Format(s):
- Medium: X Size: Article No. 014065
- Size(s):
- Article No. 014065
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
— In this paper, we first develop a low-cost surfacebased air pollutants measurement system for the real-time air pollution monitoring and forecasting applications. Then, we compare the performance achieved by the proposed system in real-time urban environment with currently used static monitoring stations by the governmental environmental protection agency (EPA). The proposed design uses particulate matter, humidity, and temperature sensors to measure the values of the air pollutant that determines the value of the Air Quality Index (AQI). The SD storage device is interfaced with the system to store the large amount of data sensed by the system. The Arduino UNO-based processing unit integrates with the sensing units to process and control the sensed air pollutants data. The proposed system is deployed in indoors and outdoor environment in under served minority communities in big cities to illustrate real-time environmental pollution measurement and monitoring applications. The system can measure, monitor and alert the level of PM2.5 and PM10 components of the AQI as they are often the main pollutant that determines the AQI value. The performance of the proposed system compares with the expensive data logger-based EPA-approved LDEQ sensorsbased air quality monitoring system. Our analysis shows that the measurement and monitoring performance of the proposed system is comparable with the EPA-approved LDEQ sensorsbased air quality monitoring system. The analysis also shows that there is a spatial and temporal variation of PM2.5 and PM10 values even for sites that are less than a mile apart. The interaction interphase of the system is simpler and easier to use as compared with bulky display systems in traditional EPA-based monitoring systems. In contrast with the traditional data logger-based system, the proposed system is smaller and quicker to deploy to test specific air pollutants in interested urban and rural locations .more » « less
-
Introduction:Traditional methods to estimate exposure to PM2.5(particulate matter with less than 2.5 µm in diameter) have typically relied on limited regulatory monitors and do not consider human mobility and travel. However, the limited spatial coverage of regulatory monitors and the lack of consideration of mobility limit the ability to capture actual air pollution exposure. Methods:This study aims to improve traditional exposure assessment methods for PM2.5by incorporating the measurements from a low-cost sensor network (PurpleAir) and regulatory monitors, an automated machine learning modeling framework, and big human mobility data. We develop a monthly-aggregated hourly land use regression (LUR) model based on automated machine learning (AutoML) and assess the model performance across eight metropolitan areas within the US. Results:Our results show that integrating low-cost sensor with regulatory monitor measurements generally improves the AutoML-LUR model accuracy and produces higher spatial variation in PM2.5concentration maps compared to using regulatory monitor measurements alone. Feature importance analysis shows factors highly correlated with PM2.5concentrations, including satellite aerosol optical depth, meteorological variables, vegetation, and land use. In addition, we incorporate human mobility data on exposure estimates regarding where people visit to identify spatiotemporal hotspots of places with higher risks of exposure, emphasizing the need to consider both visitor numbers and PM2.5concentrations when developing exposure reduction strategies. Discussion:This research provides important insights for further public health studies on air pollution by comprehensively assessing the performance of AutoML-LUR models and incorporating human mobility into considering human exposure to air pollution.more » « less
-
In urban areas like Chicago, daily life extends above ground level due to the prevalence of high-rise buildings where residents and commuters live and work. This study examines the variation in fine particulate matter (PM2.5) concentrations across building stories. PM2.5 levels were measured using PurpleAir sensors, installed between 8 April and 7 May 2023, on floors one, four, six, and nine of an office building in Chicago. Additionally, data were collected from a public outdoor PurpleAir sensor on the fourteenth floor of a condominium located 800 m away. The results show that outdoor PM2.5 concentrations peak at 14 m height, and then decline by 0.11 μg/m3 per meter elevation, especially noticeable from midnight to 8 a.m. under stable atmospheric conditions. Indoor PM2.5 concentrations increase steadily by 0.02 μg/m3 per meter elevation, particularly during peak work hours, likely caused by greater infiltration rates at higher floors. Both outdoor and indoor concentrations peak around noon. We find that indoor and outdoor PM2.5 are positively correlated, with indoor levels consistently remaining lower than outside levels. These findings align with previous research suggesting decreasing outdoor air pollution concentrations with increasing height. The study informs decision-making by community members and policymakers regarding air pollution exposure in urban settings.more » « less
-
Abstract. Aerosol particles are an important part of the Earth climate system, and their concentrations are spatially and temporally heterogeneous, as well as being variable in size and composition. Particles can interact with incoming solar radiation and outgoing longwave radiation, change cloud properties, affect photochemistry, impact surface air quality, change the albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. High particulate matter concentrations at the surface represent an important public health hazard. There are substantial data sets describing aerosol particles in the literature or in public health databases, but they have not been compiled for easy use by the climate and air quality modeling community. Here, we present a new compilation of PM2.5 and PM10 surface observations, including measurements of aerosol composition, focusing on the spatial variability across different observational stations. Climate modelers are constantly looking for multiple independent lines of evidence to verify their models, and in situ surface concentration measurements, taken at the level of human settlement, present a valuable source of information about aerosols and their human impacts complementarily to the column averages or integrals often retrieved from satellites. We demonstrate a method for comparing the data sets to outputs from global climate models that are the basis for projections of future climate and large-scale aerosol transport patterns that influence local air quality. Annual trends and seasonal cycles are discussed briefly and are included in the compilation. Overall, most of the planet or even the land fraction does not have sufficient observations of surface concentrations – and, especially, particle composition – to characterize and understand the current distribution of particles. Climate models without ammonium nitrate aerosols omit ∼ 10 % of the globally averaged surface concentration of aerosol particles in both PM2.5 and PM10 size fractions, with up to 50 % of the surface concentrations not being included in some regions. In these regions, climate model aerosol forcing projections are likely to be incorrect as they do not include important trends in short-lived climate forcers.more » « less
An official website of the United States government
