skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: When van der Waals Met Kagome: A 2D Antimonide with a Vanadium-Kagome Network
Award ID(s):
1944551
PAR ID:
10572172
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
American Chemical Society
Date Published:
Journal Name:
Journal of the American Chemical Society
Volume:
146
Issue:
39
ISSN:
0002-7863
Page Range / eLocation ID:
26786 to 26800
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract Topological kagome magnets RMn6Sn6(R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd0.38Tb0.27Dy0.20Ho0.15)Mn6Sn6. Such a high entropy material exhibits multiple spin reorientation transitions, which is not seen in all the related parent compounds and can be understood in terms of competing magnetic interactions enabled by high entropy. Furthermore, we also observed an intrinsic anomalous Hall effect, indicating that the high entropy phase preserves the non-trivial band topology. These results suggest that high entropy may provide a route to engineer the magnetic structure and expand the horizon of topological materials. 
    more » « less
  2. Whenever the elastic energy of a solid depends on magnetic field, there is a magnetostrictive response. Field-linear magnetostriction implies piezo- magnetism and vice versa. Here, we show that Mn3Sn, a non-collinear anti- ferromanget with Weyl nodes, hosts a large and almost perfectly linear magnetostriction even at room temperature. The longitudinal and transverse magnetostriction, with opposite signs and similar amplitude are restricted to the kagome planes and the out-of-plane response is negligibly small. By studying four different samples with different Mn:Sn ratios, we find a clear correlation between the linear magnetostriction, the spontaneous magneti- zation and the concentration of Sn vacancies. The recently reported piezo- magnetic data fits in our picture. We show that linear magnetostriction and piezomagnetism are both driven by the field-induced in-plane twist of spins. A quantitative account of the experimental data requires the distortion of the spin texture by Sn vacancies. We find that the field-induced domain nucleation within the hysteresis loop corresponds to a phase transition. Within the hys- teresis loop, a concomitant mesoscopic modulation of local strain and spin twist angles, leading to twisto-magnetic stripes, arises as a result of the com- petition between elastic and magnetic energies. 
    more » « less
  3. null (Ed.)
    We analyze the zero-temperature phases of an array of neutral atoms on the kagome lattice, interacting via laser excitation to atomic Rydberg states. Density-matrix renormalization group calculations reveal the presence of a wide variety of complex solid phases with broken lattice symmetries. In addition, we identify a regime with dense Rydberg excitations that has a large entanglement entropy and no local order parameter associated with lattice symmetries. From a mapping to the triangular lattice quantum dimer model, and theories of quantum phase transitions out of the proximate solid phases, we argue that this regime could contain one or more phases with topological order. Our results provide the foundation for theoretical and experimental explorations of crystalline and liquid states using programmable quantum simulators based on Rydberg atom arrays. 
    more » « less