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Abstract High-order harmonic generation (HHG) has become an indispensable process for generating attosecond pulse trains and single attosecond pulses used in the observation of nuclear and electronic motion. As such, improved control of the HHG process is desirable, and one such possibility for this control is through the use of structured laser pulses. We present numerical results from solving the one-dimensional time-dependent Schrödinger equation for HHG from hydrogen using Airy and Gaussian pulses that differ only in their spectral phase. Airy pulses have identical power spectra to Gaussian pulses, but different spectral phases and temporal envelopes. We show that the use of Airy pulses results in less ground state depletion compared to the Gaussian pulse, while maintaining harmonic yield and cutoff. Our results demonstrate that Airy pulses with higher intensity can produce similar HHG spectra to lower intensity Gaussian pulses without depleting the ground state. The different temporal envelopes of the Gaussian and Airy pulses lead to changes in the dynamics of the HHG process, altering the time-dependence of the ground state population and the emission times of the high harmonics. Graphical abstract
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Pulse characterization via two-photon auto- and cross-correlation
We present the application of a previously proposed multiple-Gaussian approach to characterize ultrashort vacuum (VUV) and deep ultraviolet (DUV) pulses via auto- and cross-correlation methods. The knowledge of the temporal variation of amplitude and phase of such pulses is important for spectroscopic and dynamical imaging techniques. The method, which is an extension of the single Gaussian autocorrelation technique, is based on the expansion of the pulse in a series of Gaussian functions at different frequencies and the use of analytic solutions for two-photon ionization of atoms by Gaussian pulses. Using this approach we compare the characterization of a pulse via the auto- and the cross-correlation techniques and find that an accurate characterization even in the case of more complex pulse forms can be achieved. Furthermore, the comparison of the application of unchirped and chirped Gaussian pulses reveals some specific advantages in the use of pulses with a linear chirp. Finally, we quantify our conclusions from the qualitative comparisons by defining errors and using results from information theory.
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- Award ID(s):
- 2207995
- PAR ID:
- 10620814
- Publisher / Repository:
- Optica Publishing Group
- Date Published:
- Journal Name:
- Optics Express
- Volume:
- 32
- Issue:
- 20
- ISSN:
- 1094-4087
- Page Range / eLocation ID:
- 34732
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
-
Accepted Manuscript
- Journal Article:
- https://doi.org/10.1364/OE.533612
