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			<titleStmt><title level='a'>Numerical simulations of laser-driven experiments of ion acceleration in stochastic magnetic fields</title></titleStmt>
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				<publisher>AIP Publishing</publisher>
				<date>12/01/2024</date>
			</publicationStmt>
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				<bibl> 
					<idno type="par_id">10621046</idno>
					<idno type="doi">10.1063/5.0223496</idno>
					<title level='j'>Physics of Plasmas</title>
<idno>1070-664X</idno>
<biblScope unit="volume">31</biblScope>
<biblScope unit="issue">12</biblScope>					

					<author>K Moczulski</author><author>H Wen</author><author>T Campbell</author><author>A Scopatz</author><author>C_A J Palmer</author><author>A_F A Bott</author><author>C D Arrowsmith</author><author>K A Beyer</author><author>A Blazevic</author><author>V Bagnoud</author><author>S Feister</author><author>J Halliday</author><author>O Karnbach</author><author>M Metternich</author><author>H Nazary</author><author>P Neumayer</author><author>A Reyes</author><author>E C Hansen</author><author>D Schumacher</author><author>C Spindloe</author><author>S Sarkar</author><author>A R Bell</author><author>R Bingham</author><author>F Miniati</author><author>A A Schekochihin</author><author>B Reville</author><author>D Q Lamb</author><author>G Gregori</author><author>P Tzeferacos</author>
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			<abstract><ab><![CDATA[<p>We present numerical simulations used to interpret laser-driven plasma experiments at the GSI Helmholtz Centre for Heavy Ion Research. The mechanisms by which non-thermal particles are accelerated in astrophysical environments, e.g., the solar wind, supernova remnants, and gamma ray bursts, is a topic of intense study. When shocks are present, the primary acceleration mechanism is believed to be first-order Fermi, which accelerates particles as they cross a shock. Second-order Fermi acceleration can also contribute, utilizing magnetic mirrors for particle energization. Despite this mechanism being less efficient, the ubiquity of magnetized turbulence in the universe necessitates its consideration. Another acceleration mechanism is the lower-hybrid drift instability, arising from gradients of both density and magnetic field, which produce lower-hybrid waves with an electric field that energizes particles as they cross these waves. With the combination of high-powered laser systems and particle accelerators, it is possible to study the mechanisms behind cosmic-ray acceleration in the laboratory. In this work, we combine experimental results and high-fidelity three-dimensional simulations to estimate the efficiency of ion acceleration in a weakly magnetized interaction region. We validate the FLASH magneto-hydrodynamic code with experimental results and use OSIRIS particle-in-cell code to verify the initial formation of the interaction region, showing good agreement between codes and experimental results. We find that the plasma conditions in the experiment are conducive to the lower-hybrid drift instability, yielding an increase in energy ΔE of ∼264keV for 242MeV calcium ions.</p>]]></ab></abstract>
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<div xmlns="http://www.tei-c.org/ns/1.0"><head>I. INTRODUCTION</head><p>Cosmic rays have been studied for well over a century, and it was only in the 1910's that we realized they came not from the Earth's crust, but bombarded the Earth's upper atmosphere <ref type="bibr">1,</ref><ref type="bibr">2</ref> . Despite more than a century of investigation, both the sites of acceleration <ref type="bibr">3</ref> and plasma processes <ref type="bibr">4</ref> that generate the range of energies measured in cosmic rays remain open questions, and thus topics of active research.</p><p>The energization mechanisms that are expected to operate in astrophysical systems rely on collisionless interaction with the electric and magnetic fields supported by the tenuous plasmas typical of these environments. The most widely invoked acceleration mechanism in astrophysics is diffusive shock acceleration <ref type="bibr">[5]</ref><ref type="bibr">[6]</ref><ref type="bibr">[7]</ref><ref type="bibr">[8]</ref> , an example of a first order Fermi mechanism. Two key requirements for such mechanisms to occur are the ability to lift a subset of particles from the thermal gas to energies where they decouple from the bulk flow, and a scattering process that can sustain the acceleration and lead to the formation of a non-thermal component, i.e., not simply a heating process. Both processes rely on the interplay between particle transport and plasma turbulence. Large scale kinetic simulations of shocks suggest that the diffusive shock acceleration process can be efficient under a broad range of plasma environmental conditions <ref type="bibr">9</ref> . Moreover, satellite measurements present compelling evidence for energization due to interactions with whistler <ref type="bibr">10</ref> as well as lower-hybrid <ref type="bibr">11</ref> waves in the case of electrons, or ion-cyclotron modes <ref type="bibr">12</ref> in the case of ions. These provide possible routes to injecting particles into the shock acceleration process. More recently, laboratory experiments and simulations of collisionless shocks have shown electron and ion spectra consistent with shock acceleration predictions <ref type="bibr">[13]</ref><ref type="bibr">[14]</ref><ref type="bibr">[15]</ref> .</p><p>That said, particle acceleration does not occur only at shocks. The acceleration mechanism originally proposed by Fermi <ref type="bibr">16</ref> posited that particles are accelerated through repeated interaction with moving magnetic field structures. In the original picture, charged particles propagating through a magnetized medium can interact with magnetic fields, the latter acting as mirrors changing the particle energy proportional to the mirror velocity. If a mirror is moving toward a particle, it will result in an energy increase. Conversely if receding, the particle gets decelerated. Unlike at shocks, where there exists a clear preferred direction, here the mirrors are assumed to be randomly oriented and the resulting energy gain averaged over many interactions is thus second order in the mirrors' velocity <ref type="bibr">17,</ref><ref type="bibr">18</ref> . While less efficient than first-order Fermi, the large extent of interstellar and intracluster mediums can increase the likelihood of meaningful contributions from second-order Fermi acceleration. Hence it is expected to modify, rather than dominate the cosmic ray spectrum <ref type="bibr">19</ref> . Despite detailed theoretical studies <ref type="bibr">20,</ref><ref type="bibr">21</ref> laboratory evidence of second-order Fermi ion acceleration has remained elusive.</p><p>Inhomogeneous environments, which are common in astrophysical contexts, can also lead to instabilities. The lowerhybrid drift instability, which develops from misaligned gradients of density and magnetic field, is one such example <ref type="bibr">22</ref> . When these gradients are present lower-hybrid waves can develop, generating electric fields that in turn accelerate charged particles. Theoretical models have been proposed to explain the hard X-ray tail emission in Cassiopeia, arguing the lowerhybrid drift instability provides the necessary acceleration for electrons <ref type="bibr">23</ref> . Simulations have expanded upon the quasi-linear theoretical framework <ref type="bibr">22</ref> , and have demonstrated electrons can be self-consistently accelerated <ref type="bibr">24</ref> . Measurements of accelerated auroral electrons have been analyzed, showing lowerhybrid waves as the cause of acceleration <ref type="bibr">25</ref> . Space probes have measured the lower-hybrid drift instability in the magnetotail current sheet <ref type="bibr">26</ref> , showing that lower-hybrid waves are generated at the separatrix. In the laboratory, high-power laser experiments have demonstrated electron acceleration from reflected ions in analogy to the solar wind interacting with a comet <ref type="bibr">27</ref> .</p><p>While many acceleration mechanisms may be operating in astrophysical environments, laboratory experiments offer the advantage of tailoring plasma conditions to probe individual mechanisms. The objective of this paper is to model experiments which measure ion acceleration in a stochastic magnetized plasma at the GSI Helmholtz Centre for Heavy Ion Research facility <ref type="bibr">28</ref> . We use a platform similar to that fielded previously to study fluctuation dynamo <ref type="bibr">[29]</ref><ref type="bibr">[30]</ref><ref type="bibr">[31]</ref><ref type="bibr">[32]</ref><ref type="bibr">[33]</ref><ref type="bibr">[34]</ref> , coupled with the The UNIversal Linear ACcelerator (UNILAC) of the GSI to launch well-characterized ions through a stochastic magnetic field. Utilizing the radiation-magneto-hydrodynamic (MHD) code FLASH, and the particle-in-cell (PIC) code OSIRIS, we calculate the plasma conditions along the calcium-ion flight path. From the plasma conditions achieved, we can estimate the efficiency of the various acceleration mechanisms and identify the dominant one. Experimental results from a campaign were used to validate the predictive capabilities of the FLASH code.</p><p>In Section II we explain the platform employed at the GSI Helmholtz Centre as well as the initialization of the FLASH simulation. Section III describes the simulation results, the temporal evolution of the plasma, plasma conditions achieved, and compares the simulated results to the experiment results. In Section IV we estimate energization of the UNILAC ions from the plasma conditions obtained. The experimental campaign was carried out at the GSI Helmholtz Institute for Heavy Ion research in Darmstadt, Germany, to observe ion acceleration in a stochastic magnetic field. The experimental configuration is shown in Fig. <ref type="figure">1</ref>. Two 20-&#181;m thick, 1-mm diameter CH foils are separated by 1.95 mm. These foils are machined to have a grooved pattern on their inner surface, facing the opposing targets. The grooves consist of ridges 10 &#181;m in height, which are 20-&#181;m wide, with a 60-&#181;m spacing between them.</p><p>Two lasers, NHELIX (Nanosecond High Energy Laser for Ion beam eXperiments) and PHELIX (Petawatt High-Energy Laser for Heavy Ion EXperiments), are used to ablate two targets and form a colliding plasma. The UNILAC generates Ca +18 ions with an energy of 242 MeV (5.052 MeV per nucleon) and spread in energy of 0.1%. The ions are directed through the center of the experimental chamber, between the two targets, forming a 100-&#181;m diameter, traveling into a diamond detector on the other side of the chamber (see also Fig. <ref type="figure">1</ref>). An optical spectroscopy diagnostic collects light from over a path integrated area with a 4.0 mm diameter, encompassing the two target, to measure electron density, electron temperature, and the RMS (root-mean-square) velocity.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>B. FLASH configuration</head><p>To model this experiment, we utilized the FLASH code. FLASH <ref type="bibr">35,</ref><ref type="bibr">36</ref> is a publicly available, high-performance computing, multi-physics, adaptive mesh refinement (AMR), finite-volume Eulerian hydrodynamics and MHD code <ref type="bibr">37</ref>  As the jets propagate and collide in the center, forming the interaction region (the region bounded by two reverse shocks), their temperature increases to over 500 eV (e). At later times, the material has cooled down to 10s of eV (f). (g) Rendering of the magnetic field at t = 2 ns. The magnetic field is generated through Biermann-battery laser-target interaction and is advected toward the center of the domain with the plasma flow. As the magnetic field reaches the center of the domain, it is flux-compressed and increased by &#8764; 15% (h). At late times, the magnetic field strength in the interaction region is higher than the surrounding region, but lower than what observed at earlier times (i).</p><p>FLASH has extensive high-energy-density physics (HEDP) capabilities 36 incorporated in recent years, which enable it to model laser-plasma experiments. HEDP experiments typically cannot be described by a thermal equilibrium between electrons, ions, and radiation. Therefore, we employ a threetemperature (3T) description to solve the extended radiation-MHD equations that describe our system. We also leverage other capabilities in FLASH such as laser ray-tracing, radiation diffusion, and multi-material EOS and opacities. For a detailed explanation see Tzeferacos et al. <ref type="bibr">36,</ref><ref type="bibr">38</ref> The 3D FLASH simulations were configured to replicate the experiments. The simulation domain extends 1.28 mm in X and Y and 3.84 mm in Z. The domain is resolved with &#8764;6.3&#215;10 6 cells, with a spacing of 10 &#181;m, which is sufficient to fully resolve the grooves, recesses, and target thickness. Outflow boundary conditions are employed to emulate the large experimental campaign. These boundary conditions fix the gradients of the flow properties to zero, except for the normal component of the magnetic field, which is set through the solenoidality condition. The multi-group, flux-limited radiation diffusion scheme uses 6 energy groups that range from 0.1 eV to 100 keV. For heat exchange, magnetic resistivity, and electron thermal conductivity, the Spitzer formula are used <ref type="bibr">39</ref> . The generation of the magnetic field is modeled using a generalized Ohm's law, which includes the resistive and Biermann-battery terms <ref type="bibr">40,</ref><ref type="bibr">41</ref> .</p><p>Two CH foils are initialized in the domain, using the parameters from the experimental platform. To accurately model the EOS and opacity of CH, a PROPACEOS 42 table is used. The density of the material is set to 1.04 g cm -3 and the initial temperature is set to room temperature. The remaining computational domain is filled with He at 1.0 &#215; 10 -6 g cm -3 and room temperature.</p><p>The NHELIX and PHELIX beams, each simulated using 10,000 rays, have a Gaussian radial profile with 100-&#181;m Gaussian FWHM (full-width at half-maximum) radius of the focal spot. The PHELIX's laser wavelength is set to 1,053 nm while NHELIX's is set to 1,064 nm. The beam power is described by a 3-ns ramp up, 4-ns plateau, and 3-ns ramp down, with a plateau power of 7.85 &#215; 10 9 W.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>III. EVOLUTION OF THE EXPERIMENT</head><p>Here we describe the temporal evolution of the experiment as seen in the 3D FLASH simulations. The evolution consists of three distinct phases. Phase I describes the laser ablation of the targets, which generates two fully ionized, counterpropagating jets. Phase II begins when the jets collide between the targets. During this phase, 1D OSIRIS and FLASH simulations are employed to assess the impact of kinetic effects during the formation of the interaction region, which is the region bounded by two reverse shocks. Finally, Phase III describes the temporal evolution and relaxation of the interaction region.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>A. Phase I: Jet generation and propagation</head><p>The temporal evolution in the simulation is shown in Fig. <ref type="figure">2</ref>. The inner face of each target is illuminated by a single beam, absorbing laser energy through electron free-free absorption, otherwise known as inverse bremsstrahlung. This results in ablation of the targets, generating two expanding, supersonic, fully ionized, asymmetric jets. The laser-target interaction generates Biermann-battery magnetic fields <ref type="bibr">43,</ref><ref type="bibr">44</ref> , which are flux-frozen into the expanding jets and advected with the jets into the center of the domain. The jets retain a density variation, as a result of the grooved pattern present on the target surface. The properties of the jets are summarized in Table <ref type="table">I</ref>. Approximately 3 ns after the laser is turned on, the jets collide in the center of the domain. Phase I concludes with the collision of the two jets.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>B. Phase II: Collision and counter-streaming</head><p>While the two jets are well described by a Maxwellian distribution, this function cannot describe the immediately postcollision plasma. The velocity (4.1 &#215; 10 7 cm s -1 ) and density (2.2 &#215; 10 18 carbon ions cm -3 ) at the jet front have an inter-jet carbon-ion mean-free path <ref type="bibr">45</ref> (eq. 14.12)</p><p>where A is the carbon-ion mass, n c is the carbon-ion density, Z is the charge of the carbon ions, and U is the jet velocity (which is the jet's relative velocity). Thus the inter-jet mean free path of the carbon ions is significantly larger than the 1mm distance the jets can counter-propagate before hitting the opposing target, giving rise to counter-streaming flows. While the initial plasma properties at the jet front yield inter-jet mean free paths larger than the system size, the velocities decrease and densities increase at later times, shortening the inter-jet mean free path. This counter-streaming cannot be accurately modeled in a single-fluid MHD simulation and therefore we need to assess how it affects the formation of the interaction region and how long it will last.</p><p>To that end, we execute a 1D OSIRIS <ref type="bibr">[46]</ref><ref type="bibr">[47]</ref><ref type="bibr">[48]</ref> PIC simulation (which can capture counter-streaming and kinetic effects). These 1D simulations will result in a longer counterstreaming time than a 3D case, thus giving an upper bound on the counter-streaming phase. The OSIRIS simulation was initialized at the time when the two jets began to merge. Two counter-streaming plasma jets, extending 12.4 mm, were initialized with spatially-varying density and velocity profiles in the 28 mm simulation domain. This setup ensured that the particle and electromagnetic-field boundaries were transparent for the physical region of interest (the central 2 mm, or -1 mm &lt; z &lt; 1 mm, region). By fine-tuning the density and velocity spatial profiles in the OSIRIS simulation, the timevarying density and velocity profiles of the inflowing plasma jets at z = &#177;1 mm were matched to those in the FLASH simulation. Within the 10 ns simulation time, the inflowing jet velocity decreases from 6 &#215; 10 7 cm s -1 to 6 &#215; 10 6 cm s -1 ; the jet density increases from 3 &#215; 10 18 cm -3 to 6 &#215; 10 18 cm -3 . The grid size of the OSIRIS simulation was set to 3.9 &#215; 10 -5 mm, resolving the Debye length for the initial temperature. The numbers of particle-per-cell (PPC) for the three species, namely electron, carbon, and hydrogen, were 28, 24, and 4, respectively. The choice of PPC numbers ensures the same numerical weight of the charge for all particles, and thus conserves energy and momentum for every binary collision event that is modeled by the collision package <ref type="bibr">49</ref> in OSIRIS. In Fig. <ref type="figure">3</ref> we show a composite image of the jet properties from the OSIRIS PIC simulation. The interpenetration is captured in Fig. <ref type="figure">3a</ref>, evidenced by the net positive velocity of all particles that constitute the left jet. However, at 4 ns post-collision (Fig. <ref type="figure">4b</ref>), the interaction region has stagnated at the center of the domain. Comparing the density to the FLASH code (Fig. <ref type="figure">3c</ref>), shows similar interaction regions at 3 ns. Note that the particle interpenetration is confined to the 1.5-mm region in the PIC simulations, indicating that the particle are bound between the 2.0-mm region between the two targets.</p><p>To build confidence in the 3D FLASH results, which cannot capture the short-lived counter-streaming phase, we compare 1D FLASH simulations with 1D OSIRIS simulations to assess how discrepant the plasma properties are in the interaction region. The 1D FLASH run is initialized in an identical manner as is done in the OSIRIS simulations. In Fig. <ref type="figure">4</ref> we compare the temporal evolution of the average electron density over a 100-&#181;m region around the center of the computational domains. Initially the electron density is higher in the FLASH calculations, as the jet is immediately stopped and cannot counter-stream. However by 2 ns FLASH and OSIRIS predict similar densities. This result suggests that while the two codes compute different plasma conditions when the flows are counter-streaming, they quickly converge to similar values. Comparing the size of the interaction region shows a smaller interaction region at first in the FLASH results, as expected. At 3 ns the two simulations yield interaction regions of similar size as well.</p><p>TABLE I: Simulated plasma properties prior to collision and post collision Plasma Property Formula Prior to collision a Post collision b Electron Density &#961; (cm -3 ) ... 2.2 &#215; 10 19 5.0 &#215; 10 19 Ion Density n i (cm -3 ) ... 6.7 &#215; 10 18 1.4 &#215; 10 19 Electron Temperature T e (eV) ... 391 584 Ion Temperature T i (eV) ... 412 536 Average Ionization Z ... &#8764;3.5 &#8764;3.5 Average Atomic mass A &#8764;6.5 &#8764;6.5 Flow velocity u (cm s -1 ) c ... 4.1 &#215; 10 7 0.99 &#215; 10 7 Reynolds Length L (cm) d ... 0.1 0.008 RMS Magnetic field B (G) ... 3.8 &#215; 10 4 1.8 &#215; 10 5 Coulomb Logarithm log&#923; 23.5log(n 1/2 e T -5/4 e ) -10 -5 + (log(T e )-2) 2 16 8.35 7.2 Sound Speed C s (cm s -1 ) 9.80 &#215; 10 5 (ZT e +(5/3)T i ) 1/2 A 1/2 1.2 &#215; 10 7 1.3 &#215; 10 7 Mach Number M u/cs 3.41 0.76 Fluid Reynolds number Re uL/&#957;(&#957; = 1.92 &#215; 10 19 T 5/2 i A 1/2 Z 4 n i log&#923; ) 46,174 205 Magnetic Reynolds number Rm uL/&#951;(&#951; = 3.2 &#215; 10 5 Zlog&#923; T 3/2 e ) 2,544 36 Magnetic Prandtl number Pm Rm/Re 0.055 0.18 a Properties in the individual jets before collision b Properties in the interaction region 10 ns post collision c Prior to collision the flow velocity is the bulk flow, while post collision RMS velocity is used d Prior to collision half of the distance between targets is used, while after collision the ridge + well width is used</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>C. Phase III: Relaxation of the interaction region</head><p>At this stage, the density has increased in the center of the domain resulting in a developed interaction region whose properties are summarized in Table <ref type="table">I</ref>. The interaction region is subsonic and expands radially. Because the inflowing plasma jets retain the variations from the grooved pattern, their interaction results in shear and stochastic fluctuations in the interaction region. While the plasma jets continue to flow toward the interaction region, at 7 ns the laser power ramps down and turns off at 10 ns, leading to a reduction in the density, temperature, and velocity. As the simulation progresses, the plasma temperature in the center reduces from 100s to 10s of eV, while the electron density drops from 5&#215;10 19 cm -3 to 2&#215;10 19 cm -3 .</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>D. Magnetic field amplification</head><p>The laser-target interactions generate large temperature and density gradients, whose cross product gives rise to a Biermann-battery magnetic field. There is no initial or background magnetic field. The magnetic field is characterized by an RMS value of 165 kG and is flux-frozen into the plasma, as seen by the large magnetic Reynolds number (&gt;1,000) in Table <ref type="table">I</ref>. The magnetic field is advected toward the center of the domain and undergoes some flux compression, which increases its value to approximately 200 kG.</p><p>Flux compression is not the only mechanism that can increase the magnetic field strength. Given the counterstreaming, we need to also consider the Weibel instability <ref type="bibr">50</ref> . The Weibel instability is a two-stream instability present in nearly homogeneous plasmas with momentum anisotropy. This instability can spontaneously generate or amplify magnetic fields <ref type="bibr">44,</ref><ref type="bibr">51,</ref><ref type="bibr">52</ref> . Since the FLASH code does not include the Weibel instability, we must assess if Weibel fields are relevant during the formation of the interaction region. To that end we follow the work done by Ryutov et al <ref type="bibr">53,</ref><ref type="bibr">54</ref> . We solve the following dispersion relation to obtain the growth rate of the instability &#915;.</p><p>where</p><p>(see also eqn. 18 and 19 in Ryutov et al <ref type="bibr">53 )</ref>. A is the carbon-ion atomic number, m p is the proton mass, Z is the charge of the carbon ions, m e is the electron mass, c is the speed of light, u is the velocity of the jets, c s is the ion sound speed, and &#951; b and &#951; s are the bulk and shear viscosities. These parameters are then modified to account for the addition of hydrogen, following the treatment in Section 4 (in Ryutov et al <ref type="bibr">53</ref> ), yielding where &#945; is the number of heavy ions per hydrogen ions, A H and A Z are the atomic masses of hydrogen-ions and carbonions respectively, and &#969; pe is the electron plasma frequency. With these considerations, we calculate the e-folding time to properties in the interaction region. The electron density in (a) is averaged over a 100-&#181;m region in the center of the domain. While both simulations are initialized with identical jet parameters, the FLASH calculation initially predicts higher densities that the OSIRIS calculation. As more material accumulates in the center of the domain, the OSIRIS particles stop counter-streaming and accumulate, resulting in a similar value to the FLASH results. Similarly, the plot of the interaction regions width in (b) shows that the interaction width predicted by FLASH is initially smaller, but at &#8771;3 ns the widths match between FLASH and OSIRIS simulations.</p><p>be &#8764; 6.7 ns. Given the counter-streaming only occurs for 3 ns in the OSIRIS simulations, the Weibel instability cannot make meaningful contributions to the magnetic field. Therefore, the magnetic field in the interaction region primarily originates from the advected Biermann-battery magnetic field, and not other processes.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>E. Validation of plasma properties</head><p>We leverage the ongoing experimental campaign to validate the FLASH simulation with optical spectroscopy data. To provide electron density, electron temperature, and a RMS velocity, an optical spectroscopy diagnostic was employed, gathering data over a path integrated area with a 4.0 mm diameter, encompassing the two targets. From this large collection region, a feature in the emitted light, near 470 &#181;m, was fit using PrismSPECT <ref type="bibr">55</ref> , providing temperature, electron density, and RMS velocity measurements. This peak in the spectra was the only consistent feature across the experimental data and was therefore the one used for the fitting procedure. The error bars on the values were calculated using the 100 best data fits. The uncertainty of the timing of the optical spectroscopy and the fitting procedure only gives approximate values. We therefore present individual values for each plasma property from the experiment, which are representative of the conditions from 15 ns to 25 ns, shown in Table <ref type="table">II</ref> under the "Experiment" column. To directly compare experimental and simulation data, we average the FLASH results over a 1.28 mm &#215; 1.28 mm &#215; 3.84 mm region (the entire simulation domain), masking for the unablated target. These values are then averaged from 15 ns to 25 ns, which corresponds to the experimental temporal window when the optical spectroscopy measurement occurred.</p><p>The experimental plasma properties and values calculated in the FLASH simulation (under the "Large Volume" column) are shown in Table <ref type="table">II</ref>. The simulated electron density is within the error bars of the experiment, in good agreement with the spectroscopic data. The ion temperature is somewhat higher than the experiment, which is due to the lack of the initial counter-streaming in the FLASH simulations, resulting in higher temperature when the two jets collide. This is also why the RMS velocity is somewhat lower in the FLASH simulations, as more kinetic energy is converted into thermal energy than in the experiment.</p><p>The comparison of the FLASH calculations and the experimental results shows agreement over a large volume, but the values of interest for energization are those along the calciumion flight path. Employing the FLASH simulations allows us to obtain the plasma conditions and magnetic field of the calcium-ion flight path. Both are required to estimate the ion acceleration and both are different between the large volume and the flight path. Since the FLASH calculations include the magnetic field generation terms and, as shown in Section III, the Weibel instability is not expected to affect the magnetic field in the interaction region, we can utilize the properties in the flight path (Table <ref type="table">II</ref>) to estimate the energization of the calcium ions.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>IV. ION ACCELERATION</head><p>A. Plasma properties in the ion path.</p><p>The plasma properties through a 100-&#181;m diameter, 1,280&#181;m long cylinder were calculated, i.e., the calcium-ion flight path. This cylindrical region is in the center of the domain, parallel to the two targets, and the results of averaging over this volume are shown in Fig. <ref type="figure">5</ref> (dashed line). As expected, the ions travel through higher densities and temperatures than those measured in the large volume (solid line) region. Conversely, the RMS velocity is lower in the calcium-ion flight path because it does not include the inflowing material. The reduced RMS velocities and increased electron temperature and electron density highlight the need for the FLASH simulations, which show that there is a substantial difference between the large volume and the calcium-ion flight path and will allow a more accurate estimation of particle energization. We calculate the magnetic field in the calcium-ion flight path, finding that it peaks at the 10-ns mark, with a value of 200 kG, dropping to approximately 80 kG by the 15-ns mark, and re-</p><p>TABLE II: Simulated plasma properties in the calcium-ion flight path, large volume, and experimental data. The calcium-ion flight path data are used to estimate the energization. Plasma Property Calcium-Ion Flight Path Large Volume Experiment Electron Density &#961; (cm -3 ) 2.2&#215; 10 19 2.1&#215; 10 19 1.9 &#177; 0.2 &#215; 10 19 Ion Temperature T i (eV) 96 55 42.1 &#177; 3.1 Velocity u rms (cm s -1 ) 7.0 &#215; 10 6 8.1 &#215; 10 6 18.1 &#177; 2.9 &#215; 10 6 Magnetic field B (G) 6.0 &#215; 10 4 3.5 &#215; 10 4 ... Ion path length L (cm) 0.3 0.3 ... Correlation length &#8467; b (cm) 0.013 ... ... Electron plasma frequency (s -1 ) 2.6 &#215; 10 14 2.5 &#215; 10 14 2.5 &#215; 10 14 Electron gyrofrequency (s -1 ) 1.1 &#215; 10 12 8.8 &#215; 10 11 ... Ion plasma frequency (s -1 ) 4.5 &#215; 10 12 4.4 &#215; 10 12 4.2 &#215; 10 12</p><p>duces approximately 50 kG by the 30-ns mark. The calculated plasma properties in the calcium-ion flight path are shown in Table <ref type="table">II</ref>.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>B. Acceleration estimates</head><p>The ion beam is not simulated in this work. The reason is two-fold, FLASH cannot accurately capture the plasma and ion-beam interaction and the computational cost associated with running this form of simulation in OSIRIS is prohibitive. Instead scaling laws are used to estimate the particle energization.</p><p>From the late-time plasma conditions that FLASH predicts in the calcium-ion path, we estimate the expected acceleration from first-order and second-order Fermi mechanism, as well as the lower-hybrid drift instability. The time frame of interest is 15-25 ns, i.e., after the interaction region has relaxed to the plasma conditions also seen in the experiment. These times were chosen as this corresponds to when the ion bunches were launched through the domain in the experiment and is also when the FLASH results match the experiment. To mirror the experimental results, we average the plasma parameters from 15 ns to 25 ns in the calcium-ion flight path and display them in Table <ref type="table">II</ref> under the "Calcium-Ion Flight Path" column.</p><p>The first-order Fermi mechanism relies on shocks. Since the interaction region is subsonic and the reverse shocks are outside the calcium-ion path, this mechanism is not expected to contribute to ion acceleration. However, second-order Fermi and lower-hybrid drift can contribute, so we examine each separately.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head n="1.">Second-order Fermi acceleration</head><p>Second-order Fermi acceleration relies on interactions of particles with magnetic mirrors. In our experiment, this translates to a diffusive acceleration of the calcium ions through magnetic fluctuations (see Fig. <ref type="figure">2g-i</ref>). To calculate the energy diffusion we follow a similar calculation to Chen et al. <ref type="bibr">21,</ref><ref type="bibr">31,</ref><ref type="bibr">56,</ref><ref type="bibr">57</ref> The energy change from a single deflection by the magnetic field is</p><p>where Z c e is the calcium-ion charge, &#8467; b is the correlation length of the magnetic field <ref type="bibr">30</ref> , c is the speed of light, and u rms and B rms are the RMS velocity and magnetic field, respectively. As the charged calcium ions traverse the interaction region, they undergo a number of such deflections which results in a diffusion. The resulting change in energy is</p><p>where N 0 is the number of deflections. This can be approximated as N 0 &#8764; L/&#8467; b , where L is the distance the calcium ions travel through. The collisional mean free path of the calcium ions is l m f p &#8776; 1.7&#215;10</p><p>4 cm, showing that collisions are not the dominant interactions these particles experience. With this estimate, we find &#8710;E &#8764; 9.7 Z c 18 u rms 7.0 &#215; 10 6 cm s -1 B rms 60 kG L&#8467; b 0.0052 cm 2 0.5 keV.</p><p>Using the plasma conditions and magnetic field obtained from the FLASH simulations, we estimate the energization the calcium ions would experience to be &#8710;E &#8764; 9.7 keV. Comparing this value to the 0.1% (or 240 keV) energy spread in the generated ions shows this mechanism will not result in an observable change to the energy spectrum.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head n="2.">Lower-hybrid drift instability</head><p>The lower-hybrid drift instability is a kinetic instability that generates kinetic waves in a magnetized plasma when there exist gradients of density and magnetic field <ref type="bibr">22,</ref><ref type="bibr">58</ref> . These lower-hybrid waves induce an electric field that can accelerate particles. It develops with a growth rate of</p><p>where v d is the drift velocity, v i is the ion velocity, and &#969; LH is the lower hybrid frequency. The change in velocity of nonresonant charged particles through a weakly turbulent medium susceptible to this instability can be modeled as a diffusion problem, with the following coefficient <ref type="bibr">25,</ref><ref type="bibr">59,</ref><ref type="bibr">60</ref> </p><p>Z c and A c are the charge and atomic number of the beam ions, &#969; pi is the ion plasma frequency, &#8710;&#969; is the bandwidth of the lower-hybrid turbulence (1 percent of the lower-hybrid frequency was used), W is the wave energy density, nT is the plasma pressure, and c s is the sound speed. The ratio of electrostatic wave energy density to thermal energy at saturation becomes 58</p><p>where &#969; pe is the electron plasma frequency and &#969; ce is the electron gyrofrequency. Using the relation <ref type="bibr">25</ref> that D &#8869; = |&#8710;v| 2 /&#964;, the change in velocity becomes</p><p>A c 48 a.m.u</p><p>-1 &#969; pi 4.5 &#215; 10 12 s -1 &#8710;&#969; 4.4 &#215; 10 10 s -1 -0.5 W nT 8.0 &#215; 10 -7 0.5 c s 9.0 &#215; 10 6 cm s -1 L 0.4 cm 0.5 v i 3.1 &#215; 10 9 cm s -1 -0.5 cm s -1 (13)</p><p>where L is the length that the calcium ions traverse and v i is the calcium ion velocity. Using the parameters from Table II yields energizations of &#8710;E of 264 keV. This corresponds to a &#8764; 0.11% change in energy, which is larger than the calcium ion thermal spread and can be resolved by the available timeof-flight diagnostics.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>V. SUMMARY</head><p>In this paper we have shown results of FLASH simulations of a laser-driven experimental campaign at the GSI Helmholtz Institute for Heavy Ion research, which aims to observe ion acceleration in stochastic magnetic fields. The laser ablation of two targets generates weakly magnetized supersonic jets which form an interaction region at the center of the chamber. The magnetic field originates from the propagation of the Biermann-battery generated magnetic field from the lasertarget interaction. While the Weibel instability may appear in the interaction region during the counter-streaming phase, we found that its growth rate is too small to have an appreciable effect on the magnetic field.</p><p>We validated the simulation results with optical spectroscopy from the experiments and then used the validated FLASH simulations to infer the plasma properties on the calcium-ion flight path. Using the plasma properties calculated using FLASH, we estimated the energization due to second-order Fermi acceleration and lower-hybrid drift instability that would be expected in this experiment. While second-order Fermi acceleration might be acting on the ions, the effect will not be observable. Conversely, the electric field from the lower-hybrid drift instability was found to have a more appreciable effect on the ion energy. The latter is expected to result in energy gains of &#8710;E &#8764; 264 keV, which can be resolved by the time-of-flight diagnostics at the GSI.</p></div>
<div xmlns="http://www.tei-c.org/ns/1.0"><head>VI. ACKNOWLEDGMENTS</head><p>The results presented here are based on the experiment P-22-00089, which was performed at the target station Z6 at the GSI Helmholtzzentrum f&#252;r Schwerionenforschung, Darmstadt (Germany) in the frame of FAIR Phase-0. The TDYNO team would like to thank the operators and technicians of GSI, specifically those who assisted on the UNILAC accelerator, the Z6 experimental hall, and the PHELIX and </p></div></body>
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