This work presents numerical modeling-based investigations for detecting and monitoring damage growth and material nonlinearity in plate structures using topological acoustic (TA) and sideband peak count (SPC)-based sensing techniques. The nonlinear ultrasonic SPC-based technique (SPC-index or SPC-I) has shown its effectiveness in monitoring damage growth affecting various engineering materials. However, the new acoustic parameter, “geometric phase change (GPC)” and GPC-index (or GPC-I), derived from the TA sensing technique adopted for monitoring damage growth or material nonlinearity has not been reported yet. The damage growth modeling is carried out by the peri-ultrasound technique to simulate nonlinear interactions between elastic waves and damages (cracks). For damage growth with a purely linear response and for the nonlinearity arising from only the nonlinear stress–strain relationship of the material, the numerical analysis is conducted by the finite element method (FEM) in the Abaqus/CAE 2021 software. In both numerical modeling scenarios, the SPC- and GPC-based techniques are adopted to capture and compare those responses. The computed results show that, from a purely linear scattering response in FEM modeling, the GPC-I can effectively detect the existence of damage but cannot monitor damage growth since the linear scattering differences are small when crack thickness increases. The SPC-I does not show any change when a nonlinear response is not generated. However, the nonlinear response from the damage growth can be efficiently modeled by the nonlocal peri-ultrasound technique. Both the GPC-I and SPC-I techniques can clearly show the damage evolution process if the frequencies are properly chosen. This investigation also shows that the GPC-I indicator has the capability to distinguish nonlinear materials from linear materials while the SPC-I is found to be more effective in distinguishing between different types of nonlinear materials. This work can reveal the mechanism of GPC-I for capturing linear and nonlinear responses, and thus can provide guidance in structural health monitoring (SHM).
more »
« less
This content will become publicly available on July 1, 2026
Resonant Soft X-Ray Scattering in Polymer Materials
Resonant soft X-ray scattering (RSoXS) is a powerful tool for chemically and orientationally resolved nano-to-mesoscale characterization of complex molecular materials. Through its development over the past 15 years, its use has been extended to uniquely characterize structures, not only dry, thin films for devices, coatings, photolithography, and liquid crystalline ordering, but also solvated nanostructures in biology for therapeutics and hydrated membranes for filtration or biosensing. Here, we review progress in this exciting and maturing technique with an eye toward the materials scientist or engineer who has little experience with RSoXS but would like to know more about how the technique would fit into their toolset.
more »
« less
- Award ID(s):
- 2247711
- PAR ID:
- 10638365
- Publisher / Repository:
- Annual Reviews
- Date Published:
- Journal Name:
- Annual Review of Materials Research
- Volume:
- 55
- Issue:
- 1
- ISSN:
- 1531-7331
- Page Range / eLocation ID:
- 1 to 35
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Charge order has been a central focus in the study of cuprate high-temperature superconductors due to its intriguing yet not fully understood connection to superconductivity. Recent advances in resonant inelastic x-ray scattering (RIXS) in the soft x-ray regime have enabled the first momentum-resolved studies ofdynamiccharge order correlations in the cuprates. This progress has opened a window for a more nuanced investigation into the mechanisms behind the formation of charge order (CO) correlations. This review provides an overview of RIXS-based measurements of dynamic CO correlations in various cuprate materials. It specifically focuses on electron-doped cuprates and Bi-based hole-doped cuprates, where the CO-related RIXS signals may reveal signatures of the effective Coulomb interactions. This aims to explore a connection between two central phenomena in the cuprates: strong Coulomb correlations and CO-forming tendencies. Finally, we discuss current open questions and potential directions for future RIXS studies as the technique continues to improve and mature, along with other probes of dynamic correlations that would provide a more comprehensive picture.more » « less
-
Abstract Physically soft magnetic materials (PSMMs) represent an emerging class of materials that can change shape or rheology in response to an external magnetic field. However, until now, no studies have investigated using an electropermanent magnet (EPM) and magnetic repulsion to magnetically deform PSMMs. Such capabilities would enable the ability to deform PSMMs without the need for continuous electrical input and produce PSMM film deformation without an air gap, as would be required with magnetic attraction. To address this, we introduce a PSMM-EPM architecture in which the shape of a soft deformable thin film is controlled by switching between bistable on/off states of the EPM circuit. We characterized the deflection of a PSMM thin film when placed at controlled distances normal to the surface of the EPM and compared its response for cases when the EPM is in the ‘on’ and ‘off’ states. This work is the first to demonstrate a magnetically repelled soft deformable thin film that achieves two electronically-controlled modes of deformation through the on and off states of an EPM. This work has the potential to advance the development of new magneto-responsive soft materials and systems.more » « less
-
As a real-space technique, atomic-resolution STEM imaging contains both amplitude and geometric phase information about structural order in materials, with the latter encoding important information about local variations and heterogeneities present in crystalline lattices. Such phase information can be extracted using geometric phase analysis (GPA), a method which has generally focused on spatially mapping elastic strain. Here we demonstrate an alternative phase demodulation technique and its application to reveal complex structural phenomena in correlated quantum materials. As with other methods of image phase analysis, the phase lock-in approach can be implemented to extract detailed information about structural order and disorder, including dislocations and compound defects in crystals. Extending the application of this phase analysis to Fourier components that encode periodic modulations of the crystalline lattice, such as superlattice or secondary frequency peaks, we extract the behavior of multiple distinct order parameters within the same image, yielding insights into not only the crystalline heterogeneity but also subtle emergent order parameters such as antipolar displacements. When applied to atomic-resolution images spanning large (~0.5 × 0.5 μ m 2 ) fields of view, this approach enables vivid visualizations of the spatial interplay between various structural orders in novel materials.more » « less
-
Abstract Three-dimensional (3D) bioprinting is a promising technique for spatially patterning cells and materials into constructs that mimic native tissues and organs. However, a trade-off exists between printability and biological function, where weak materials are typically more suited for 3D cell culture but exhibit poor shape fidelity when printed in air. Recently, a new class of assistive materials has emerged to overcome this limitation and enable fabrication of more complex, biologically relevant geometries, even when using soft materials as bioinks. These materials include support baths, which bioinks are printed into, and sacrificial inks, which are printed themselves and then later removed. Support baths are commonly yield-stress materials that provide physical confinement during the printing process to improve resolution and shape fidelity. Sacrificial inks have primarily been used to create void spaces and pattern perfusable networks, but they can also be combined directly with the bioink to change its mechanical properties for improved printability or increased porosity. Here, we outline the advantages of using such assistive materials in 3D bioprinting, define their material property requirements, and offer case study examples of how these materials are used in practice. Finally, we discuss the remaining challenges and future opportunities in the development of assistive materials that will propel the bioprinting field forward toward creating full-scale, biomimetic tissues and organs.more » « less
An official website of the United States government
