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Abstract The rise of quantum science and technologies motivates photonics research to seek new platforms with strong light-matter interactions to facilitate quantum behaviors at moderate light intensities. Topological polaritons (TPs) offer an ideal platform in this context, with unique properties stemming from resilient topological states of light strongly coupled with matter. Here we explore polaritonic metasurfaces based on 2D transition metal dichalcogenides (TMDs) as a promising platform for topological polaritonics. We show that the strong coupling between topological photonic modes of the metasurface and excitons in TMDs yields a topological polaritonic Z2phase. We experimentally confirm the emergence of one-way spin-polarized edge TPs in metasurfaces integrating MoSe2and WSe2. Combined with the valley polarization in TMD monolayers, the proposed system enables an approach to engage the photonic angular momentum and valley and spin of excitons, offering a promising platform for photonic/solid-state interfaces for valleytronics and spintronics.
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This content will become publicly available on September 2, 2026
Topological Polaritonic Metamaterials Realized in Bulk Transition Metal Dichalcogenide Crystals
Due to the enhanced nature of the interactions of light with quantum excitations, topological polaritonic (TP) systems form a unique platform that offers on‐chip control over half‐light, half‐matter excitations via synthetic degrees of freedom. Among other polaritonic platforms, van der Waals materials (vdW) have recently attracted significant interest due to the relative simplicity of their integration into topological photonic structures. Several TP insulators based on vdW materials have been demonstrated; however, they rely on hybrid structures with nanopatterned dielectric substrates, which limit the strength of light‐matter interactions. Here, a monolithic all‐vdW TP insulator based on bulk crystals of transition metal dichalcogenide WS2is designed and experimentally realized. Due to their high refractive index and the presence of exciton modes, these nanomaterials prove to be excellent platforms for TPs, offering both excellent confinement and strong light‐matter interactions in monolithic structures. The emergence of TP boundary modes is confirmed by Fourier and real‐space imaging, and a dramatic reduction in dissipation is observed at cryogenic temperatures. The proposed monolithic all‐vdW topological insulators, which are characterized by extreme confinement of optical fields and moderate losses, can serve as an alternative to silicon photonics‐based systems in the quest for the development of polaritonic quantum technologies.
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- Award ID(s):
- 2328993
- PAR ID:
- 10639278
- Publisher / Repository:
- Wiley
- Date Published:
- Journal Name:
- Small Structures
- ISSN:
- 2688-4062
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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