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Title: Magnetotransport properties of layered Fe 3 GeTe 2 crystals
Abstract Van der Waals layered magnetic materials have recently received significant attention for their ability to exhibit antiferromagnetic or ferromagnetic (FM) properties, even at the few-layer or monolayer scale. Among them, Fe3GeTe2is one of the most extensively studied systems, crystallizing in a hexagonal structure as an itinerant FM with a Curie temperature (TC) of ∼220 K in bulk form and strong magnetic anisotropy. In this study, temperature and magnetic field dependence of the four-probe resistance ( Rxx ), thermopower (TEP) (S), and Hall resistance ( Rxy ) were investigated in thick Fe3GeTe2flakes with different thicknesses to understand electron and spin transport, as well as spin and magnetic states. Rxx decreased with decreasing temperature, confirming metallic behavior, consistent with the observed reduction in the magnitude of the negative TEP. Negative magnetoresistance (MR) with the magnetic field normal to the sample plane exhibited a quadratic field dependence belowTC. An anomalous Hall effect was observed belowTC, where Rxy ( B ) showed a linear field dependence at low fields and saturation at higher fields. The anomalous Hall resistance ( RxyA ) followed a dependence of α Rxx +β Rxx2 . A positive in-plane MR was observed when the current was perpendicular to the magnetic field, attributed to increased scattering from the enhanced Lorentz force and related orbital effects. Additionally, a hysteresis behavior was observed when cycling the in-plane magnetic field, likely due to the delay in domain alignment in response to the changing field.  more » « less
Award ID(s):
2039380
PAR ID:
10702280
Author(s) / Creator(s):
; ; ; ; ; ; ; ;
Publisher / Repository:
IOP
Date Published:
Journal Name:
Journal of Physics: Materials
Volume:
9
Issue:
2
ISSN:
2515-7639
Page Range / eLocation ID:
025009
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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