Abstract Superconducting performance is tunable not only via chemical modification or defect engineering, but also through external parameters such as pressure, though this method remains less readily accessible. In this work, we study how compression influences vortex dynamics and critical currents in an iron-based superconductor. Specifically, we perform magnetization measurements using an off-the-shelf pressure cell to investigate the effects of hydrostatic pressures up to 1.08 GPa on the magnetic properties of BaFe (As P ) crystals across a range of temperatures and magnetic fields . Although these pressures minimally affect the superconducting critical temperature, they produce a clear increase in the critical current density , a pronounced reduction in the rate of thermally activated vortex motion , and can change the dominant vortex pinning mechanism. Furthermore, the effects of pressure are irreversible: after pressurization and subsequent release at room temperature, high-density microcracks are observed and the crystals retain their enhanced critical current densities. The second magnetization peak vanishes above 18 K after the pressure cycle, which we attribute to a transition from predominantly pinning to a mixed mechanism of and surface pinning. Lastly, a threefold increase in , a more than 40% reduction in at 8 K and 0.5 T, and an expanded elastic-creep region were achieved after pressure cycles. These findings demonstrate the potential utility of pressure cycling for improving , which may offer a simpler alternative compared to approaches such as chemical doping or the introduction of artificial pinning centers.
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This content will become publicly available on July 3, 2027
Lessons from α -RuCl 3 for pursuing quantum spin liquid physics in atomically thin materials
Abstract Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on the pursuit of phenomena related to Kitaev magnetism in layered and exfoliatable materials, which offer numerous opportunities to apply powerful techniques from the field of atomically thin materials. We primarily focus on the antiferromagnetic Mott insulator -RuCl , which exhibits Kitaev couplings and is readily exfoliated to single- or few-layer sheets, and thus serves as a test bed for developing probes of Kitaev phenomena in atomically thin materials and devices. We introduce the Kitaev model and how it is realized in -RuCl and other material candidates; and cover -RuCl synthesis and fabrication into van der Waals heterostructure devices. A key discovery is a work-function-mediated charge transfer that heavily dopes both the -RuCl and proximate materials, and can enhance Kitaev interactions by up to 50%. We further discuss a wide range of recent results in electronic transport and optical and tunneling spectroscopies of -RuCl devices. The experimental techniques and theoretical insights developed for -RuCl establish a framework for discovering and engineering superior two-dimensional Kitaev materials that may ultimately realize elusive quantum spin liquid phases.
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- Award ID(s):
- 2425133
- PAR ID:
- 10704003
- Author(s) / Creator(s):
- ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »
- Publisher / Repository:
- IOP Science
- Date Published:
- Journal Name:
- Journal of Physics: Condensed Matter
- Volume:
- 38
- Issue:
- 26
- ISSN:
- 0953-8984
- Page Range / eLocation ID:
- 263001
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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