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Impacts of aerosol particles on clouds, precipitation, and climate remain one of the significant uncertainties in climate change. Aerosol particles entrained at cloud top and edge can affect cloud microphysical and macrophysical properties, but the process is still poorly understood. Here we investigate the cloud microphysical responses to the entrainment of aerosol-laden air in the Pi convection-cloud chamber. Results show that cloud droplet number concentration increases and mean radius of droplets decreases, which leads to narrower droplet size distribution and smaller relative dispersion. These behaviors are generally consistent with the scenario expected from the first aerosol-cloud indirect effect for a constant liquid water content (L). However, L increases significantly in these experiments. Such enhancement of L can be understood as suppression of droplet sedimentation removal due to small droplets. Further, an increase in aerosol concentration from entrainment reduces the effective radius and ultimately increases cloud optical thickness and cloud albedo, making the clouds brighter. These findings are of relevance to the entrainment interface at stratocumulus cloud top, where modeling studies have suggested sedimentation plays a strong role in regulating L. Therefore, the results provide insights into the impacts of entrainment of aerosol-laden air on cloud, precipitation, and climate.
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This content will become publicly available on December 16, 2026
High-resolution lidar observations of sedimentation-induced size sorting of droplets near a laboratory cloud top
Cloud optical properties and precipitation, which are crucial to weather and climate, are strongly influenced by cloud microphysical properties that are still poorly understood. Here, we develop a high-resolution time-correlated single-photon-counting lidar and apply it to observe cloud microphysical properties at one-centimeter range resolution in a convection chamber under well-controlled conditions. Together with concurrent in-situ measurements and theoretical analysis, our lidar observations indicate that although turbulent mixing tends to homogenize the cloud in the bulk region, entrainment and sedimentation cause inhomogeneities in droplet concentrations near the cloud top. Specifically, the topmost region is directly affected by entrainment, and lidar profiles show clear evidence of entrained air and detrained cloud filament. The transition region below exhibits vertical size sorting of cloud droplets caused by sedimentation. Our results suggest that using a single sedimentation velocity for all cloud droplets, as is done in many atmospheric models, overlooks key physics relevant to the microphysical structure near the cloud top. Our conceptual model used to describe these measurements can serve as a step toward improving the current modeling of processes in the cloud top region.
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- Award ID(s):
- 2217182
- PAR ID:
- 10704931
- Publisher / Repository:
- PNAS
- Date Published:
- Journal Name:
- Proceedings of the National Academy of Sciences
- Volume:
- 122
- Issue:
- 50
- ISSN:
- 0027-8424
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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