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The Green River Formation preserves an extraordinary archive of terrestrial paleoclimate during the Early Eocene Climate Optimum (EECO; ~53-50 Ma), expressing multiple scales of sedimentary cyclicity previously interpreted to reflect annual to Milankovitch-scale forcing. Here we utilize X-ray fluorescence (XRF) core scanning and micro X-ray fluorescence (micro-XRF) scanning in combination with radioisotopic age data to evaluate a rock core record of laminated oil shale and carbonate mudstone from Utah’s Uinta Basin, with the parallel objectives of elucidating the paleo-environmental significance of the sedimentary rhythms, testing a range of forcing hypotheses, and evaluating potential linkages between high- and low-frequency forcing. This new assessment reveals that the ~100 μm-scale laminae – the most fundamental rhythm of the Green River Formation –are most strongly expressed by variations in iron and sulfur abundance. We propose that these variations reflect changes in redox state, consistent with annual stratification of the lake. In contrast to previous studies, no support was found for ENSO or sunspot cycles. However, millimeter to centimeter-scale rhythms—temporally constrained to the decadal to centennial scale—are strongly expressed as alternations in the abundance of silicate- versus carbonate-associated elements (e.g., Al and Si vs. Ca), suggesting changes in precipitation and sediment delivery to the paleo-lake.more »