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  1. Motivated by the recent developments in moiré superlattices of van der Waals magnets and the desire to control the magnetic interactions of α-RuCl3, here we present a comprehensive theory of the long-range ordered magnetic phases of twisted bilayer α-RuCl3. Using a combination of first-principles calculations and atomistic simulations, we show that the stacking-dependent interlayer exchange gives rise to an array of magnetic phases that can be realized by controlling the twist angle. In particular, we discover a complex hexagonal domain structure in which multiple zigzag orders coexist. This multidomain order minimizes the interlayer energy while enduring the energy cost due to domain wall formation. Further, we show that quantum fluctuations can be enhanced across the phase transitions. Our results indicate that magnetic frustration due to stacking-dependent interlayer exchange in moiré superlattices can be exploited to tune quantum fluctuations and the magnetic ground state of α-RuCl3. 
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    Free, publicly-accessible full text available January 10, 2025
  2. We study the phase diagram of the Yao-Lee model with Kitaev-type spin-orbital interactions in the presence of Dzyaloshinskii-Moriya interactions and external magnetic fields. Unlike the Kitaev model, the Yao-Lee model can still be solved exactly under these perturbations due to the enlarged local Hilbert space. Through a variational analysis, we obtain a rich ground-state phase diagram that consists of a variety of vison crystals with periodic arrangements of background Z2 flux (i.e., visons). With an out-of-plane magnetic field, these phases have gapped bulk and chiral edge states, characterized by a Chern number ν and an associated chiral central charge c=ν/2 of edge states. We also find helical Majorana edge states that are protected by magnetic mirror symmetry. For the bilayer systems, we find that interlayer coupling can also stabilize new topological phases. Our results spotlight the tunability and the accompanying rich physics in exactly solvable spin-orbital generalizations of the Kitaev model. 
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  3. Abstract

    We determine the phase diagram of a bilayer, Yao-Lee spin-orbital model with inter-layer interactions (J), for several stackings and moiré superlattices. For AA stacking, a gapped$${{\mathbb{Z}}}_{2}$$Z2quantum spin liquid phase emerges at a finiteJc. We show that this phase survives in the well-controlled large-Jlimit, where an isotropic honeycomb toric code emerges. For moiré superlattices, a finite-qinter-layer hybridization is stabilized. This connects inequivalent Dirac points, effectively ‘untwisting’ the system. Our study thus provides insight into the spin-liquid phases of bilayer spin-orbital Kitaev materials.

     
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  5. Abstract

    Bio-inspired Topographically Mediated Surfaces (TMSs) based on high aspect ratio nanostructures have recently been attracting significant attention due to their pronounced antimicrobial properties by mechanically disrupting cellular processes. However, scalability of such surfaces is often greatly limited, as most of them rely on micro/nanoscale fabrication techniques. In this report, a cost-effective, scalable, and versatile approach of utilizing diamond nanotechnology for producing TMSs, and using them for limiting the spread of emerging infectious diseases, is introduced. Specifically, diamond-based nanostructured coatings are synthesized in a single-step fabrication process with a densely packed, needle- or spike-like morphology. The antimicrobial proprieties of the diamond nanospike surface are qualitatively and quantitatively analyzed and compared to other surfaces including copper, silicon, and even other diamond surfaces without the nanostructuring. This surface is found to have superior biocidal activity, which is confirmed via scanning electron microscopy images showing definite and widespread destruction ofE. colicells on the diamond nanospike surface. Consistent antimicrobial behavior is also observed on a sample prepared seven years prior to testing date.

    Graphical Abstract

     
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  7. Abstract

    The physics potential of detecting8B solar neutrinos will be exploited at the Jiangmen Underground Neutrino Observatory (JUNO), in a model-independent manner by using three distinct channels of the charged current (CC), neutral current (NC), and elastic scattering (ES) interactions. Due to the largest-ever mass of13C nuclei in the liquid scintillator detectors and the expected low background level,8B solar neutrinos are observable in the CC and NC interactions on13C for the first time. By virtue of optimized event selections and muon veto strategies, backgrounds from the accidental coincidence, muon-induced isotopes, and external backgrounds can be greatly suppressed. Excellent signal-to-background ratios can be achieved in the CC, NC, and ES channels to guarantee the observation of the8B solar neutrinos. From the sensitivity studies performed in this work, we show that JUNO, with 10 yr of data, can reach the 1σprecision levels of 5%, 8%, and 20% for the8B neutrino flux,sin2θ12, andΔm212, respectively. Probing the details of both solar physics and neutrino physics would be unique and helpful. In addition, when combined with the Sudbury Neutrino Observatory measurement, the world's best precision of 3% is expected for the measurement of the8B neutrino flux.

     
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    Free, publicly-accessible full text available April 1, 2025