skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Search for: All records

Creators/Authors contains: "Aroeira, Gustavo_J R"

Note: When clicking on a Digital Object Identifier (DOI) number, you will be taken to an external site maintained by the publisher. Some full text articles may not yet be available without a charge during the embargo (administrative interval).
What is a DOI Number?

Some links on this page may take you to non-federal websites. Their policies may differ from this site.

  1. Molecular exciton-polaritons exhibit long-range, ultrafast propagation, yet recent experiments have reported far slower propagation than expected. In this work, we implement a nonperturbative approach to quantify how static energetic disorder renormalizes polariton group velocity in strongly coupled microcavities. The method requires no exact diagonalization or master equation propagation and depends only on measurable parameters: the mean exciton energy and its probability distribution, the microcavity dispersion, and the Rabi splitting. Using parameters corresponding to recently probed organic microcavities, we show that exciton inhomogeneous broadening slows both lower and upper polaritons, particularly when the mean exciton energy fluctuation approaches the collective light–matter coupling strength. A detailed discussion and interpretation of these results is provided using perturbation theory in the limit of weak resonance scattering. The magnitude of the effects examined in this work supports the conclusion that most of the reported polaritonic slowdown arises from dynamical (phonon-assisted) disorder, with static energetic disorder contributing only secondarily. 
    more » « less
    Free, publicly-accessible full text available September 28, 2026