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Piezoelectric energy harvesting from ambient vibrations is well studied, but harvesting from quasi-static responses is not yet fully explored. The lack of attention is because quasi-static actions are much slower than the resonance frequency of piezoelectric oscillators to achieve optimal outputs; however, they can be a common mechanical energy resource: from large civil structure deformations to biomechanical motions. The recent advances in bio-micro-electro-mechanical systems and wireless sensor technologies are motivating the study of piezoelectric energy harvesting from quasi-static conditions for low-power budget devices. This article presents a new approach of using quasi-static deformations to generate electrical power through an axially compressed bilaterally constrained strip with an attached piezoelectric layer. A theoretical model was developed to predict the strain distribution of the strip’s buckled configuration for calculating the electrical energy generation. Results from an experimental investigation and finite element simulations are in good agreement with the theoretical study. Test results from a prototyped device showed that a peak output power of 1.33 μW/cm²was generated, which can adequately provide power supply for low-power budget devices. And a parametric study was also conducted to provide design guidance on selecting the dimensions of a device based on the external embedding structure.