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High-frequency mechanical oscillators with long coherence times are essential for realizing a variety of high-fidelity quantum sensors, transducers and memories. However, the coherence times needed for quantum applications require advances in probing and mitigating the origins of phonon decoherence in the materials used for mechanical oscillators. Here we identify key sources of phonon decoherence in crystalline media by combining non-invasive laser spectroscopy with materials analysis. Using micro-fabricated high-overtone bulk acoustic-wave resonators as an experimental test bed, we find that phonon–surface interactions are the dominant source of phonon decoherence in crystalline quartz. The probable causes are lattice distortion, subsurface damage and a high concentration of elemental impurities. We use an optimized polishing process to remove the compromised surface layer and produce resonators with quality factors exceeding 240 million at 12 GHz, corresponding to phonon coherence times of over 6 ms. We verify that these mechanical oscillators have negligible dephasing. Building on these results, we propose a path that could reach coherence times beyond 100 ms as the basis for high-frequency quantum memories. These findings demonstrate that enhanced control over surfaces enables a substantial reduction in dissipation and noise. 

Recognized as a potential resource for quantum technologies and a possible test bed for fundamental physics, the control and preparation of nonclassical states of mechanical oscillators have been explored extensively. Within optomechanics, quantum state synthesis can be realized by entangling photonic and phononic degrees of freedom followed by optical detection. Single-photon detection enables one of the most powerful forms of such heralded quantum state preparation, permitting the creation of single-phonon states when applied to conventional cavity optomechanical systems. As the complexity of optomechanical systems increases, single-photon detection may provide heralded access to a larger class of exotic quantum states. Here, we examine the quantum dynamics of optomechanical systems that permit forward Brillouin scattering, where a single-phonon mode mediates transitions between a collection of equally spaced optical resonances. Solving both the Schrodinger equation and the Lindblad master equation for this system, we find that initial states comprised of single photons or weak laser pulses evolve into complex quantum states where the frequency of single-photon states and the phonon occupation number are entangled. Physically, these interactions permit a single photon to scatter to lower frequencies, where phonon excitation occurs for each scattering event. Combining this result with frequency filtering, we show how single-photon detection can herald selected multiphonon Fock states, even in the presence of optical losses. We also present an approach for quantum tomography of the heralded phonon states, which in the form of a state swap from the phononic to photonic domain enables on-demand generation of multiphoton Fock states. 

The integration of stabilized lasers, sources that generate spectrally pure light, will provide compact, low-cost solutions for applications including quantum information sciences, precision navigation and timing, metrology, and high-capacity fiber communications. We report a significant advancement in this field, demonstrating stabilization of an integrated waveguide Brillouin laser to an integrated waveguide reference cavity, where both resonators are fabricated using the same CMOS-compatible integration platform. We demonstrate reduction of the free running Brillouin laser linewidth to a 292 Hz integral linewidth and carrier stabilization to a 4.9 × 10 −13 fractional frequency at 8 ms reaching the cavity-intrinsic thermorefractive noise limit for frequencies down to 80 Hz. We achieve this level of performance using a pair of 56.4 × 10 6 quality factor Si 3 N 4 waveguide ring-resonators that reduce the high-frequency noise by the nonlinear Brillouin process and the low-frequency noise by Pound–Drever–Hall locking to the ultra-low loss resonator. These results represent an important step toward integrated stabilized lasers with reduced sensitivity to environmental disturbances for atomic, molecular, and optical physics (AMO), quantum information processing and sensing, and other precision scientific, sensing, and communications applications. 

Abstract Narrow linewidth visible light lasers are critical for atomic, molecular and optical (AMO) physics including atomic clocks, quantum computing, atomic and molecular spectroscopy, and sensing. Stimulated Brillouin scattering (SBS) is a promising approach to realize highly coherent on-chip visible light laser emission. Here we report demonstration of a visible light photonic integrated Brillouin laser, with emission at 674 nm, a 14.7 mW optical threshold, corresponding to a threshold density of 4.92 mW μm −2 , and a 269 Hz linewidth. Significant advances in visible light silicon nitride/silica all-waveguide resonators are achieved to overcome barriers to SBS in the visible, including 1 dB/meter waveguide losses, 55.4 million quality factor (Q), and measurement of the 25.110 GHz Stokes frequency shift and 290 MHz gain bandwidth. This advancement in integrated ultra-narrow linewidth visible wavelength SBS lasers opens the door to compact quantum and atomic systems and implementation of increasingly complex AMO based physics and experiments.