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Precambrian terrains preserving rocks older than 3.5 Ga contain an essential record of the crustal evolution of the primitive Earth. In this study, we investigated Eo-Paleoarchean rocks from the northern S˜ao Francisco Craton (NSFC) and the Borborema Province in northeastern Brazil to contribute to a more complete global isotopic record of this pivotal time in Earth’s history. Zircon U-Pb ages along with zircon Hf isotope compositions were obtained for migmatitic gneiss complexes in both terrains. Zircon U-Pb data from the NSFC yield well-defined populations with 207Pb/206Pb ages from 3.61 to 3.59 Ga and younger components at ~3.5 and ~3.4 Ga. Similarly, the Borborema Province gneiss yields a main zircon age population of 3.58 Ga and a younger ~3.5 Ga age component. The ~3.6 Ga zircon components yield consistently sub-chondritic Hf isotopic compositions with initial εHf between −1.9 and −3.1 for the NSFC and of εHf −0.5 for the Borborema Province. Gneisses from northeastern Brazil record a main crust forming period at 3.65–3.60 Ga with sub-chondritic Hf isotope compositions that indicate derivation from melting of a ~3.8 Ga source of broadly chondritic isotope composition, similar to that of many Eo-Paleoarchean gneisses worldwide. This Hf isotope record supports the existence of broadly chondritic mantle reservoir in the Eoarchean with development of depleted mantle and the appearance of evolved crust later in the Paleoarchean.