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Free, publicly-accessible full text available July 1, 2022
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Small molecule guests influence the functional properties of supramolecular hydrogels. Molecular-level understanding of such sol-gel compositions and structures is challenging due to the lack of long-range order and inherently heterogeneous sol-gel interface. In this study, insight into the uptake process of biologically relevant small molecules into guanosine-quartet(G4) borate hydrogels is obtained by gel-state magic-angle spinning (MAS) NMR spectroscopy. G4∙K + borate hydrogel can absorb up to 0.3 equivalent of cationic methylene blue (MB) without a significant disruption of the G4 fibrils that make up the gel, whereas the addition of over 0.3 equivalents of MB to the same gel leadsmore »
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Abstract The selection of low-radioactive construction materials is of utmost importance for the success of low-energy rare event search experiments. Besides radioactive contaminants in the bulk, the emanation of radioactive radon atoms from material surfaces attains increasing relevance in the effort to further reduce the background of such experiments. In this work, we present the
Rn emanation measurements performed for the XENON1T dark matter experiment. Together with the bulk impurity screening campaign, the results enabled us to select the radio-purest construction materials, targeting a$$^{222}$$ Rn activity concentration of$$^{222}$$ in$$10\,\mathrm{\,}\upmu \mathrm{Bq}/\mathrm{kg}$$ of xenon. The knowledge of the distribution of the$$3.2\,\mathrm{t}$$ Rn sources allowed us to selectivelymore »$$^{222}$$ -
Abstract The DARWIN observatory is a proposed next-generation experiment to search for particle dark matter and for the neutrinoless double beta decay of $$^{136}$$ 136 Xe. Out of its 50 t total natural xenon inventory, 40 t will be the active target of a time projection chamber which thus contains about 3.6 t of $$^{136}$$ 136 Xe. Here, we show that its projected half-life sensitivity is $$2.4\times {10}^{27}\,{\hbox {year}}$$ 2.4 × 10 27 year , using a fiducial volume of 5 t of natural xenon and 10 year of operation with a background rate of less than 0.2 events/(t $$\cdot $$ · year) in the energymore »