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The dynamics of bimolecular photoinduced electron transfer from the doublet excited state of the anion radical ofN,N′-dioctylnaphthalene diimide (NDI) have been investigated. 

By exploiting symmetries of finite fields, covering perfect hash families provide a succinct representation for covering arrays of index one. For certain parameters, this connection has led to both the best current asymptotic existence results and the best known efficient construction algorithms for covering arrays. The connection generalizes in a straightforward manner to arrays in which every t-way interaction is covered λ > 1 times, i.e., to covering arrays of index more than one. Using this framework, we focus on easily computed, explicit upper bounds on numbers of rows for various parameters with higher index. 

Detecting arrays provide test suites for complex engineered systems in which many factors interact. The determination of which interactions have a significant impact on system behaviour requires not only that each interaction appear in a test, but also that its effect can be distinguished from those of other significant interactions. In this paper, compact representations of detecting arrays using vectors over the finite field are developed. Covering strong separating hash families exploit linear independence over the field, while the weaker elongated covering perfect hash families permit some linear dependence. For both, probabilistic analyses are employed to establish effective upper bounds on the number of tests needed in a detecting array for a wide variety of parameters. The analyses underlie efficient algorithms for the explicit construction of detecting arrays. 

Abstract We present new Atacama Large Millimeter/submillimeter Array observations that, for the first time, detect hydrogen and helium radio recombination lines from a protoplanetary disk. We imaged the Orion Nebula Cluster at 3.1 mm with a spectral setup that covered then= 42 → 41 transitions of hydrogen (H41α) and helium (He41α). The unprecedented sensitivity of these observations enables us to search for radio recombination lines toward the positions of ∼200 protoplanetary disks. We detect H41αfrom 17 disks, all of which are HST-identified “proplyds.” The detected H41αemission is spatially coincident with the locations of proplyd ionization fronts, indicating that proplyd H41αemission is produced by gas that has been photoevaporated off the disk and ionized by UV radiation from massive stars. We measure the fluxes and widths of the detected H41αlines and find line fluxes of ∼30–800 mJy km s⁻¹and line widths of ∼30–90 km s⁻¹. The derived line widths indicate that the broadening of proplyd H41αemission is dominated by outflowing gas motions associated with external photoevaporation. The derived line fluxes, when compared with measurements of 3.1 mm free–free flux, imply that the ionization fronts of H41α-detected proplyds have electron temperatures of ∼6000–11,000 K and electron densities of ∼10⁶–10⁷cm⁻³. Finally, we detect He41αtoward one H41α-detected source and find evidence that this system is helium-rich. Our study demonstrates that radio recombination lines are readily detectable in ionized photoevaporating disks, providing a new way to measure disk properties in clustered star-forming regions. 

We investigate whether Alfvénic fluctuations (AFs) can affect the structure of magnetic ejecta (ME) within interplanetary coronal mass ejections (ICMEs). We study an ICME observed on 2001 December 29 at 1 au by the Advanced Composition Explorer (ACE) and Wind, at a total angular separation of ~0.8 degree (~0.014 au). We focus on the correlation and complexity of its magnetic structure measured between two spacecraft in association with large-amplitude AFs. The Alfvénicity of the ME is investigated in terms of the residual energy and cross helicity of fluctuations. We find that as for the event of interest, large-amplitude AFs occur in the rear region of the ME at both Wind and ACE with a duration of about 6 hr. We compare the correlation of the magnetic field strength and vector components measured between Wind and ACE, and investigate complexity in terms of the magnetic hodograms. The region showing AFs is found to be associated with a decreased correlation of the magnetic field components and an increased complexity of the ME magnetic configuration detected at ACE and Wind, which may be due to the fact that the two spacecraft crossing the same ME along different trajectories likely sampled AFs in different oscillation phases. Combining multipoint in situ measurements and remote-sensing observations of the ICME source region, we further discuss different potential sources of the AFs. 

Abstract The aim of this study is to use multispacecraft measurements of interplanetary magnetic clouds (MCs) to better constrain and understand the effect of expansion on their magnetic field properties. We develop a parameter (γ) for comparing magnetic field components measured at multiple spacecraft. We use the minimum variance technique on the magnetic field data to obtain the axial and azimuthal components. The parameterγacts at the front boundary as a measure of the global difference in the evolution with heliospheric distance of the axial and azimuthal magnetic field components of MCs. Our goal is to determine whether the studied MCs exhibit self-similar expansion and, if so, whether this expansion is predominantly isotropic or radial, based on the estimatedγ. Through our analysis of data from multiple spacecraft, we observe a notable consistency in theγvalues across the examples examined. We find that the overall expansion of these MCs tends to be isotropic, while the local expansion of MCs, derived from theγvalues measured at the rear boundary of MCs, usually shows anisotropic behavior, particularly when the distances between the observations from the two spacecraft are relatively short. This discovery offers insights for refining flux rope models and advancing our comprehension of the expansion processes associated with coronal mass ejections.