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Creators/Authors contains: "Chen, Jia-Wei"

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  1. ; ; ; ; ; ; ( , Green Chemistry)
    Transformation of multifunctional materials with control over site-selectivity and chemical diversity remains challenging. Herein, we present a metal-free, one-pot strategy for the defluorophosphorylation of polyfluoroalkyl peroxides that enables expedient construction of structurally diverse phosphoryl-containing heterocyclic libraries. By judicious choice of reaction conditions, C 3,4-diphosphoryl furans and C 4-monophosphoryl furans can be easily accessed. In addition, synthetic derivatization of the obtained organophosphorus heteroarenes to value-added monodentate and bidentate phosphines has been demonstrated. Mechanistic studies revealed that regioselective defluorophosphorylation allows divergent product formation in two reaction modes. 
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    Free, publicly-accessible full text available March 6, 2024
  2. ; ; ; ; ; ; ; ; ; ; et al ( , ACS Applied Materials & Interfaces)
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