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null (Ed.)Single-crystal nanooptomechanical transduction occurs in [Ru(SO 2 )(NH 3 ) 4 (H 2 O)]chlorobenzenesulfonate 2 , reaching maximal levels within 40 s at 100 K when photostimulated by 505 nm light. Its in situ light-induced crystal structure reveals the molecular origins of this optical actuation: 26.0(3)% of the η 1 -SO 2 ligand photoconverts into an η 1 -OSO photoisomer which, in turn, induces a 49.6(9)° arene ring rotation in its neighbouring counter ion.more » « less