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  1. The effects of surfactants on a mechanically generated plunging breaker are studied experimentally in a laboratory wave tank. Waves are generated using a dispersively focused wave packet with a characteristic wavelength of$\lambda _0 = 1.18$m. Experiments are performed with two sets of surfactant solutions. In the first set, increasing amounts of the soluble surfactant Triton X-100 are mixed into the tank water, while in the second set filtered tap water is left undisturbed in the tank for wait times ranging from 15 min to 21 h. Increasing Triton X-100 concentrations and longer wait times lead to surfactant-induced changes in the dynamic properties of the free surface in the tank. It is found that low surface concentrations of surfactants can dramatically change the wave breaking process by changing the shape of the jet and breaking up the entrained air cavity at the time of jet impact. Direct numerical simulations (DNS) of plunging breakers with constant surface tension are used to show that there is significant compression of the free surface near the plunging jet tip and dilatation elsewhere. To explore the effect of this compression/dilatation, the surface tension isotherm is measured in all experimental cases. The effects of surfactants on the plunging jet are shown to be primarily controlled by the surface tension gradient ($\Delta \mathcal {E}$) while the ambient surface tension of the undisturbed wave tank ($\sigma _0$) plays a secondary role.

     
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  2. We present high-resolution three-dimensional (3-D) direct numerical simulations of breaking waves solving for the two-phase Navier–Stokes equations. We investigate the role of the Reynolds number ( Re , wave inertia relative to viscous effects) and Bond number ( Bo , wave scale over the capillary length) on the energy, bubble and droplet statistics of strong plunging breakers. We explore the asymptotic regimes at high Re and Bo , and compare with laboratory breaking waves. Energetically, the breaking wave transitions from laminar to 3-D turbulent flow on a time scale that depends on the turbulent Re up to a limiting value $Re_\lambda \sim 100$ , consistent with the mixing transition in other canonical turbulent flows. We characterize the role of capillary effects on the impacting jet and ingested main cavity shape and subsequent fragmentation process, and extend the buoyant-energetic scaling from Deike et al. ( J. Fluid Mech. , vol. 801, 2016, pp. 91–129) to account for the cavity shape and its scale separation from the Hinze scale, $r_H$ . We confirm two regimes in the bubble size distribution, $N(r/r_H)\propto (r/r_H)^{-10/3}$ for $r>r_H$ , and $\propto (r/r_H)^{-3/2}$ for $r more » « less
  3. Abstract

    Bubbles bursting at the ocean surface are an important source of ocean‐spray aerosol, with implications on radiative and cloud processes. Yet, very large uncertainties exist on the role of key physical controlling parameters, including wind speed, sea state and water temperature. We propose a mechanistic sea spray generation function that is based on the physics of bubble bursting. The number and mean droplet radius of jet and film drops is described by scaling laws derived from individual bubble bursting laboratory and numerical experiments, as a function of the bubble radius and the water physico‐chemical properties (viscosity, density and surface tension, all functions of temperature), with drops radii at production from 0.1 to 500 µm. Next, we integrate over the bubble size distribution entrained by breaking waves. Finally, the sea spray generation function is obtained by considering the volume flux of entrained bubbles due to breaking waves in the field constrained by the third moment of the breaking distribution (akin to the whitecap coverage). This mechanistic approach naturally integrates the role of wind and waves via the breaking distribution and entrained air flux, and a sensitivity to temperature via individual bubble bursting mechanisms. The resulting sea spray generation function has not been tuned or adjusted to match any existing data sets, in terms of magnitude of sea salt emissions and recently observed temperature dependencies. The remarkable coherence between the model and observations of sea salt emissions therefore strongly supports the mechanistic approach and the resulting sea spray generation function.

     
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  4. Air bubbles at the surface of water end their life in a particular way: when bursting, they may eject drops of liquid in the surrounding environment. Many uncertainties remain regarding collective effects of bubbles at the water–air interface, despite extensive efforts to describe the bursting mechanisms, motivated by their critical importance in mass transfers between the ocean and the atmosphere in the production of sea spray aerosols. We investigate the effect of surfactant on the collective dynamics and statistics of air bubbles evolving freely at the surface of water, through an experimental set-up controlling the bulk distribution of bubbles with nearly monodisperse millimetric air bubbles. We observe that for low contamination, bubble coalescence is inevitable and leads to a broad surface size distribution. For higher surfactant concentrations, coalescence at the surface is prevented and bubble lifetime is increased, leading to the formation of rafts with a surface size distribution identical to the bulk distribution. This shows that surface contamination has a first-order influence on the transfer function from bulk size distribution to surface size distribution, an intermediate step which needs to be considered when developing sea spray source function as droplet production by bubble bursting depends on the bubble size. We measure the bursting and merging rates of bubbles as a function of contamination through a complementary freely decaying raft experiment. We propose a cellular automaton model that includes the minimal ingredients to reproduce the experimental results in the statistically stationary configuration: production, coalescence and bursting after a finite lifetime. 
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  5. Abstract

    Gas bubbles bursting at the sea surface produce drops, which contribute to marine aerosols. The contamination or enrichment of water by surface‐active agents, of biological or anthropogenic origin, has long been recognized as affecting the bubble bursting processes and the spray composition. However, despite an improved understanding of the physics of a single bursting event, a quantitative understanding of the role of the physico‐chemical conditions on assemblies of bursting bubbles remains elusive. We present experiments on the drop production by millimetric, collective bursting bubbles, under varying surfactant concentration and bubble density. We demonstrate that the production of supermicron droplets (with radius larger than 35 μm) is non‐monotonic as the surfactant concentration increases. The bursting efficiency is optimal for short‐lived, sparsely distributed and non‐coalescing bubbles. We identify the combined role of contamination on the surface bubble arrangement and the modification of the jet drop production process in the bursting efficiency.

     
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  6. Abstract

    Laboratory measurements of droplet size, velocity, and accelerations generated by mechanically and wind‐forced water breaking waves are reported. The wind free stream velocity is up to 12 m/s, leading to wave slopes from 0.15 to 0.35 at a fetch of 23 m. The ratio of wind free stream and wave phase speed ranges from 5.9 to 11.1, depending on the mechanical wave frequency. The droplet size distribution in all configurations can be represented by two power laws,N(d) ∝ d−1for drops from 30 to 600 μm andN(d) ∝ d−4above 600 μm. The horizontal and vertical droplet velocities appear correlated, with drops with slower horizontal speed more likely to move upward. The velocity and acceleration distributions are found to be asymmetric, with the velocity probability density functions (PDFs) being described by a normal‐inverse‐Gaussian distribution. The horizontal acceleration PDF are found to follow a shape close to the one predicted for small particles in homogeneous and isotropic turbulence, while the vertical distribution follows an asymmetric normal shape, showing that both acceleration components are controlled by different physical processes.

     
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