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Acoustic levitation in air provides a containerless, gravity-free platform for investigating driven many-particle systems with nonconservative interactions and underdamped dynamics. In prior work the interactions among levitated particles were limited to attractive forces from scattered sound and repulsion from hydrodynamic microstreaming. We report on experiments in which contact cohesion provides a third type of interaction. When particle size and separation are both much smaller than the sound wavelength, this interplay of three interactions results in forces that are attractive over several particle diameters, become repulsive at close approach, and are again attractive at contact. In the presence of sound-induced athermal fluctuations that generate particle collisions, the interplay of these three forces enables the formation of particle chains with anisotropic interactions that depend on chain size and shape due to multibody effects. With the control of the kinetic pathways and the strength of the contact cohesion, different patterns can be assembled, from triangular lattices to labyrinthine patterns of chains to lacelike networks of interconnected rings. These results shed light on the multibody character of acoustic interactions and can be utilized to direct the self-assembly of particles. Published by the American Physical Society2025 

Abstract Millions of people a year receive magnetic resonance imaging (MRI) contrast agents for the diagnosis of conditions as diverse as fatty liver disease and cancer. Gadolinium chelates, which provide preferredT₁contrast, are the current standard but face an uncertain future due to increasing concerns about their nephrogenic toxicity as well as poor performance in high‐field MRI scanners. Gadolinium‐containing nanocrystals are interesting alternatives as they bypass the kidneys and can offer the possibility of both intracellular accumulation and active targeting. Nanocrystal contrast performance is notably limited, however, as their organic coatings block water from close interactions with surface Gadoliniums. Here, these steric barriers to water exchange are minimized through shape engineering of plate‐like nanocrystals that possess accessible Gadoliniums at their edges. Sulfonated surface polymers promote second‐sphere relaxation processes that contribute remarkable contrast even at the highest fields (r₁= 32.6 × 10⁻³mGd⁻¹s⁻¹at 9.4 T). These noncytotoxic materials release no detectable free Gadolinium even under mild acidic conditions. They preferentially accumulate in the liver of mice with a circulation half‐life 50% longer than commercial agents. These features allow theseT₁MRI contrast agents to be applied for the first time to the ex vivo detection of nonalcoholic fatty liver disease in mice.