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Abstract The late Ediacaran to early Cambrian witnessed significant Earth system changes, including animal life diversification and an enigmatic paleomagnetic record. This study focuses on the Nama Group, a key geological unit for understanding the Ediacaran‐Cambrian transition. Previous paleomagnetic studies in the Nama Group identified complex remagnetization patterns but lacked a detailed examination of remanence carriers. To address this, we conducted a series of rock magnetic experiments on unweathered borehole core samples to better constrain the remagnetization mechanisms. Thermal demagnetization identified two magnetic components.C₁, a recent viscous remanent magnetization, used for borehole core orientation, andC₂, a stable remagnetization component carried by single‐domain (SD) pyrrhotite and magnetite. Magnetic mineralogy and paleomagnetic data suggest that the remanence acquisition mechanism ofC₂is best explained by thermoviscous remanent magnetization (TVRM) and thermal remanent magnetization (TRM), rather than chemical remanent magnetization (CRM). The presence of low unblocking temperatures, coupled with thermochronological evidence of prolonged heating during tectonic collisions and subsequent cooling, supports this interpretation. The remagnetization event is linked to the final consolidation of West Gondwanaland during the late stages of megacontinent assembly (∼490–480 Ma), coinciding with regional uplift and a stable geomagnetic field during the Moyero reverse superchron. These findings challenge the CRM hypothesis, as the quasi‐synchronous remagnetization across cratonic blocks and the predominance of single reverse polarity are better explained by thermal processes. This study highlights the critical role of thermoviscous relaxation in large‐scale remagnetization and provides new insights into the tectonic evolution of West Gondwanaland.