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  1. We report on the use of extreme ultraviolet (XUV, 30.3 nm) radiation from the Free-electron LASer in Hamburg (FLASH) and visible (Vis, 405 nm) photons from an optical laser to investigate the relaxation and fragmentation dynamics of fluorene ions. The ultrashort laser pulses allow to resolve the molecular processes occurring on the femtosecond timescales. Fluorene is a prototypical small polycyclic aromatic hydrocarbon (PAH). Through their infrared emission signature, PAHs have been shown to be ubiquitous in the universe, and they are assumed to play an important role in the chemistry of the interstellar medium. Our experiments track the ionization and dissociative ionizationmore »products of fluorene through time-of-flight mass spectrometry and velocity-map imaging. Multiple processes involved in the formation of each of the fragment ions are disentangled through analysis of the ion images. The relaxation lifetimes of the excited fluorene monocation and dication obtained through the fragment formation channels are reported to be in the range of a few tens of femtoseconds to a few picoseconds.« less
    Free, publicly-accessible full text available May 12, 2023
  2. Abstract Polycyclic aromatic hydrocarbons (PAHs) play an important role in interstellar chemistry and are subject to high energy photons that can induce excitation, ionization, and fragmentation. Previous studies have demonstrated electronic relaxation of parent PAH monocations over 10–100 femtoseconds as a result of beyond-Born-Oppenheimer coupling between the electronic and nuclear dynamics. Here, we investigate three PAH molecules: fluorene, phenanthrene, and pyrene, using ultrafast XUV and IR laser pulses. Simultaneous measurements of the ion yields, ion momenta, and electron momenta as a function of laser pulse delay allow a detailed insight into the various molecular processes. We report relaxation times formore »the electronically excited PAH * , PAH +* and PAH 2+* states, and show the time-dependent conversion between fragmentation pathways. Additionally, using recoil-frame covariance analysis between ion images, we demonstrate that the dissociation of the PAH 2+ ions favors reaction pathways involving two-body breakup and/or loss of neutral fragments totaling an even number of carbon atoms.« less
    Free, publicly-accessible full text available December 1, 2022
  3. Abstract The ATLAS experiment at the Large Hadron Collider has a broad physics programme ranging from precision measurements to direct searches for new particles and new interactions, requiring ever larger and ever more accurate datasets of simulated Monte Carlo events. Detector simulation with Geant4 is accurate but requires significant CPU resources. Over the past decade, ATLAS has developed and utilized tools that replace the most CPU-intensive component of the simulation—the calorimeter shower simulation—with faster simulation methods. Here, AtlFast3, the next generation of high-accuracy fast simulation in ATLAS, is introduced. AtlFast3 combines parameterized approaches with machine-learning techniques and is deployed tomore »meet current and future computing challenges, and simulation needs of the ATLAS experiment. With highly accurate performance and significantly improved modelling of substructure within jets, AtlFast3 can simulate large numbers of events for a wide range of physics processes.« less
    Free, publicly-accessible full text available December 1, 2023
  4. Free, publicly-accessible full text available May 1, 2023
  5. Free, publicly-accessible full text available May 1, 2023
  6. Abstract The energy response of the ATLAS calorimeter is measured for single charged pions with transverse momentum in the range $$10more »situ single-particle measurements. The calorimeter response to single-pions is observed to be overestimated by $${\sim }2\%$$ ∼ 2 % across a large part of the $$p_{\text {T}}$$ p T spectrum in the central region and underestimated by $${\sim }4\%$$ ∼ 4 % in the endcaps in the ATLAS simulation. The uncertainties in the measurements are $${\lesssim }1\%$$ ≲ 1 % for $$15« less
    Free, publicly-accessible full text available March 1, 2023
  7. A bstract Searches are conducted for new spin-0 or spin-1 bosons using events where a Higgs boson with mass 125 GeV decays into four leptons ( ℓ = e , μ ). This decay is presumed to occur via an intermediate state which contains two on-shell, promptly decaying bosons: H → XX/ZX → 4 ℓ , where the new boson X has a mass between 1 and 60 GeV. The search uses pp collision data collected with the ATLAS detector at the LHC with an integrated luminosity of 139 fb − 1 at a centre-of-mass energy $$ \sqrt{s} $$ smore »= 13 TeV. The data are found to be consistent with Standard Model expectations. Limits are set on fiducial cross sections and on the branching ratio of the Higgs boson to decay into XX/ZX , improving those from previous publications by a factor between two and four. Limits are also set on mixing parameters relevant in extensions of the Standard Model containing a dark sector where X is interpreted to be a dark boson.« less
    Free, publicly-accessible full text available March 1, 2023
  8. Abstract This paper presents a measurement of the electroweak production of two jets in association with a $$Z\gamma $$ Z γ pair, with the Z boson decaying into two neutrinos. It also presents a search for invisible or partially invisible decays of a Higgs boson with a mass of 125  $$\text {GeV}$$ GeV produced through vector-boson fusion with a photon in the final state. These results use data from LHC proton–proton collisions at $$\sqrt{s}$$ s = 13  $$\text {TeV}$$ TeV collected with the ATLAS detector and corresponding to an integrated luminosity of 139  $$\hbox {fb}^{-1}$$ fb - 1 . Themore »event signature, shared by all benchmark processes considered for the measurements and searches, is characterized by a significant amount of unbalanced transverse momentum and a photon in the final state, in addition to a pair of forward jets. Electroweak $$Z\gamma $$ Z γ production in association with two jets is observed in this final state with a significance of 5.2 (5.1 expected) standard deviations. The measured fiducial cross-section for this process is $$1.31\pm 0.29$$ 1.31 ± 0.29  fb. An observed (expected) upper limit of 0.37 ( $$0.34^{+0.15}_{-0.10}$$ 0 . 34 - 0.10 + 0.15 ) at 95% confidence level is set on the branching ratio of a 125  $$\text {GeV}$$ GeV Higgs boson to invisible particles, assuming the Standard Model production cross-section. The signature is also interpreted in the context of decays of a Higgs boson into a photon and a dark photon. An observed (expected) 95% CL upper limit on the branching ratio for this decay is set at 0.018 ( $$0.017^{+0.007}_{-0.005}$$ 0 . 017 - 0.005 + 0.007 ), assuming the Standard Model production cross-section for a 125  $$\text {GeV}$$ GeV Higgs boson.« less
    Free, publicly-accessible full text available February 1, 2023
  9. Abstract During LHC Run 2 (2015–2018) the ATLAS Level-1 topological trigger allowed efficient data-taking by the ATLAS experiment at luminosities up to 2.1 $$\times $$ × 10 $$^{34}$$ 34  cm $$^{-2}$$ - 2 s $$^{-1}$$ - 1 , which exceeds the design value by a factor of two. The system was installed in 2016 and operated in 2017 and 2018. It uses Field Programmable Gate Array processors to select interesting events by placing kinematic and angular requirements on electromagnetic clusters, jets, $$\tau $$ τ -leptons, muons and the missing transverse energy. It allowed to significantly improve the background event rejection andmore »signal event acceptance, in particular for Higgs and B -physics processes.« less
    Free, publicly-accessible full text available January 1, 2023