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Lead-208 is the heaviest known doubly magic nucleus and its structure is therefore of special interest. Despite this magicity, which acts to provide a strong restorative force toward sphericity, it is known to exhibit both strong octupole correlations and some of the strongest quadrupole collectivity observed in doubly magic systems. In this Letter, we employ state-of-the-art experimental equipment to conclusively demonstrate, through four Coulomb-excitation measurements, the presence of a large, negative, spectroscopic quadrupole moment for both the vibrational octupole $3_1^{-}$and quadrupole $2_1^{+}$state, indicative of a preference for prolate deformation of the states. The observed quadrupole moment is discussed in the context of the expected splitting of the $3^{-}\otimes 3^{-}$two-phonon states, due to the coupling of the quadrupole and octupole motion. These results are compared with theoretical values from three different methods, which are unable to reproduce both the sign and magnitude of this deformation. Thus, in spite of its well-studied nature, ${}^{208}\mathrm{Pb}$remains a puzzle for our understanding of nuclear structure. Published by the American Physical Society2025 

We used the 138Baðd; αÞ reaction to carry out an in-depth study of states in 136Cs, up to around 2.5 MeV. In this Letter, we place emphasis on hitherto unobserved states below the first 1þ level, which are important in the context of solar neutrino and fermionic dark matter (FDM) detection in large-scale xenon-based experiments. We identify for the first time candidate metastable states in 136Cs, which would allow a realtime detection of solar neutrino and FDM events in xenon detectors, with high background suppression. Our results are also compared with shell-model calculations performed with three Hamiltonians that were previously used to evaluate the nuclear matrix element (NME) for 136Xe neutrinoless double beta decay.We find that one of these Hamiltonians, which also systematically underestimates the NME compared with the others, dramatically fails to describe the observed low-energy 136Cs spectrum, while the other two show reasonably good agreement.